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A newly described cellulosomal cellobiohydrolase, CelO, from Clostridium thermocellum: investigation of the exo-mode of hydrolysis, and binding capacity to crystalline cellulose The GenBank accession number for the sequence determined in this work is AJ275975.

Vladimir V. Zverlov、G. A. Velikodvorskaya、Wolfgang H. Schwarz2002-01-01Microbiology

The sequence of the celO gene from Clostridium thermocellum F7 was determined. The gene product, cellulase CelO (Ct-Cel5F), had a modular structure consisting of a carbohydrate-binding module of the CBM3 family and a catalytic domain of the glycosyl hydrolase family 5. The presence of the dockerin module indicated tha…

Biofuel production and bioconversionAdvanced Cellulose Research StudiesPolysaccharides and Plant Cell Walls

Phase Transformations And Dynamics Of 4-Cyano-4′-Pentylbiphenyl (5cb) By Nuclear Magnetic Resonance, Analysis Differential Scanning Calorimetry, And Wideangle X-Ray Diffraction Analysis

T. Mansaré、R. Decressain、C. Gors 等 4 位作者2002-01-01Molecular Crystals and Liquid Crystals

The polymorphism of 4-cyano-4′-pentylbiphenyl (5CB) was investigated by means of differential scanning calorimetry (DSC), X-ray diffraction, and proton nuclear magnetic resonance (NMR) experiments. Three new phases has been identified and characterized structurally and dynamically. By a slow cooling at a rate ≤ 0.2 K/…

Liquid Crystal Research AdvancementsMaterial Dynamics and PropertiesMolecular spectroscopy and chirality

Effect of Mold Material and Binder on Metal-Mold Interfacial Reaction for Investment Castings of Titanium Alloys

Myoung-Gyun Kim、S KIM、Young‐Jig Kim2002-01-01MATERIALS TRANSACTIONS

The aim of the present paper is to investigate the combined effect of mold material and binder for investment casting of titanium and titanium alloys. A plasma arc melting furnace was used for melting titanium alloy, and the interfacial reaction of titanium castings was determined by optical microscope, SEM, EDS analy…

Aluminum Alloys Composites PropertiesTitanium Alloys Microstructure and PropertiesAdvanced materials and composites

Plasma treatment of polycarbonate for improved adhesion

A. Hofrichter、Pavel Bulkin、B. Drévillon2002-01-01Journal of Vacuum Science & Technology A Vacuum Surfaces and Films

The deposition of silicon alloys for protective and optical coatings on polymers is of increasing interest. The understanding of the plasma polymer interaction is of prime importance here. In this work, we report a study of the influence of N2, H2, and O2 plasma treatments on pure and commercial grade polycarbonate (P…

Surface Modification and SuperhydrophobicityAdvanced Sensor and Energy Harvesting MaterialsDiamond and Carbon-based Materials Research

Factors influencing the stability of low temperature tetragonal ZrO2

Goran Štefanić、Svetozar Musić2002-01-01Institutional Repository of the Ruđer Bošković Institute (Ruđer Bošković Institute)

Various factors that influence the appearance of a tetragonal (t-) ZrO2 polymorph at room temperature have been extensively investigated. Several proposed models emphasize the role of anionic impurities (SO42-, OH-), crystallite size (surface energy), structural similarities between the starting material and t-ZrO2, l…

Advanced ceramic materials synthesisIntermetallics and Advanced Alloy PropertiesNuclear Materials and Properties

Thermal Expansion of Rare-Earth-Doped Ceria Ceramics.

Soichiro Sameshima、Manabu Kawaminami、Yoshihiro Hirata2002-01-01Journal of the Ceramic Society of Japan

The thermal expansion of CeO2 and rare-earth-doped ceria (Ce0.8R0.2O1.9, R: Yb, Y, Gd, Sm, Nd and La) was measured in the temperature range from 298 to 1473 K. The coefficients of thermal expansion (CTE) were determined by differentiating the thermal expansion expressed by a polynominal equation of temperature with re…

Catalytic Processes in Materials ScienceNuclear Materials and PropertiesThermal and Kinetic Analysis

The structure and spectroscopy of lanthanide( iii ) complexes with 2,2′-bipyridine-1,1′-dioxide in solution and in the solid state: effects of ionic size and solvent on photophysics, ligand structure and coordination

