Materials Literature
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We report a detailed investigation of resistance noise in single layer graphene films on Si/SiO2 substrates obtained by chemical vapor deposition (CVD) on copper foils. We find that noise in these systems to be rather large, and when expressed in the form of phenomenological Hooge equation, it corresponds to Hooge par…
A method for the study of conjugated polyelectrolyte (CPE) photophysics in solution at the single-molecule level is described. Extended observation times of single polymer molecules are enabled by the encapsulation of the CPEs within 200-nm lipid vesicles, which are in turn immobilized on a surface. When combined with…
Gold nanoparticles of 10 nm and 250 nm were intravenously injected in rats. At 24 h after administration, tissues were collected and prepared for transmission electron microscopy (TEM). In the liver and spleen of animals treated with 10 nm gold nanoparticles, groups of nanoparticles were observed that could be positiv…
Nanofluidic transport in lab-on-chip devices requires nanochannels that are difficult to fabricate since they require challenging top-down technological approaches. We present a bottom-up, scalable, low-cost, and robust alternative to construct large areas of extremely homogeneous Pillared Planar Nanochannels (PPNs) f…
Molecular dynamics simulations can aid studies of the structural and physicochemical properties of proteins, by predicting their dynamics, energetics, and interactions with their local environment at the atomistic level. We argue that nonstandard protocols are needed to realistically model collagen proteins, which in…
Photochromic bis(thiazol-4-yl)maleimides, displaying enhanced binding affinity to complementary melamine receptors in their ring-closed switching state, have been developed and could pave the way to light-responsive supramolecular assemblies.
In this paper, we described a strategy for synthesis of thiol-coated CdTe/CdS/ZnS (core-shell-shell) quantum dots (QDs) via aqueous synthesis approach. The synthesis conditions were systematically optimized, which included the size of CdTe core, the refluxing time and the number of monolayers and the ligands, and then…
Using time-resolved photoluminescence spectroscopy, we analyze single and multiexciton emission energies and decay dynamics of CdS/ZnSe core/shell nanocrystals (NCs). The NCs exhibit a characteristic type-II band alignment that leads to spatially separated charges; this effect is at the origin of long radiative excito…
We present the results of calculations of surface relaxations, rumplings, energetics, optical band gaps, and charge distribution for the SrZrO(3) and PbZrO(3) (001) and (011) surfaces using the ab initio code CRYSTAL and a hybrid description of exchange and correlation. We consider both SrO(PbO) and ZrO(2) termination…
The electron mean free path (lgr) is “locally” evaluated by scanning capacitance spectroscopy on graphene obtained with different preparation methods and on different substrates, i.e., graphene exfoliated from highly oriented pyrolitic graphite (HOPG) and deposited (DG) on 4H-SiC(0001) and on SiO2 and epitaxial graphe…
Abstract N ‐carboxymethyl chitosans ( N ‐CMC) were synthesized from chitosan in water with chloroacetic acid instead of comparatively expensive glyoxylic acid. The optimal reaction conditions were 90°C and 4 h with a ratio of chloroacetic acid to chitosan 5 : 1(w/w). The degree of substitution of product exceeded 1.32…
Based on the form invariance of Helmholtz equation, we present a rhombic acoustic cloak constructed with homogeneous metamaterials. In free space, the proposed cloak can effectively conceal an object inside under a given incident direction. Another application, namely carpet cloak, was also demonstrated by full wave s…
The dielectric resonance and multiple magnetic resonances which correspond to multiple microwave absorptions in the 2–18 GHz range have been studied in the composite Fe/TiO2. The Fe grain size is found to have great impact on the dielectric resonance in this metal-semiconductor composite. The polarization mechanism is…
Ab initio molecular dynamics simulations have been carried out to determine both threshold displacement energies, E(d), and corresponding defect configurations, and ab initio methods have been used to determine defect formation energies in Y(2)Ti(2)O(7). The minimum E(d) is found to be 27 eV for a Y recoil along the {…
Herein we are the first to report that single-walled carbon nanotubes (SWCNTs) exhibit dual-phase regulation to Arabidopsis mesophyll cells exposed to different concentration of SWCNTs. The mesophyll protoplasts were prepared by enzyme digestion, and incubated with 15, 25, 50, 100 μg/ml SWCNTs for 48 h, and then were…
In this letter, we report an experimental demonstration on voltage tunable short wire-pair metamaterial with negative permeability at microwave frequencies. After infiltrated by nematic liquid crystal, magnetic resonance of short wire-pair can be effectively tuned via relatively low static electric field. The results…
Mixed mode fracture resistance was analyzed for some previously tested ceramics using a three‐parameter fracture criterion called the generalized maximum tangential stress (GMTS) criterion. For using this fracture criterion, the size of a critical distance from the crack tip was required. Therefore, an analytical mode…
To develop a new system for site-specific targeting, superparamagnetic CaCO(3) mesocrystals with the properties of biocompatibility and biodegradability are designed and synthesized. They serve as carriers for the co-delivery of drug and gene nanoparticles via a multistage method for cancer therapy. With a porous stru…
Nanoparticles (NPs) offer promise for a multitude of biological applications including cellular probes at the bio-interface for targeted delivery of anticancer substances, Raman and fluorescent-based imaging and directed cell growth. Nanodiamonds (NDs), in particular, have several advantages compared to other carbon-b…
Cubic BaCo 0.7 Fe 0.3− x Y x O 3−δ (BCFY, x = 0.08−0.2) was prepared by the conventional solid state reaction route as oxygen permeation membranes. The effects of Y-doping on the crystal structure, electrical conductivity, and oxygen permeability are investigated, and the factors influencing the activation energy of o…