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Towards wafer-scale diamond nano- and quantum technologies

Richard Nelz、Johannes Görlitz、Dennis Herrmann 等 11 位作者2018-10-22arXiv

We investigate native nitrogen (NV) and silicon vacancy (SiV) color centers in commercially available, heteroepitaxial, wafer-sized, mm thick, single-crystal diamond. We observe single, native NV centers with a density of roughly 1 NV per $μm^3$ and moderate coherence time ($T_2 = 5 μs$) embedded in an ensemble of SiV…

Materials ScienceApplied Physicsphysics.opticsquant-ph

Surface Termination Dependent Quasiparticle Scattering Interference and Magneto-transport Study on ZrSiS

Chih-Chuan Su、Chi-Sheng Li、Tzu-Cheng Wang 等 10 位作者2018-10-22arXiv

Dirac nodal line semimetals represent a new state of quantum matters in which the electronic bands touch to form a closed loop with linear dispersion. Here, we report a combined study on ZrSiS by density functional theory calculation, scanning tunneling microscope (STM) and magneto-transport measurements. Our STM meas…

Materials Science

Investigation of the Microstructures of Graphene Quantum Dots (GQDs) by Surface-Enhanced Raman Spectroscopy

Junxiao Wu、Peijie Wang、Fu-He Wang 等 4 位作者2018-10-22Nanomaterials

Photoluminescence (PL) is the most significant feature of graphene quantum dots (GQDs). However, the PL mechanism in GQDs has been debated due to the fact that the microstructures, such as edge and in-plane defects that are critical for PL emission, have not been convincingly identified due to the lack of effective de…

Carbon and Quantum Dots ApplicationsNanocluster Synthesis and ApplicationsGraphene and Nanomaterials Applications

Effects of Zinc Oxide Nanoparticles on the Properties of Pectin/Alginate Edible Films

Thi Minh Phuong Ngo、Thi Mong Quyen Dang、Thi Xo Tran 等 4 位作者2018-10-22International Journal of Polymer Science

This study aimed at developing the functional packaging properties of pectin/alginate films by adding zinc oxide nanoparticles (ZnO-NPs). The ZnO-NPs were added to the pectin/alginate film at the concentrations of 0.5, 2.5, 5, and 25 g/100 g of blended polymer. The effects of the ZnO-NP incorporation on the mechanical…

Nanoparticles: synthesis and applicationsNanocomposite Films for Food Packagingbiodegradable polymer synthesis and properties

Effect of Various Chemical Treatments of Prosopis juliflora Fibers as Composite Reinforcement: Physicochemical, Thermal, Mechanical, and Morphological Properties

P. Madhu、Sanjay Mavinkere Rangappa、P. Senthamaraikannan 等 7 位作者2018-10-22Journal of Natural Fibers

The present environmental regulations enforced by the government authorities have made the investigators around the globe to make use of more and more green materials particularly in composite systems. In this context, natural fibers play an important role and proven to be excellent reinforcements in polymer matrices.…

Nanocomposite Films for Food PackagingPolymer Nanocomposites and PropertiesNatural Fiber Reinforced Composites

Preparation and Characterization of Potato Starch Film with Various Size of Nano-SiO2

Rongfei Zhang、Xiangyou Wang、Meng Cheng2018-10-22Polymers

The various sizes (15, 30, 80, and 100 nm) of nano-SiO2/potato starch films were synthesized and characterized. The gas permeability, antibacterial properties, and mechanical properties of the films were evaluated to their potential for application as food packaging materials. Results indicated that the 100 nm nano-Si…

Postharvest Quality and Shelf Life ManagementNanocomposite Films for Food Packagingbiodegradable polymer synthesis and properties

Tutorial: Basic principles, limits of detection, and pitfalls of highly sensitive SQUID magnetometry for nanomagnetism and spintronics

Martin Buchner、K. Höfler、Bastian Henne 等 5 位作者2018-10-22Journal of Applied Physics

