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SERS‐Active MIL‐100(Fe) Sensory Array for Ultrasensitive and Multiplex Detection of VOCs

Jinghao Fu、Zhen Zhong、Dan Xie 等 10 位作者2020-08-03Angewandte Chemie

Abstract The application of metal–organic frameworks (MOFs) as SERS‐active platforms in multiplex volatile organic compounds (VOCs) detection is still unexplored. Herein, we demonstrate that MIL‐100 (Fe) serves as an ideal SERS substrate for the detection of VOCs. The limit of detection (LOD) of MIL‐100(Fe) for toluen…

Gas Sensing Nanomaterials and SensorsMolecular Sensors and Ion DetectionAdvanced Nanomaterials in Catalysis

Construction of Interpenetrating Transport Channels and Compatible Interfaces via a Zeolitic Imidazolate Framework “Bridge” for Nanofibrous Hybrid PEMs with Enhanced Proton Conduction and Methanol Resistance

Liyuan Wang、Nanping Deng、Gang Wang 等 7 位作者2020-08-03ACS Sustainable Chemistry & Engineering

A novel three-dimensional sulfonated poly(ether sulfone) (SPES) nanofiber@ZIF-8 network (ZSNF) with an interlaced structure was designed and prepared by an in situ assembling zeolitic imidazolate framework-8 (ZIF-8) shell on electrospun SPES nanofiber surfaces. By incorporating ZSNFs into the Nafion matrix, highly com…

Fuel Cells and Related MaterialsConducting polymers and applicationsAdvanced Battery Technologies Research

Frozen patterns of impacted droplets: From conical tips to toroidal shapes

Man Hu、Feng Wang、Qian Tao 等 6 位作者2020-08-03Physical Review Fluids

We report frozen patterns for the water droplets impacting on a cold substrate through fast-speed images. These patterns can be manipulated by several physical parameters (the droplet size, falling height, and substrate temperature), and the scaling analysis has a remarkable agreement with the phase diagram. The obser…

Surface Modification and SuperhydrophobicityFluid Dynamics and Heat TransferFluid Dynamics Simulations and Interactions

The 3D-Printed Bilayer’s Bioactive-Biomaterials Scaffold for Full-Thickness Articular Cartilage Defects Treatment

Kittiya Thunsiri、Siwasit Pitjamit、Peraphan Pothacharoen 等 6 位作者2020-08-03Materials

The full-thickness articular cartilage defect (FTAC) is an abnormally severe grade of articular cartilage (AC) injury. An osteochondral autograft transfer (OAT) is the recommended treatment, but the increasing morbidity rate from osteochondral plug harvesting is a limitation. Thus, the 3D-printed bilayer's bioactive-b…

Bone Tissue Engineering MaterialsOsteoarthritis Treatment and MechanismsSilk-based biomaterials and applications

Regulating Electronic Status of Platinum Nanoparticles by Metal–Organic Frameworks for Selective Catalysis

Yu Shen、Ting Pan、Peng Wu 等 13 位作者2020-08-03CCS Chemistry

Open AccessCCS ChemistryRESEARCH ARTICLE1 May 2021Regulating Electronic Status of Platinum Nanoparticles by Metal–Organic Frameworks for Selective Catalysis Yu Shen†, Ting Pan†, Peng Wu, Jiawei Huang, Hongfeng Li, Islam E. Khalil, Sheng Li, Bing Zheng, Jiansheng Wu, Qiang Wang, Weina Zhang, Wei David Wei and Fengwei H…

Metal-Organic Frameworks: Synthesis and ApplicationsCatalytic Processes in Materials ScienceNanomaterials for catalytic reactions

Many-body reactive force field development for carbon condensation in C/O systems under extreme conditions

Rebecca Lindsey、Nir Goldman、Laurence E. Fried 等 4 位作者2020-08-03The Journal of Chemical Physics

We describe the development of a reactive force field for C/O systems under extreme temperatures and pressures, based on the many-body Chebyshev Interaction Model for Efficient Simulation (ChIMES). The resulting model, which targets carbon condensation under thermodynamic conditions of 6500 K and 2.5 g cm−3, affords a…

Advanced Chemical Physics StudiesHigh-pressure geophysics and materialsMachine Learning in Materials Science

Fabrication of flexible self-powered humidity sensor based on super-hydrophilic titanium oxide nanotube arrays

