Materials Literature
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Using the first-principles method, we have studied the stability and electronic band structures of the transparent conducting oxides $\mathrm{Sn}{\mathrm{Zn}}_{2}{\mathrm{O}}_{4}$, $\mathrm{Sn}{\mathrm{Cd}}_{2}{\mathrm{O}}_{4}$, and $\mathrm{Cd}{\mathrm{In}}_{2}{\mathrm{O}}_{4}$. Our calculated lowest-energy phases of…
Tiopronin monolayer-protected silver nanoparticles with different core sizes (average diameter = 2, 5, 20 nm) were prepared by using different mole ratios of silver nitrate/tiopronin. Ligands on the silver particles were partially displaced by fluorescein-labeled thiolate single-stranded oligonucleotides or their comp…
We propose a kinetic theory of transport in metals embedded with ferromagnetic nanoclusters, describing the dependence of the form of magnetoresistance on anisotropy characteristics of the ensemble of clusters and the influence of the electron spin depolarisation by clusters. We note that this effect is strongest when…
A microscopic model is employed to calculate the spectrum of spin waves in quasiperiodic magnetic multilayers in the dipole-exchange regime. Results are presented for structures in which thin ferromagnetic films are separated by non-magnetic spacers following a Fibonacci sequence and extend previous magnetostatic calc…
The exchange coupling at the interfaces of magnetic superlattices consisting of ferromagnetic $SrRuO_3$ and antiferromagnetic $SrMnO_3$ grown on (001) oriented $SrTiO_3$ is studied with in-plane and out-of-plane orientations, with respect to the substrate plane, of the cooling magnetic field. The magnetization of the…
We report on magnetic and electrical transport properties of ${\mathrm{Sb}}_{2\ensuremath{-}x}{\mathrm{Cr}}_{x}{\mathrm{Te}}_{3}$ single crystals with $0\ensuremath{\leqslant}x\ensuremath{\leqslant}0.095$ over temperatures from $2\phantom{\rule{0.3em}{0ex}}\mathrm{K}$ to $300\phantom{\rule{0.3em}{0ex}}\mathrm{K}$. A f…
We show for the system La1-xCexCoO3 (0.1 <= x <= 0.4) that it is possible to synthesize electron-doped cobaltites by the growth of epitaxial thin films. For La1-xCexCoO3, ferromagnetic order is observed within the entire doping range (with the maximum of the Curie temperature, Tc, at x ca. 0.3), resulting in a magneti…
We review the progress in the spatial resolution of atomic force microscopy (AFM) in vacuum. After an introduction of the basic principle and a conceptual comparison to scanning tunneling microscopy, the main challenges of AFM and the solutions that have evolved in the first twenty years of its existence are outlined.…
Pairs of electrodes with nanometer separation (nano-gap) are achieved through an electromigration-induced break-junction (EIBJ) technique at room temperature. Lithographically defined gold (Au) wires are formed by e-beam evaporation over oxide coated silicon substrates silanized with (3-Mercaptopropyl)trimethoxysilane…
The ring-opening polymerization of rac-lactide at a beta-diketiminate magnesium center, [HC{CMeN-2,6-(i)Pr(2)C(6)H(3)}(2)]Mg(OMe)(THF), has been investigated using a B3-LYP density functional procedure employing three different layers of basis set: 6-311G(3d) at the Mg center, 6-31G(d) for both the ligand skeleton and…
Taking advantage of the stability and penetrability of layer-by-layer (LbL) films, we develop a novel method to fabricate a branchlike structure of Ag aggregates on the matrix of a LbL polyelectrolyte multilayer by an electrodeposition technique. The morphology of Ag aggregates can be adjusted by electrodeposition tim…
The mechanism of lasing in single cadmium sulfide (CdS) nanowire cavities was elucidated by temperature-dependent and time-resolved photoluminescence (PL) measurements. Temperature-dependent PL studies reveal rich spectral features and show that an exciton-exciton interaction is critical to lasing up to 75 K, while an…
Paramagnetic lanthanide complexes that display unusually slow water exchange between an inner sphere coordination site and bulk water may serve as a new class of MRI contrast agents with the use of chemical exchange saturation transfer (CEST) techniques. To aid in the design of paramagnetic CEST agents for reporting i…
The present difficulties in synthesis of one-dimensional copper are short length, nonlinear morphology, polydispersivity, poor crystallinity, low yield, and process complexity. In this work, we demonstrate that high-quality ultralong copper nanowires (90-120 nm in diameter, 40-50 microm in length; aspect ratio >350-45…
Electron transfer across the molecule-semiconductor interface is a fundamental process that is relevant to many applications of nanoparticles, such as dye-sensitized solar cells and molecular electronics. This review summarizes recent progress in understanding electron transfer dynamics from molecular adsorbates to se…
Superhydrophobic surfaces have important technical applications ranging from self-cleaning window glasses, paints, and fabrics to low-friction surfaces. The archetype superhydrophobic surface is that of the lotus leaf. When rain falls on lotus leaves, water beads up with a contact angle in the superhydrophobic range o…
A thermodynamic framework is presented for the theory of Viscoplasticity Based on Overstress (VBO) developed by Krempl and co-workers (Krempl, E., and Ho, K., 2001, in Lemaitre Handbook of Materials Behavior Models, Academic Press, New York, pp. 336–348; 2000, in Time Dependent and Nonlinear Effects in Polymers and Co…
A modified experimental apparatus with improved angular resolution and stability has been used to measure the total electron scattering cross sections for $\mathrm{S}{\mathrm{F}}_{6}$ and $\mathrm{S}{\mathrm{F}}_{5}\mathrm{C}{\mathrm{F}}_{3}$ in the energy range of $100--5000\phantom{\rule{0.3em}{0ex}}\mathrm{eV}$. A…
Simulations show that CO2 adsorbed in the groove sites of carbon nanotubes displays unique quasi-one-dimensional behavior. Clusters containing only odd numbers of molecules are formed at finite CO2 coverages and low temperatures. The molecules are orientationally ordered with respect to the nanotube groove axis and az…
This work reports on the investigation of nanosized CeO 2 -ZnO systems prepared by Pechini'smethod. The structural and morphological characterization of CeO 2 -ZnO systems as well as thecharacterization of CeO 2 and ZnO separately, showed that the employed method result in powders withspheroidal particles whose size a…