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Enhanced Passivation and Carrier Collection in Ink-Processed PbS Quantum Dot Solar Cells via a Supplementary Ligand Strategy

Xiaokun Yang、Ji Yang、Muhammad Ullah 等 10 位作者2020-08-03ACS Applied Materials & Interfaces

Solution-processed semiconductors have opened promising avenues for next-generation semiconductor and optoelectronic industries. Colloidal quantum dots (QDs) as one of the most typical materials are widely utilized for the design and development of light-emitting diodes, photodetectors, and solar cells. Recently, an e…

Perovskite Materials and ApplicationsQuantum Dots Synthesis And PropertiesChalcogenide Semiconductor Thin Films

Acoustic phonon recycling for photocarrier generation in graphene-WS2 heterostructures

Ke Wei、Yizhen Sui、Zhongjie Xu 等 12 位作者2020-08-03Nature Communications

Abstract Electron-phonon scattering is the key process limiting the efficiency of modern nanoelectronic and optoelectronic devices, in which most of the incident energy is converted to lattice heat and finally dissipates into the environment. Here, we report an acoustic phonon recycling process in graphene-WS 2 hetero…

Graphene research and applications2D Materials and ApplicationsThermal properties of materials

Accelerating Crystallization of Open Organic Materials by Poly(ionic liquid)s

Suyun Zhang、H. Miao、Hemin Zhang 等 9 位作者2020-08-03Angewandte Chemie International Edition

The capability to significantly shorten the synthetic period of a broad spectrum of open organic materials presents an enticing prospect for materials processing and applications. Herein we discovered 1,2,4-triazolium poly(ionic liquid)s (PILs) could serve as a universal additive to accelerate by at least one order of…

Metal-Organic Frameworks: Synthesis and ApplicationsLuminescence and Fluorescent MaterialsCovalent Organic Framework Applications

Steric Engineering of Cyclometalated Pt(II) Complexes toward High-Contrast Monomer–Excimer-Based Mechanochromic and Vapochromic Luminescence

Chen‐Yu Lien、Ying‐Feng Hsu、Yi‐Hung Liu 等 6 位作者2020-08-03Inorganic Chemistry

Ligands play a crucial role in the supramolecular photoluminescence properties of Pt(II) square-planar complexes. To improve the luminescence color responses of N∧C∧N cyclometalated Pt(II) complexes to external stimuli such as mechanical stress and chemical vapors, we have conducted a steric engineering of the previou…

Organic Light-Emitting Diodes ResearchLuminescence and Fluorescent MaterialsSynthesis and Reactivity of Heterocycles

Narrow-Linewidth Tin-Vacancy Centers in a Diamond Waveguide

Alison E. Rugar、Constantin Dory、Shahriar Aghaeimeibodi 等 9 位作者2020-08-03ACS Photonics

Integrating solid-state quantum emitters with photonic circuits is essential for realizing large-scale quantum photonic processors. Negatively charged tin-vacancy (SnV – ) centers in diamond have emerged as promising candidates for quantum emitters because of their excellent optical and spin properties, including narr…

Diamond and Carbon-based Materials ResearchMechanical and Optical ResonatorsNonlinear Optical Materials Studies

Conductive Polyacrylic Acid-Polyaniline as a Multifunctional Binder for Stable Organic Quinone Electrodes of Lithium-Ion Batteries

Jing Tong、Cuiping Han、Xiaorui Hao 等 5 位作者2020-08-03ACS Applied Materials & Interfaces

High solubility in aprotic organic electrolytes and poor electrical conductivity are the main restrictions of organic electrodes in practical application. Conductive binder contributes to the high-performance electrodes as it enables both mechanical and electronic integrity of the electrode, which have been scarcely e…

Advancements in Battery MaterialsAdvanced Battery Materials and TechnologiesConducting polymers and applications

Estimation of Particle Size and Band Gap of Zinc Oxide Nanoparticle Synthesized by Chemical Precipitation Method

Surendra Kumar Gautam、Bibek Sapkota、Arun Bhujel 等 4 位作者2020-08-03Journal of Nepal Chemical Society