Elham Farahani、Raheleh Mohammadpour2020-08-03Scientific Reports

Abstract Stable and flexible super-hydrophilic nanotubular-based titanium oxide electrode has been utilized as the active electrode of self-powered humidity sensor. TiO2 nanotubular electrodes fabricated through anodization method and utilized in combination with Kapton electrode as the triboelectric nanogenerator (TE…

Advanced Sensor and Energy Harvesting MaterialsGas Sensing Nanomaterials and SensorsConducting polymers and applications

Deep learning on the 2-dimensional Ising model to extract the crossover region with a variational autoencoder

Nicholas Walker、Ka-Ming Tam、Mark Jarrell2020-08-03Scientific Reports

The 2-dimensional Ising model on a square lattice is investigated with a variational autoencoder in the non-vanishing field case for the purpose of extracting the crossover region between the ferromagnetic and paramagnetic phases. The encoded latent variable space is found to provide suitable metrics for tracking the…

Theoretical and Computational PhysicsQuantum many-body systemsMachine Learning in Materials Science

Silicon Nanowires and Their Impact on Cancer Detection and Monitoring

Rasheid Smith、Sean M. Geary、Aliasger K. Salem2020-08-03ACS Applied Nano Materials

Since the inception of silicon nanowires (SINWs)-based biosensors in 2001, SINWs employed in various detection schemes have routinely demonstrated label-free, real-time, sub femtomolar detection of both protein and nucleic acid analytes. This has allowed SiNW-based biosensors to integrate into the field of cancer dete…

Advanced biosensing and bioanalysis techniquesNanowire Synthesis and ApplicationsAnodic Oxide Films and Nanostructures

Improved Quantum Efficiency by Advanced Light Management in Nanotextured Solution-Processed Perovskite Solar Cells

Philipp Tockhorn、Johannes Sutter、Rémi Colom 等 11 位作者2020-08-03ACS Photonics

High Resolution Image Download MS PowerPoint Slide Light management strategies can increase the efficiency of perovskite single-junction and tandem solar cells. In this study, we present perovskite solar cells deposited on different shallow nanotextures by spin-coating. A morphological and optoelectronic analysis demo…

Perovskite Materials and ApplicationsChalcogenide Semiconductor Thin FilmsConducting polymers and applications

Electrostatic Conjugation of Nanoparticle Surfaces with Functional Peptide Motifs

Natalie Boehnke、Kate J. Dolph、Valeria M. Juarez 等 5 位作者2020-08-03Bioconjugate Chemistry

We report the surface functionalization of anionic layer by layer nanoparticles (LbL NPs) with cationic tumor-penetrating peptides (TPPs) via electrostatic adsorption while retaining particle stability and charge characteristics. This strategy eliminates the need for structural modifications of the peptide and enables…

Nanoparticle-Based Drug DeliveryAdvanced biosensing and bioanalysis techniquesPolymer Surface Interaction Studies

Recent Advances in the Construction of Flexible Sensors for Biomedical Applications

Nan Zhou、Tianjiao Liu、Bianying Wen 等 6 位作者2020-08-03Biotechnology Journal

The fabrication of flexible sensors is a potential way to promote the progress of modern social science and technology due to their wide applications in high-performance electronic equipment and devices. Flexible sensors based on organic materials combine the unique advantages of flexibility and low cost, increasing i…

Advanced Sensor and Energy Harvesting MaterialsConducting polymers and applicationsNanowire Synthesis and Applications

Electrochemical Denitrification and Oxidative Dehydrogenation of Ethylbenzene over N-doped Mesoporous Carbon: Atomic Level Understanding of Catalytic Activity by 15N NMR Spectroscopy

Ireneusz Szewczyk、Anna Rokicińska、Marek Michalík 等 10 位作者2020-08-03Chemistry of Materials

Abstract Spherical mesoporous carbon (with a particle size in the range of 40?75 ?m) was synthesized by nanoreplication of a hard silica template using sucrose as the carbon precursor. The mesoporous carbon with BET surface areas higher than 1200 m2/g was doped with N by a treatment in an aqueous solution of nitric ac…

Metal-Organic Frameworks: Synthesis and ApplicationsCatalytic Processes in Materials ScienceAmmonia Synthesis and Nitrogen Reduction

