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Fabrication of Nanoscale Patternable Films of Silk Fibroin Using Benign Solvents

Alessio Bucciarelli、Ramendra K. Pal、Devid Maniglio 等 7 位作者2017-04-20Macromolecular Materials and Engineering

The silk protein fibroin is a wondrous biopolymer widely used to form structures that interface with biological entities. In addition to tissue scaffolds, sponges, and films, biochemically modified fibroins can be used in conjunction with techniques such as photolithography and soft lithography to expand their reperto…

Polymer Surface Interaction StudiesSilk-based biomaterials and applicationsNanofabrication and Lithography Techniques

Design and Experimental Investigation of Thermoelectric Generators for Wearable Applications

Yun Goo Lee、Junsoo Kim、Junsoo Kim 等 14 位作者2017-04-20Advanced Materials Technologies

A critical challenge in using thermoelectric generators (TEGs) for charging the portable or wearable electronics has been their limited outputs, as available temperature differential on human body (∆ T ext ) is typically less than 10 K. Furthermore, the thermal resistance ( R th ) at the TEG–air interface often overwh…

Advanced Thermoelectric Materials and DevicesPerfectionism, Procrastination, Anxiety StudiesThermal Radiation and Cooling Technologies

Physicomechanical, friction, and abrasion properties of EVA/PU blend foams foamed by supercritical nitrogen

Zhen Xiu Zhang、Tao Zhang、Dan Wang 等 6 位作者2017-04-20Polymer Engineering and Science

Elastomer foams based on EVA, PU, and EVA/PU blends formulated for shoe‐sole applications were prepared by a supercritical N 2 batch foaming process and characterized for physicomechanical, friction and abrasion properties. The blending of EVA with PU was aimed for improving the friction and wear characteristics of th…

Polymer crystallization and propertiesTribology and Wear AnalysisPolymer Foaming and Composites

Pure Blue and Highly Luminescent Quantum‐Dot Light‐Emitting Diodes with Enhanced Electron Injection and Exciton Confinement via Partially Oxidized Aluminum Cathode

Tai Cheng、Zhibin Wang、Shengli Jin 等 10 位作者2017-04-20Advanced Optical Materials

The balance injection of holes and electrons into a thin emissive quantum dot (QD) layer for efficient radiative recombination is critical to the color purity, stability, and efficiency of the QD‐based light‐emitting diodes (QD‐LEDs). Due to the difficulty of charge injection into wide band gap blue QD layer, the perf…

Perovskite Materials and ApplicationsQuantum Dots Synthesis And PropertiesChalcogenide Semiconductor Thin Films

Plant-Mediated Synthesis of Au Nanoparticles: Separation and Identification of Active Biomolecule in the Water Extract of Cacumen Platycladi

Hai Liu、Ting Lian、Yang Liu 等 6 位作者2017-04-20Industrial & Engineering Chemistry Research

In order to investigate the roles of active molecules during the bioinspired synthesis process of gold nanoparticles by Cacumen platycladi leaf extract, flash column chromatography was employed to separate the Cacumen platycladi leaf extract according to the polarity differences. Fourier transform infrared spectroscop…

Nanoparticles: synthesis and applicationsGold and Silver Nanoparticles Synthesis and Applications

Broadband and conformal metamaterial absorber

Xiangkun Kong、Junyi Xu、Jinjun Mo 等 4 位作者2017-04-20Frontiers of Optoelectronics

In this study, a new broadband and conformal metamaterial absorber using two flexible substrates was proposed. Simulation results showed that the proposed absorber exhibited an absorption band from 6.08 to 13.04 GHz and a high absorption of 90%, because it was planar. The absorber was broadband as its relative absorpt…

Antenna Design and AnalysisMetamaterials and Metasurfaces ApplicationsAdvanced Antenna and Metasurface Technologies

Abrasion‐Resistant, Hot Water‐Repellent and Self‐Cleaning Superhydrophobic Surfaces Fabricated by Electrophoresis of Nanoparticles in Electrodeposited Sol–Gel Films

Xuefen Zhang、Jipeng Zhao、Ji‐Ming Hu2017-04-20Advanced Materials Interfaces

The present work reports on a new strategy for fabrication of mechanically stable and environmental‐friendly superhydrophobic surfaces. First, a novel cost‐effective approach is developed to synthesize superhydrophobic SiO 2 (SH‐SiO 2 ) nanoparticles at room temperature through the reaction between the surface reactiv…

Surface Modification and SuperhydrophobicityAdvanced Sensor and Energy Harvesting MaterialsPhotonic Crystals and Applications

Error estimates for a fully discretized scheme to a Cahn-Hilliard phase-field model for two-phase incompressible flows

Yongyong Cai、Jie Shen2017-04-20Mathematics of Computation

In this paper, we carry out a rigorous error analysis for a finite-element discretization of the linear, weakly coupled energy stable scheme introduced by Shen and Yang for a Cahn-Hilliard phase-field model of two-phase incompressible flows with matching density.