Zinc oxide (ZnO) nanoparticles were synthesized by chemical precipitation method using 0.1M and 0.3M [Zn(NO3)2.6H2O] and Na2CO3 solutions. The particle size and band gap of ZnO nanoparticles were estimated and effect of concentration on it was investigated. The synthesized nanoparticles were characterized by X-ray dif…

ZnO doping and properties

Room-temperature quantum spin Hall phase in laser-patterned few-layer 1T′- MoS2

Naoki Katsuragawa、Mizuki Nishizawa、Taketomo Nakamura 等 9 位作者2020-08-03Communications Materials

Abstract The quantum-spin-Hall (QSH) phase of 2D topological insulators has attracted increased attention since the onset of 2D materials research. While large bulk gaps with vanishing edge gaps in atomically thin layers have been reported, verifications of the QSH phase by resistance measurements are comparatively fe…

2D Materials and ApplicationsTopological Materials and PhenomenaChemical and Physical Properties of Materials

Paraelectric/antiferroelectric/ferroelectric phase transformation in As-deposited ZrO2 thin films by the TiN capping engineering

Chunyuan Wang、Chin-I Wang、Sheng‐Han Yi 等 8 位作者2020-08-03Materials & Design

Based on the engineering of the TiN capping layer, the tailoring of the crystalline phases and the paraelectric(PE)/antiferroelectric(AFE)/ferroelectric(FE) properties of nanoscale ZrO2 thin films are demonstrated without any post-annealing treatment. The capping by the TiN layer leads to the conversion of ZrO2 from t…

Ferroelectric and Piezoelectric MaterialsAcoustic Wave Resonator TechnologiesFerroelectric and Negative Capacitance Devices

Glycerin/NaOH Aqueous Solution as a Green Solvent System for Dissolution of Cellulose

Ke Li、Huiyu Yang、Lang Jiang 等 8 位作者2020-08-03Polymers

Dissolving cellulose in water-based green solvent systems is highly desired for further industrial applications. The green solvent glycerin—which contains hydrogen-bonding acceptors—was used together with NaOH and water to dissolve cellulose. This mixed aqueous solution of NaOH and glycerin was employed as the new gre…

Biofuel production and bioconversionAdvanced Cellulose Research StudiesCatalysis for Biomass Conversion

Prospects for microwave plasma synthesized N-graphene in secondary electron emission mitigation applications

N. Bundaleska、Ana Dias、Nenad Bundaleski 等 17 位作者2020-08-03Scientific Reports

The ability to change the secondary electron emission properties of nitrogen-doped graphene (N-graphene) has been demonstrated. To this end, a novel microwave plasma-enabled scalable route for continuous and controllable fabrication of free-standing N-graphene sheets was developed. High-quality N-graphene with prescri…

Graphene research and applicationsSemiconductor materials and devicesDiamond and Carbon-based Materials Research

Growth of α- and β-Ga 2 O 3 epitaxial layers on sapphire substrates using liquid-injection MOCVD

Fridrich Egyenes、Filip Gucmann、K. Hušeková 等 8 位作者2020-08-03Semiconductor Science and Technology

Abstract Ga 2 O 3 , a wide-bandgap semiconductor material, offers a great potential for power and high-voltage electronic devices. We report on the growth of undoped α - and β -phase Ga 2 O 3 using liquid-injection metal-organic chemical vapor deposition (LI-MOCVD) on sapphire substrates. Using the same precursor (gal…

Advanced Photocatalysis TechniquesZnO doping and propertiesGa2O3 and related materials

Dielectric response with short-ranged electrostatics

Stephen J. Cox2020-08-03Proceedings of the National Academy of Sciences

The dielectric nature of polar liquids underpins much of their ability to act as useful solvents, but its description is complicated by the long-ranged nature of dipolar interactions. This is particularly pronounced under the periodic boundary conditions commonly used in molecular simulations. In this article, the die…

Material Dynamics and PropertiesForce Microscopy Techniques and ApplicationsSpectroscopy and Quantum Chemical Studies

Sustainable Development of Enhanced Luminescence Polymer-Carbon Dots Composite Film for Rapid Cd2+ Removal from Wastewater