Transparent and UV Blocking Structural Colored Hydrogel for Contact Lenses

Xiuqing Shen、Jiayuan Du、Jiaxin Sun 等 6 位作者2020-08-03ACS Applied Materials & Interfaces

Usually, materials with perfect structures possess excellent properties, but it is not always the case. Here, a new approach is reported to construct structural colored hydrogel films with excellent ultraviolet (UV) blocking performance for contact lenses. The theoretical simulation predicts that with perfect periodic…

Liquid Crystal Research AdvancementsPhotonic Crystals and ApplicationsOcular Surface and Contact Lens

Scopy: an integrated negative design python library for desirable HTS/VS database design

Ziyi Yang、Zhijiang Yang、Aiping Lü 等 5 位作者2020-08-03Briefings in Bioinformatics

BACKGROUND: High-throughput screening (HTS) and virtual screening (VS) have been widely used to identify potential hits from large chemical libraries. However, the frequent occurrence of 'noisy compounds' in the screened libraries, such as compounds with poor drug-likeness, poor selectivity or potential toxicity, has…

Computational Drug Discovery MethodsMachine Learning in Materials ScienceCell Image Analysis Techniques

Incorporation of Alkali-Activated Municipal Solid Waste Incinerator Bottom Ash in Mortar and Concrete: A Critical Review

Rawaz Kurda、Rui V. Silva、Jorge de Brito2020-08-03Materials

In the light of one of the most common waste management issues in urban areas, namely the elimination of municipal solid waste (MSW; about 486 kg of the waste per capita were generated in the EU in 2017), this study discusses one technique as an outlet in the construction industry for the by-product of the waste's inc…

Concrete and Cement Materials ResearchRecycling and utilization of industrial and municipal waste in materials productionMagnesium Oxide Properties and Applications

Highly Ordered Nanoporous Carbon Scaffold with Controllable Wettability as the Microporous Layer for Fuel Cells

Muhammad Naoshad Islam、Udit N. Shrivastava、Marwa Atwa 等 6 位作者2020-08-03ACS Applied Materials & Interfaces

We introduce a novel self-standing, nanoporous carbon scaffold (NCS, 25 μm thick), with an ordered inverse opal pore structure (∼85 nm pore) as a microporous layer (MPL) in a polymer electrolyte membrane fuel cell. Unlike previous studies, through chemical functionalization of the pore surfaces, the wettability of the…

Electrocatalysts for Energy ConversionSupercapacitor Materials and FabricationFuel Cells and Related Materials

as-Indaceno[3,2,1,8,7,6-ghijklm]terrylene as a near-infrared absorbing C70-fragment

Yuki Tanaka、Norihito Fukui、Hiroshi Shinokubo2020-08-03Nature Communications

Abstract Carbon and hydrogen are fundamental components of organic molecules and a fascinating plethora of functions can be generated using these two elements. Yet, realizing attractive electronic structures only by using carbon and hydrogen remains challenging. Herein, we report the synthesis and properties of the C…

Graphene research and applicationsFullerene Chemistry and ApplicationsSynthesis and Properties of Aromatic Compounds

Stability, Reduction, and Cytotoxicity of Platinum(IV) Anticancer Prodrugs Bearing Carbamate Axial Ligands: Comparison with Their Carboxylate Analogues

Shu Chen、Houzong Yao、Qiyuan Zhou 等 6 位作者2020-08-03Inorganic Chemistry

Platinum(IV) complexes containing carboxylate and carbamate ligands at the axial position have been reported previously. A better understanding of the similarity and difference between the two types of ligands will provide us with new insights and more choices to design novel Pt(IV) complexes. In this study, we system…

Metal complexes synthesis and propertiesNanocluster Synthesis and ApplicationsFerrocene Chemistry and Applications

Fracture of magnesium matrix nanocomposites - A review

Xiao Song、Parisa Bayati、Manoj Gupta 等 5 位作者2020-08-03International Journal of Lightweight Materials and Manufacture

As one of the lightest metallic materials, magnesium is considered as a promising replacement for aluminum, titanium, and steel. However, lightweight energy-saving magnesium and magnesium alloys suffer from poor ductility (5%–8%) due to their hexagonal closed packed crystalline structure and a limited number of easily…

Magnesium Alloys: Properties and ApplicationsAluminum Alloys Composites PropertiesMXene and MAX Phase Materials