In the field of nanomagnetism and spintronics, integral magnetometry is nowadays challenged by samples with low magnetic moments and/or low coercive fields. Commercial superconducting quantum interference device magnetometers are versatile experimental tools to magnetically characterize samples with ultimate sensitivi…

Physics of Superconductivity and MagnetismMagnetic properties of thin filmsMagnetic and transport properties of perovskites and related materials

Cooperative mechanisms of oxygen vacancy stabilization and migration in the isolated tetrahedral anion Scheelite structure

Xiaoyan Yang、Alberto J. Fernández‐Carrión、Jiehua Wang 等 7 位作者2018-10-22Nature Communications

Abstract Tetrahedral units can transport oxide anions via interstitial or vacancy defects owing to their great deformation and rotation flexibility. Compared with interstitial defects, vacancy-mediated oxide-ion conduction in tetrahedra-based structures is more difficult and occurs rarely. The isolated tetrahedral ani…

Ferroelectric and Piezoelectric MaterialsAdvanced Condensed Matter PhysicsNuclear materials and radiation effects

Tunable Water Harvesting Surfaces Consisting of Biphilic Nanoscale Topography

Youmin Hou、Yuhe Shang、Miao Yu 等 6 位作者2018-10-22ACS Nano

Water scarcity has become a global issue of severe concern. Great efforts have been undertaken to develop low-cost and highly efficient condensation strategies to relieve water shortages in arid regions. However, the rationale for design of an ideal condensing surface remains lacking due to the conflicting requirement…

Surface Modification and SuperhydrophobicityAdvanced Sensor and Energy Harvesting MaterialsSolar-Powered Water Purification Methods

Synthetic Control of Two-Dimensional NiTe2 Single Crystals with Highly Uniform Thickness Distributions

Bei Zhao、Weiqi Dang、Yuan Liu 等 13 位作者2018-10-22Journal of the American Chemical Society

Two-dimensional (2D) layered materials have stimulated extensive research interest for their unique thickness-dependent electronic and optical properties. However, the layer-number-dependent studies on 2D materials to date are largely limited to exfoliated flakes with relatively small lateral size and poor yield. The…

2D Materials and ApplicationsAdvanced Thermoelectric Materials and DevicesMXene and MAX Phase Materials

High-Performance n-Type PbSe–Cu2Se Thermoelectrics through Conduction Band Engineering and Phonon Softening

Chongjian Zhou、Yuan Yu、Yong Kyu Lee 等 10 位作者2018-10-22Journal of the American Chemical Society

From a structural and economic perspective, tellurium-free PbSe can be an attractive alternative to its more expensive isostructural analogue of PbTe for intermediate temperature power generation. Here we report that PbSe 0.998 Br 0.002 -2%Cu 2 Se exhibits record high peak ZT 1.8 at 723 K and average ZT 1.1 between 30…

Quantum Dots Synthesis And PropertiesAdvanced Thermoelectric Materials and DevicesChalcogenide Semiconductor Thin Films

Porphyrin Boxes

Rahul Dev Mukhopadhyay、Younghoon Kim、Jaehyoung Koo 等 4 位作者2018-10-22Accounts of Chemical Research

In order to fabricate efficient molecular photonic devices, it has been a long-held aspiration for chemists to understand and mimic natural light-harvesting complexes where a rapid and efficient transfer of excitation energy between chlorophyll pigments is observed. Synthetic porphyrins are attractive building blocks…

Supramolecular Chemistry and ComplexesPorphyrin and Phthalocyanine ChemistryCovalent Organic Framework Applications

Wavelength‐Controlled Dynamic Metathesis: A Light‐Driven Exchange Reaction between Disulfide and Diselenide Bonds

Fuqiang Fan、Shaobo Ji、Chenxing Sun 等 7 位作者2018-10-22Angewandte Chemie International Edition

Wavelength-controlled dynamic processes are mostly based on light-triggered isomerization or the cleavage/formation of molecular connections. Control over dynamic metathesis reactions by different light wavelengths, which would be useful in controllable dynamic chemistry, has rarely been studied. Taking advantage of t…