Ewa Huskowska、Ilona Turowska‐Tyrk、J. Legendziewicz 等 4 位作者2002-01-01New Journal of Chemistry

Single crystals of [Ln(2,2′-bipyridine-1,1′-dioxide)4](ClO4)3 (Ln = Nd, Lu) have been obtained and the crystal structures determined. By comparison with previous structural determinations, it is demonstrated that steric crowding associated with the decreasing lanthanide ions radius causes changes of the angles between…

Metal complexes synthesis and propertiesMagnetism in coordination complexesLanthanide and Transition Metal Complexes

Survey of factors determining the circularly polarised luminescence of macrocyclic lanthanide complexes in solution

James I. Bruce、David Parker、Stefan Lopinski 等 4 位作者2002-01-01Chirality

The development of emissive lanthanide complexes as structural or reactive probes to signal changes in their local chiral or ionic environment has been inhibited by the lack of understanding of correlating structural and electronic spectral information. The definition of relatively rigid enantiopure macrocyclic lantha…

Magnetism in coordination complexesLanthanide and Transition Metal ComplexesAdvanced NMR Techniques and Applications

Self-assembly of gold nanoparticles through tandem hydrogen bonding and polyoligosilsequioxane (POSS)–POSS recognition processes

Joseph B. Carroll、Benjamin L. Frankamp、Vincent M. Rotello2002-01-01Chemical Communications

Diaminopyridine-functionalized polyhedral oligomeric silsequioxanes (POSS-DAP) self-assemble with complementary thymine-functionalized Au nanoparticles (Thy-Au) into well-defined spherical aggregates, providing highly structured nanocomposites.

Dendrimers and Hyperbranched PolymersMarine Biology and Environmental ChemistrySilicone and Siloxane Chemistry

Effect of free surface heat loss and rotation on transition to oscillatory thermocapillary convection

Bok-Cheol Sim、Abdelfattah Zebib2002-01-01Physics of Fluids

Oscillatory thermocapillary convection in an open cylindrical annulus heated from the inside wall is investigated numerically. Results for aspect ratio of 1 and Prandtl number of 30 are obtained to compare the simulations with available space experiments. The influence of surface heat loss as quantified by a Biot numb…

Solidification and crystal growth phenomenaFluid Dynamics and Thin FilmsCharacterization and Applications of Magnetic Nanoparticles

Mechanical properties of layered InSe and GaSe single crystals

D. H. Mosca、N. Mattoso、C.M. Lepienski 等 7 位作者2002-01-01Journal of Applied Physics

The mechanical properties of InSe and GaSe single crystals have been studied by means of nanoindentation tests. Both bulk crystals are well ordered and present a predominant γ-type interlayer stacking sequence as determined by x-ray diffraction and transmission electron microscopy measurements. The course of plastic d…

Boron and Carbon Nanomaterials ResearchSemiconductor materials and interfacesSolid-state spectroscopy and crystallography

Solid-State Characterization of Fluconazole

Khouloud A. Alkhamis、Aiman A. Obaidat、Adi Al-Nuseirat2002-01-01Pharmaceutical Development and Technology

Two polymorphs and three solvates of fluconazole were isolated and characterized by x-ray powder diffractometry, IR spectroscopy, differential scanning calorimetry (DSC), thermogravimetry, and their dissolution rates. The different forms were prepared by crystallization of the original powder in different solvents at…

Crystallization and Solubility StudiesThermal and Kinetic AnalysisX-ray Diffraction in Crystallography

Reaction pathways and reaction progress for the smectite‐to‐chlorite transformation: evidence from hydrothermally altered metabasites

D. Robinson、S. Th. Schmidt、Azucena Zamora2002-01-01Journal of Metamorphic Geology

Abstract The transformation from smectite to chlorite has been interpreted as involving either a disequilibrium chlorite/smectite mixed‐layering sequence, or an equilibrated discontinuous sequence involving smectite–corrensite–chlorite. Here, analysis of the smectite to chlorite transition in different geothermal syst…

Geological and Geochemical AnalysisCO2 Sequestration and Geologic InteractionsClay minerals and soil interactions

Functionally Graded Cathodes for Honeycomb Solid Oxide Fuel Cells

Changrong Xia、William L. Rauch、William B. Wellborn 等 4 位作者2002-01-01Electrochemical and Solid-State Letters