Mohammed Issa、Zurina Zainal Abidin2020-08-03Molecules

As a remedy for environmental pollution, a versatile synthetic approach has been developed to prepare polyvinyl alcohol (PVA)/nitrogen-doped carbon dots (CDs) composite film (PVA-CDs) for removal of toxic cadmium ions. The CDs were first synthesized using carboxymethylcellulose (CMC) of oil palms empty fruit bunch was…

Mercury impact and mitigation studiesCarbon and Quantum Dots ApplicationsNanocluster Synthesis and Applications

Surface enhanced Raman spectroscopy for bacteria analysis: a review

Elie Akanny、Anne Bonhommé、François Bessueille 等 5 位作者2020-08-03Applied Spectroscopy Reviews

Surface Enhanced Raman spectroscopy (SERS) technique was developed to provide a high enhancement of Raman scattering from molecules adsorbed on nanostructured noble metal surfaces. This technique has gained tremendous interest in the past few years for the detection, identification and quantification of bacteria. Inde…

Gold and Silver Nanoparticles Synthesis and ApplicationsSpectroscopy Techniques in Biomedical and Chemical ResearchBiosensors and Analytical Detection

Two dimensional ferroelectrics: Candidate for controllable physical and chemical applications

Jing Shang、Xiao Tang、Liangzhi Kou2020-08-03Wiley Interdisciplinary Reviews Computational Molecular Science

Abstract The recent emerged two‐dimensional (2D) ferroelectrics have attracted tremendous research interests due to their promising application in nonvolatile electronics devices. The reversible electric polarization of ferroelectrics from the off‐centered positive and negative surfaces can effectively lift the band s…

Ferroelectric and Piezoelectric Materials2D Materials and ApplicationsMultiferroics and related materials

The Effect of Copper Content on the Mechanical and Tribological Properties of Hypo-, Hyper- and Eutectoid Ti-Cu Alloys

Yiku Xu、Jianli Jiang、Zehui Yang 等 6 位作者2020-08-03Materials

Titanium alloys are widely used in aerospace, chemical, biomedical and other important fields due to outstanding properties. The mechanical behavior of Ti alloys depends on microstructural characteristics and type of alloying elements. The purpose of this study was to investigate the effects of different Cu contents (…

Metal and Thin Film MechanicsTitanium Alloys Microstructure and PropertiesAdvanced materials and composites

Ab initio quantum dynamics of charge carriers in graphitic carbon nitride nanosheets

Sraddha Agrawal、Wei Lin、Oleg V. Prezhdo 等 4 位作者2020-08-03The Journal of Chemical Physics

Graphitic carbon nitride (g-C3N4), a metal-free and visible light responsive photocatalyst, has garnered much attention due to its wide range of applications. In order to elucidate the role of dimensionality on the properties of photo-generated charge carriers, we apply nonadiabatic (NA) molecular dynamics combined wi…

Advanced Photocatalysis TechniquesGraphene research and applications2D Materials and Applications

Green Synthesis of Hydrocalumite (CaAl-OH-LDH) from Ca(OH)2 and Al(OH)3 and the Parameters That Influence Its Formation and Speciation

Bianca R. Gevers、Frederick J. W. J. Labuschagné2020-08-03Crystals

Hydrocalumite is a layered double hydroxide (LDH) that is finding increased application in numerous scientific fields. Typically, this material is produced through environmentally polluting methods such as co-precipitation, sol-gel synthesis and urea-hydrolysis. Here, the hydrothermal green (environmentally friendly)…

Layered Double Hydroxides Synthesis and ApplicationsPhosphorus and nutrient managementMagnesium Oxide Properties and Applications

Polymer-Assisted Fabrication of Silver Nanowire Cellular Monoliths: Toward Hydrophobic and Ultraflexible High-Performance Electromagnetic Interference Shielding Materials

Zhihui Zeng、Weiwei Li、Na Wu 等 5 位作者2020-08-03ACS Applied Materials & Interfaces

Metal nanofibers with excellent electrical conductivity and superior mechanical flexibility have great potentials for fabrication of lightweight, flexible, and high-performance electromagnetic interference (EMI) shielding architectures. The weak interactions and large contact resistance among the wires, however, hinde…

Electromagnetic wave absorption materialsAdvanced Antenna and Metasurface Technologies