Materials Literature
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Resolving the structure of energy bands in transport experiments is a major challenge in condensed matter physics and material science. Sometimes, however, traditional electrical conductance or resistance measurements only provide very small signals, and thus limit the ability to obtain direct band structure informati…
We have studied the growth of metastable face-centered-cubic, non-magnetic Fe78Ni22 thin films on silicon substrates. These films undergo a magnetic (paramagnetic to ferromagnetic) and structural (fcc to bcc) phase transformation upon ion beam irradiation and thus can serve as a template for direct writing of magnetic…
Multifold fermions are generalizations of two-fold degenerate Weyl fermions with three-, four-, six- or eight-fold degeneracies protected by crystal symmetries, of which only the last type is necessarily non-chiral. Their low energy degrees of freedom can be described as emergent particles not present in the Standard…
Within 4 different crystal structures, 2280 ternary intermetallic configurations have been investigated via high-throughput density functional theory calculations in order to discover new semiconducting materials. The screening is restricted to intermetallics with the equimolar composition TMX, where T is a transition…
Novel topological phenomena are anticipated for three-dimensional (3D) Dirac electrons. The magnetotransport properties of cubic ${\rm Sr_{3}PbO}$ antiperovskite, theoretically proposed to be a 3D massive Dirac electron system, are studied. The measurements of Shubnikov-de Haas oscillations and Hall resistivity indica…
We investigate electronic transport in twisted bilayer graphene (tBLG) under variable temperatures ($T$), carrier densities ($n$), and transverse magnetic fields, focusing on samples with small twist angles (\ensuremath{\theta}). These samples show prominent signatures associated with the van Hove singularities (VHSs)…
We demonstrate an extreme variability and tunability of the molecular gyromagnetic coupling $g$-tensor with respect to the geometric and electronic structure in a much studied class of organic semiconductors (OSCs). This class of OSCs is composed of a structural theme of phenyl- and chalcogenophene (group XVI element…
Charge trapping and the formation of polarons is a pervasive phenomenon in transition-metal oxide compounds, in particular at the surface, affecting fundamental physical properties and functionalities of the hosting materials. Here we investigate via first-principles techniques the formation and dynamics of small pola…
Organic-inorganic halide perovskite solar cells have recently attracted much attention due to their low-cost fabrication, flexibility, and high-power conversion efficiency. The reduction from three- to two-dimension (2D) promises an exciting opportunity to tune the electronic properties of organic-inorganic halide per…
Small-molecule fluorescent probes are powerful tools for chemical biology; however, despite the large number of probes available, there is still a need for a simple fluorogenic scaffold, which allows for the rational design of molecules with predictable photophysical properties and is amenable to concise synthesis for…
Improving the wetting ability of Ag on chemically heterogeneous oxides is technically important to fabricate ultrathin, continuous films that would facilitate the minimization of optical and electrical losses to develop qualified transparent Ag film electrodes in the state-of-the-art optoelectronic devices. This goal…
Abstract Phonon engineering is expected to contribute to further development of various fields and technologies such as electronics, photonics, thermal engineering, and materials science. Although phonons inherently exist in condensed matter, their behavior strongly depends on the scale of the system and the materials…
Layered transition-metal dichalcogenides that host coexisting charge-density wave (CDW) and superconducting orders provide ideal systems for exploring the effects of dimensionality on correlated electronic phases. Dimensionality has a profound effect on both superconductivity and CDW instabilities. Here we report a su…
Spinel type manganese oxide (Mn3O4) nanoparticles were synthesized by ultrasonic irradiation assisted co-precipitation method using PEG and NaOH. The formation of tetragonal hausmannite phase (Mn3O4) with spinel structure was confirmed from XRD and FTIR studies. The average crystallite size of Mn3O4 nanoparticles was…
Based on a transformation optics method, a flat compact dual-polarized Luneburg lens antenna is proposed and implemented using the printed-circuit-board-stacked gradient-index metamaterials for beamscanning and multibeam applications at X-bands. The transformed material properties of the planar Luneburg lens are desig…
Abstract First-order magnetic transitions (FOMTs) with a large discontinuity in magnetization are highly sought in the development of advanced functional magnetic materials. Isosymmetric magnetoelastic FOMTs that do not perturb crystal symmetry are especially rare, and only a handful of material families, almost exclu…
To investigate the Li + doping effect on the structure and reactivity of NiO, a series of NiO catalysts doped by Li + cations have been synthesized and probed by using CO oxidation as a model reaction. With a combination of experimental methods and DFT calculations, it has been revealed that the Li + cations preferent…
Conspectus Thiolate-protected gold nanoparticles (AuNPs) are a special class of nanomaterials that form atomically precise NPs with distinct numbers of Au atoms ( n ) and thiolate (−SR, R = hydrocarbon tail) ligands ( m ) with molecular formula [Au n (SR) m ]. These are generally termed Au nanomolecules (AuNMs), nanoc…
We study the effects of different electrolyte anions on the mixed ionic/electronic transport properties of organic electrochemical transistors (OECTs) based on poly(3-hexylthiophene-2,5-diyl). We show that the transport properties depend on the anion present in the electrolyte, with greater source-drain currents resul…
Abstract Compared to traditional metal oxides, metal‐organic frameworks exhibit excellent properties, such as a high surface area, significant thermal stability, low density, and excellent electrochemical performance. Here, a simple process is proposed for the fabrication of rod‐like vanadium metal‐organic frameworks…