Materials Literature
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In this work we develop an algorithm for signal reconstruction from the magnitude of its Fourier transform in a situation where some (non-zero) parts of the sought signal are known. Although our method does not assume that the known part comprises the boundary of the sought signal, this is often the case in microscopy…
Scanning tunneling microscopy
In this work, polyacrylamide is investigated as an ultralow fouling surface coating to highly resist protein adsorption, cell adhesion, and bacterial attachment. Polyacrylamide was grafted on gold surfaces via surface-initiated atom transfer radical polymerization (ATRP). Protein adsorption from a wide range of biolog…
High-mobility solution-processed all-inorganic solid state nanocrystal (NC) transistors with low operation voltage and near-zero hysteresis are demonstrated using high-capacitance ZrO(x) and hydroxyl-free Cytop gate dielectric materials. The use of inorganic capping ligands (In(2)Se(4)(2-) and S(2-)) allowed us to ach…
Enzyme works for plasmonic nanostructure: an interesting enzyme-responsive hybrid Ag/Au-GOx bimetallic nanoshell (NS) system is reported, in which control over the enzyme reaction of glucose oxidase (GOx) can automatically fine-tune the morphology (from complete NS to porous NS) and optical properties of the hybrid na…
While the rheology of non-brownian suspensions in the dilute regime is well understood, their behavior in the dense limit remains mystifying. As the packing fraction of particles increases, particle motion becomes more collective, leading to a growing length scale and scaling properties in the rheology as the material…
Mercaptocarboxylic acids with different carbon chain lengths were used for stabilizing uniform 15 nm copper nanoparticles. The effects of surface chemistry such as ligand type and surface oxidation on the reactive oxygen species (ROS) generated by the copper nanoparticles were examined. Transmission electron microscop…
Two new significant discoveries are reported: i) the dragline silk of N. clavipes spider has an exceptionally high thermal conductivity: up to 416 W/m·K that beats most materials; ii) contrary to normal materials, its thermal conductivity increases with strain (19% increase under ∼20% strain). These new findings will…
9,10-Dihydro-9-oxa-10-phosphaphenanthrene-10-oxide (DOPO) has been grafted onto the surface of graphene oxide (GO) by reacting epoxy ring groups together with the reduced graphene structure (DOPO-rGO). X-ray photoelectron spectroscopy (XPS), X-ray diffraction (XRD), Fourier transform infrared (FTIR) spectroscopy, Rama…
This paper presents a flexible solid-state supercapacitor of high energy density. The electrodes of the supercapacitor are made of porous and absorbent cotton paper coated with single-wall carbon nanotubes. To ensure all solid-state configuration, a solid-state polymer-based electrolyte (poly (vinyl alcohol)/phosphori…
We have previously shown that square arrays of three-dimensional gold helices can serve as compact broadband circular polarizers. Here, we show by heuristic reasoning supported by numerical calculations that the bandwidth of the device can realistically be increased to 1.5 octaves by tapering the gold-helix radius. Th…
Methane-producing hollow nanocubes: Hybrid CuO-TiO(2-x)N(x) hollow nanocubes have been synthesized by first depositing TiO(2) onto Cu(3)N nanocube templates, then heating in air to oxidize the Cu(3)N to CuO while concomitantly incorporating nitrogen into the TiO(2). The nanostructured CuO-TiO(2-x)N(x) material photoca…
We demonstrate atomic-layer-deposited (ALD) high-kdielectric integration on 2-D layer-structured molybdenum disulfide (MoS2) crystals and MoS2dual-gate n-channel MOSFETs with ALD Al2O3as the gate dielectric. OurC-Vstudy of MOSFET structures shows good interface between 2-D MoS2crystal and ALD Al2O3. Maximum drain curr…
We report a novel nanoparticulate drug delivery system that undergoes reversible volume change from 150 to 40 nm upon phototriggering with UV light. The volume change of these monodisperse nanoparticles comprising spiropyran, which undergoes reversible photoisomerization, and PEGylated lipid enables repetitive dosing…
Synthetic materials that are capable of autonomous healing upon damage are being developed at a rapid pace because of their many potential applications. Despite these advancements, achieving self-healing in permanently cross-linked hydrogels has remained elusive because of the presence of water and irreversible cross-…
A microwave ultra-broadband polarization-independent metamaterial absorber is demonstrated. It is composed of a periodic array of metal-dielectric multilayered quadrangular frustum pyramids. These pyramids possess resonant absorption modes at multi-frequencies, of which the overlapping leads to the total absorption of…
Four new mesogenic homologous series, each containing a 6-alkoxy 2-naphthoic acid and Schiff base-ester as central linkage, have been synthesised by esterification of 4-{[(4-hydroxyphenyl) imino] methyl} phenyl 4-propoxy benzoate, 4-{[(4-hydroxyphenyl) imino] methyl} phenyl 4- (pentyloxy) benzoate, 4-{[(4-hydroxypheny…
We report the development of highly chemically crosslinked, ultra low density (~0.015 g/cc) polyurethane shape memory foams synthesized from symmetrical, low molecular weight and branched hydroxyl monomers. Sharp single glass transitions (Tg) customizable in the functional range of 45-70 °C were achieved. Thermomechan…
Silicene is a monolayer of silicon atoms forming a two-dimensional honeycomb lattice, which shares almost every remarkable property with graphene. The low energy structure of silicene is described by Dirac electrons with relatively large spin-orbit interactions due to its buckled structure. The key observation is that…
To predict the thermal conductivity of a dielectric or insulating material requires the phonon frequencies and lifetimes. Techniques for predicting these quantities have been proposed based in molecular dynamics simulation and lattice dynamics calculations. Here, two expressions for the phonon spectral energy density…