Synthetic Organic Chemistry MethodsPhotochromic and Fluorescence ChemistrySulfur-Based Synthesis Techniques

Full-Color Tunable Fluorescent and Chemiluminescent Supramolecular Nanoparticles for Anti-counterfeiting Inks

Minzan Zuo、Weirui Qian、Tinghan Li 等 6 位作者2018-10-22ACS Applied Materials & Interfaces

A drive for anti-counterfeiting technology has attracted considerable interests in developing nanomaterials with a wide range of colors and tunable optical properties in solid state. Herein, with a series of conjugated polymers and based on the host–guest driven self-assembly strategy, a color-tunable supramolecular n…

Luminescence and Fluorescent MaterialsCarbon and Quantum Dots ApplicationsPolydiacetylene-based materials and applications

Layered graphene/GaS van der Waals heterostructure: Controlling the electronic properties and Schottky barrier by vertical strain

Khang D. Pham、Nguyen N. Hieu、Huynh V. Phuc 等 7 位作者2018-10-22Applied Physics Letters

In this work, we construct an ultrathin graphene/GaS heterostructure and investigate its electronic properties as well as the effect of vertical strain using density functional theory. The calculated results of the equilibrium interlayer spacing (3.356 Å) and the binding energy show that the intrinsic properties of is…

Graphene research and applications2D Materials and ApplicationsMXene and MAX Phase Materials

Compatibilization of Isotactic Polypropylene (iPP) and High-Density Polyethylene (HDPE) with iPP–PE Multiblock Copolymers

Jun Xu、James M. Eagan、Sung‐Soo Kim 等 13 位作者2018-10-22Macromolecules

High Resolution Image Download MS PowerPoint Slide A series of isotactic polypropylene ( i PP) and polyethylene (PE) diblock, tetrablock, and hexablock copolymers (BCPs) were synthesized with tunable molecular weights using a hafnium pyridylamine catalyst. The BCPs were melt blended with 70 wt % high-density PE (HDPE)…

Polymer crystallization and propertiesPolymer Nanocomposites and Propertiesbiodegradable polymer synthesis and properties

The Nuclearity of the Active Site for Methane to Methanol Conversion in Cu-Mordenite: A Quantitative Assessment

Dimitrios K. Pappas、Andrea Martini、Michael Dyballa 等 16 位作者2018-10-22Journal of the American Chemical Society

The direct conversion of methane to methanol (MTM) is a reaction that has the potential to disrupt a great part of the synthesis gas-derived chemical industry. However, despite many decades of research, active enough catalysts and suitable processes for industrial application are still not available. Recently, several…

Catalytic Processes in Materials ScienceCatalysts for Methane ReformingCatalysis and Oxidation Reactions

SIFTS: updated Structure Integration with Function, Taxonomy and Sequences resource allows 40-fold increase in coverage of structure-based annotations for proteins

Jose M Dana、Aleksandras Gutmanas、Nidhi Tyagi 等 7 位作者2018-10-22OpenAlex

The Structure Integration with Function, Taxonomy and Sequences resource (SIFTS; http://pdbe.org/sifts/) was established in 2002 and continues to operate as a collaboration between the Protein Data Bank in Europe (PDBe; http://pdbe.org) and the UniProt Knowledgebase (UniProtKB; http://uniprot.org). The resource is ins…

Genomics and Phylogenetic StudiesProtein Structure and DynamicsEnzyme Structure and Function

Activity enhancement of cobalt catalysts by tuning metal-support interactions

Carlos Hernández Mejía、Tom W. van Deelen、Krijn P. de Jong2018-10-22OpenAlex

Abstract Interactions between metal nanoparticles and support materials can strongly influence the performance of catalysts. In particular, reducible oxidic supports can form suboxides that can decorate metal nanoparticles and enhance catalytic performance or block active sites. Therefore, tuning this metal-support in…

Catalytic Processes in Materials ScienceCatalysts for Methane ReformingCatalysis and Hydrodesulfurization Studies