Functionally graded cathodes were fabricated by slurry coating process for honeycomb solid oxide fuel cells with yttria-stabilized zirconia (YSZ) electrolytes. The cathodes are composed of strontium-doped lanthanum manganate (LSM), gadolinia-doped ceria, and La 0.6 Sr 0.4 Co 0.2 Fe 0.8 O 3 (LSCF). The LSM content was…

Advancements in Solid Oxide Fuel CellsCatalysis and Oxidation ReactionsElectronic and Structural Properties of Oxides

Synthesis, structure and luminescence properties of new rare earth metal complexes with 1-phenyl-3-methyl-4-acylpyrazol-5-ones

Claudio Pettinari、F. Marchetti、Riccardo Pettinari 等 7 位作者2002-01-01Journal of the Chemical Society Dalton Transactions

The isolation and characterization of new lanthanide complexes of formula [Ln(QL)3(EtOH)(H2O)], (Ln = La, Pr, Nd, Sm, Eu, Gd, Tb, Dy, Ho, Er, Tm, Yb; HQL = 1-phenyl-3-methyl-4-phenylacetylpyrazol-5-one) [Ln(QL)3(H2O)2] (L = La or Lu), [Ln(QS)3(EtOH)(H2O)] (Ln = Tb or Eu; HQS = 1-phenyl-3-methyl-4-thienoylpyrazol-5-one…

Organometallic Complex Synthesis and CatalysisMagnetism in coordination complexesLanthanide and Transition Metal Complexes

Aqueous synthesis of III–V semiconductor GaP and InP exhibiting pronounced quantum confinement

Shanmin Gao、Jun Lu、Nan Chen 等 5 位作者2002-01-01Chemical Communications

A mild aqueous synthesis route was successfully established to synthesize well crystallized and monodisperse GaP and InP nanocrystals, which were proved to exhibit pronounced quantum confinement by room-temperature UV/Vis adsorption and photoluminescence (PL) spectra.

Quantum Dots Synthesis And PropertiesChalcogenide Semiconductor Thin FilmsNanowire Synthesis and Applications

Thermal shock and thermal fatigue study of ceramic materials on a newly developed ascending thermal shock test equipment

Prashant Panda、T. S. Kannan、J. Harry DuBois 等 5 位作者2002-01-01Science and Technology of Advanced Materials

A test equipment was designed to study thermal shock and thermal fatigue of ceramic materials subjected to fast heating (ascending). The equipment was designed to generate thermal stress in a test specimen by heating one surface of it by an oxy-hydrogen flame while cooling the opposite surface. The sample cracked when…

Advanced ceramic materials synthesisNuclear Materials and PropertiesAdvanced materials and composites

Seeding Effect on Product Crystal Size in Batch Crystallization.

Noriaki Kubota、Norihito Doki、Masaaki Yokota 等 4 位作者2002-01-01JOURNAL OF CHEMICAL ENGINEERING OF JAPAN

This paper reviews research work concerning the size distribution of product crystals in batch crystallization of well-soluble materials. The discussion was made with particular emphasis on seeding effect on product crystal size distribution and crystallizer performance. First, it is shown by a brief survey of the his…

Minerals Flotation and Separation TechniquesCrystallization and Solubility StudiesFreezing and Crystallization Processes

Anti-Stokes Photoluminescence in II-VI Colloidal Nanocrystals

Yury P. Rakovich、Sergej Filonovich、M. J. M. Gomes 等 7 位作者2002-01-01physica status solidi (b)

For the first time highly efficient photon energy up-conversion (anti-Stokes photoluminescence) has been observed in colloids of CdTe nanocrystals (NCs) and CdSe NCs covered by ZnS shell. The maximum magnitude of the up-converted blue shift ΔEUCmax = 335 meV was obtained for CdSe/ZnS NCs under excitation by a low-powe…

Quantum Dots Synthesis And PropertiesChalcogenide Semiconductor Thin FilmsNonlinear Optical Materials Studies

Fabric development with nearest‐neighbor interaction and dynamic recrystallization

Þröstur Þorsteinsson2002-01-01Journal of Geophysical Research Atmospheres

Polycrystals undergoing ductile deformation develop lattice‐preferred orientation (fabric) as a result of intracrystalline slip. A consequence of fabric development is that bulk physical properties become anisotropic. Fabric development and macroscopic deformation are studied by examining three effects: nearest‐neighb…

Microstructure and mechanical propertiesMicrostructure and Mechanical Properties of SteelsCryospheric studies and observations