Aluminum Alloy Microstructure PropertiesSolidification and crystal growth phenomenaFluid Dynamics and Thin Films

Monitoring global protein thiol-oxidation and protein S-mycothiolation in Mycobacterium smegmatis under hypochlorite stress

Mélanie Hillion、Jörg Bernhardt、Tobias Busche 等 12 位作者2017-04-20Scientific Reports

Mycothiol (MSH) is the major low molecular weight (LMW) thiol in Actinomycetes. Here, we used shotgun proteomics, OxICAT and RNA-seq transcriptomics to analyse protein S-mycothiolation, reversible thiol-oxidations and their impact on gene expression in Mycobacterium smegmatis under hypochlorite stress. In total, 58 S-…

Bacterial Genetics and BiotechnologyTrace Elements in HealthEnzyme Structure and Function

Transparent and Gas‐Permeable Liquid Marbles for Culturing and Drug Sensitivity Test of Tumor Spheroids

Hualin Li、Peng Liu、Guneet Kaur 等 5 位作者2017-04-20Advanced Healthcare Materials

Transparent nanoparticle-based liquid marbles with high gas-permeability are prepared to culture tumor spheroids in 3D without the need of supplementary growth factor. The culturing process of spheroids from a population of cancer cells or a single cell in the transparent liquid marbles can be optically recorded conti…

Surface Modification and SuperhydrophobicityPickering emulsions and particle stabilizationBiocrusts and Microbial Ecology

Investigation of the Relationship between the Structure and Conductivity of the Novel Oxide Ionic Conductor Ba3MoNbO8.5

Sacha Fop、Eve J. Wildman、John T. S. Irvine 等 7 位作者2017-04-20Chemistry of Materials

A variable temperature neutron diffraction study of the novel oxide ion conductor Ba 3 MoNbO 8.5 has been performed between 25 and 600 °C. Nonmonotonic behavior of the cell parameters, bond lengths, and angles are observed indicating a structural rearrangement above 300 °C. The oxygen/vacancy distribution changes as t…

Advancements in Solid Oxide Fuel CellsCatalysis and Oxidation ReactionsElectronic and Structural Properties of Oxides

Active Phase of FeOx/Pt Catalysts in Low-Temperature CO Oxidation and Preferential Oxidation of CO Reaction

Hao Chen、Yun Liu、Fan Yang 等 10 位作者2017-04-20The Journal of Physical Chemistry C

The interface between metal and reducible oxide has attracted increasing interest in catalysis. The FeO x –Pt interface has been a typical example, which showed remarkable activity for the preferential oxidation of CO (PROX) at low temperatures. However, model catalytic studies under vacuum conditions or in high-press…

Catalytic Processes in Materials ScienceCatalysts for Methane ReformingCatalysis and Oxidation Reactions

Broadband and Robust Metalens with Nonlinear Phase Profiles for Efficient Terahertz Wave Control

Quanlong Yang、Jianqiang Gu、Yuehong Xu 等 9 位作者2017-04-20Advanced Optical Materials

Metasurfaces, 2D artificial electromagnetic media, open up a new frontier of functional device design ranging from radio waves to the visible region. Particularly, metasurface‐based lenses are indispensable in various practical terahertz applications. The authors aim at achieving flexible and robust metalenses for eff…

Metamaterials and Metasurfaces ApplicationsPlasmonic and Surface Plasmon ResearchMillimeter-Wave Propagation and Modeling

One-Step Fabrication of Non-Fluorinated Transparent Super-Repellent Surfaces with Tunable Wettability Functioning in Both Air and Oil

Mengying Long、Shan Peng、Xiaojun Yang 等 11 位作者2017-04-20ACS Applied Materials & Interfaces

