Materials Literature
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We report on the realization of ZnO homojunction light-emitting diodes (LEDs) fabricated by metalorganic chemical vapor deposition on (0001) ZnO bulk substrate. The p-type ZnO epilayer was formed by nitrogen incorporation using N2O gas as oxidizing and doping sources. Distinct electroluminescence (EL) emissions in the…
A spontaneous luminescence is reported when epoxy resin samples are heated in air. This phenomenon is very sensitive to the nature of the atmosphere. The same treatment in nitrogen leads to an extinction of the luminescence. The emission process is restored when samples are kept for a sufficient time in air. In order…
The metal-support interactions on a series of catalysts of different acidities, including platinum-modified zeolites and H-MCM-41, are investigated by means of XPS, CO and pyridine adsorption, and a model reaction (ring opening of decalin). The electronic properties of Pt are influenced by the acidity of the support,…
Using high precision Monte Carlo simulations and a mean-field theory, we explore coarsening phenomena in a simple driven diffusive system. The model is reminiscent of vehicular traffic on a two-lane ring road. At sufficiently high density, the system develops jams (clusters) which coarsen with time. A key parameter is…
Rubber composites containing multiwalled carbon nanotubes have been irradiated with near-infrared light to study their reversible photomechanical actuation response. We demonstrate that the actuation is reproducible across differing polymer systems. The response is directly related to the degree of uniaxial alignment…
We investigate photoluminescence from a high-density electron-hole plasma in semiconductor quantum wells created via intense femtosecond excitation in a strong perpendicular magnetic field, a fully-quantized and tunable system. At a critical magnetic field strength and excitation fluence, we observe a clear transition…
The influence of an externally applied magnetic field upon classic cubic quintic dissipative solitons is investigated using both exact simulations and a Lagrangian technique. The basic approach is to use a spatially inhomogeneous magnetic field and to consider two important geometries, namely the Voigt and the Faraday…
Spin relaxation under identical Dresselhaus and Rashba coupling strengths in GaAs quantum wells is studied in both the traditional collinear statistics, where the energy spectra do not contain the spin-orbit coupling terms, and the helix statistics, where the spin-orbit couplings are included in the energy spectra. We…
Theoretical models for small ferroelectric particles predict a progressive decrease of the Curie temperature, spontaneous lattice strain, and polarization until the critical size corresponding to transition to the cubic phase and disappearance of ferroelectricity is reached. In contrast, the behavior of nanocrystallin…
Gold nanorods were attached to the gene of enhanced green fluorescence protein (EGFP) for the remote control of gene expression in living cells. The UV-vis spectroscopy, electrophoresis, and transmission electron microscopy (TEM) were used to study the optical and structural properties of the EGFP DNA and gold nanorod…
We measured the electronic local density of states (LDOS) of graphite surfaces near monoatomic step edges, which consist of either the zigzag or armchair edge, with the scanning tunneling microscopy (STM) and spectroscopy (STS) techniques. The STM data reveal that the $(\sqrt{3}\ifmmode\times\else\texttimes\fi{}\sqrt{…
Nanocrystals of different size and functionality (e.g., noble metals, semiconductors, oxides, magnetic alloys) can be induced to self-assemble into ordered binary superlattices (also known as opals or colloidal crystals), retaining the size tunable properties of their constituents. We have built a variety of binary su…
Self-assembly of charged, equally sized metal nanoparticles of two types (gold and silver) leads to the formation of large, sphalerite (diamond-like) crystals, in which each nanoparticle has four oppositely charged neighbors. Formation of these non-close-packed structures is a consequence of electrostatic effects spec…
The cyclic instability phenomenon is investigated at the modeling of large elasto-plastic strains. The instability is observed at large strains for some elasto-plastic material models with a kinematic hardening in contrast to the small strain case. The cyclic instability manifests itself as a changing of shape, sizes…
Bicomponent fibers, in the range of 100 nm to a few microns, of miscible poly(vinylchloride)/segmented polyurethane (PVC/Estane®) and immiscible poly(vinyl chloride)/poly(vinylidienefluoride) (PVC/PVDF) were produced respectively by electrospinning two polymer solutions in a side-by-side approach. For each of the pair…
Conducting polymers, carbon nanotubes, and their hybrid structures are promising for various sensing applications. While the electrospun lithium perchlorate (LiClO 4 )-doped polyethylene oxide (PEO) nanofibers have been shown to be good humidity sensing materials, camphosulfonic acid (HCSA)-doped polyaniline (PANI)/po…
This paper considers the development of a comprehensive model of the electrospinning process. All stages of the electrospinning process, from the preparation of the solution to the collection of the nanofibers are discussed together from the point of view of manufacturing. Experimental observations of the three-dimens…
We have successfully developed a unique multiple-jet electrospinning technology at STAR, Inc. and Stony Brook University. The development of this technology was primarily accomplished by the incorporation of secondary electrodes to isolate the electric field distribution of the primary electrode spinnerets, the design…
The crystal structure of an uncharacterized conserved protein (residues 1–243) expressed by yfiH gene of Shigella flexneri 2a str.2457T (gi 30042248),1 has been determined and refined to 2.01 Å by single wavelength anomalous dispersion (SAD) method. The YfiH protein belongs to a vast protein family of at least 201 unc…
Four low molecular mass lysine dendrimers were synthesized by Boc chemistry in solution (155 and 169) and Fmoc chemistry on solid support (P2 and P13). The structure and fragmentation mode of the above dendrimers was investigated in gas phase by the LSI-MS and ESI-MS techniques. (1)H and (13)C NMR analysis in solution…