In this paper, we have developed a one-step thermal treatment of polydimethylsiloxane (PDMS) liquid to create transparent super-repellent surface (TSS) and super-repellent powder. They are super-repellent toward water and ethylene glycol. During the one-step thermal treatment, PDMS soot is generated and deposited onto…

Surface Modification and SuperhydrophobicityFluid Dynamics and Heat TransferAdhesion, Friction, and Surface Interactions

Ammonothermal Synthesis of Earth‐Abundant Nitride Semiconductors ZnSiN2 and ZnGeN2 and Dissolution Monitoring by In Situ X‐ray Imaging

Jonas Häusler、Saskia Schimmel、Peter J. Wellmann 等 4 位作者2017-04-20Chemistry - A European Journal

Abstract In this contribution, first synthesis of semiconducting ZnSiN 2 and ZnGeN 2 from solution is reported with supercritical ammonia as solvent and KNH 2 as ammonobasic mineralizer. The reactions were conducted in custom‐built high‐pressure autoclaves made of nickel‐based superalloy. The nitrides were characteriz…

Metal and Thin Film MechanicsSemiconductor materials and devicesMachine Learning in Materials Science

Fed-Batch Synthesis of Poly(3-Hydroxybutyrate) and Poly(3-Hydroxybutyrate-co-4-Hydroxybutyrate) from Sucrose and 4-Hydroxybutyrate Precursors by Burkholderia sacchari Strain DSM 17165

Miguel Miranda de Sousa Dias、Martin Koller、Dario Puppi 等 6 位作者2017-04-20Bioengineering

Based on direct sucrose conversion, the bacterium Burkholderia sacchari is an excellent producer of the microbial homopolyester poly(3-hydroxybutyrate) (PHB). Restrictions of the strain's wild type in metabolizing structurally related 3-hydroxyvalerate (3HV) precursors towards 3HV-containing polyhydroxyalkanoate (PHA)…

Biofuel production and bioconversionEnzyme Catalysis and Immobilizationbiodegradable polymer synthesis and properties

Enhanced optical performance of multifocal metalens with conic shapes

Yanjun Bao、Qiao Jiang、Yimin Kang 等 5 位作者2017-04-20Light Science & Applications

A multifocal metalens, which focuses incident light at multiple foci, has many applications in imaging systems and optical communications. However, the traditional design strategy of a multifocal metalens combines several lenses that have different focal points into a planar integrated unit, resulting in low imaging q…

Metamaterials and Metasurfaces ApplicationsPlasmonic and Surface Plasmon ResearchAdvanced Antenna and Metasurface Technologies

In muro deacetylation of xylan affects lignin properties and improves saccharification of aspen wood

Prashant Mohan‐Anupama Pawar、Marta Derba‐Maceluch、Sun‐Li Chong 等 15 位作者2017-04-20Biotechnology for Biofuels

Lignocellulose from fast growing hardwood species is a preferred source of polysaccharides for advanced biofuels and “green” chemicals. However, the extensive acetylation of hardwood xylan hinders lignocellulose saccharification by obstructing enzymatic xylan hydrolysis and causing inhibitory acetic acid concentration…

Advanced Cellulose Research StudiesPolysaccharides and Plant Cell WallsLignin and Wood Chemistry

Stratification and Size Segregation of Ternary and Polydisperse Colloidal Suspensions during Drying

Andrea Fortini、Richard P. Sear2017-04-20Langmuir

We investigate the drying process of three-component and polydisperse colloidal suspensions using Brownian dynamics simulations. We have previously reported (Phys. Rev. Lett. 2016, 116, 118301) on the drying of binary mixtures. For binary mixtures, we found that a gradient of colloidal osmotic pressure develops during…

Material Dynamics and PropertiesMicrofluidic and Bio-sensing TechnologiesAdvanced Thermodynamics and Statistical Mechanics

Polyhydroxyalkanoate‐associated phasins as phylogenetically heterogeneous, multipurpose proteins

Beatriz Maestro、Jesús M. Sanz2017-04-20Microbial Biotechnology

Polyhydroxyalkanoates (PHAs) are natural polyesters of increasing biotechnological importance that are synthesized by many prokaryotic organisms as carbon and energy storage compounds in limiting growth conditions. PHAs accumulate intracellularly in form of inclusion bodies that are covered with a proteinaceous surfac…

biodegradable polymer synthesis and propertiesElectrospun Nanofibers in Biomedical ApplicationsMicroplastics and Plastic Pollution