Materials Literature
按标题、摘要、年份、主题和来源检索公开元数据。结果保留作者、摘要、分类与原始来源链接。
Crystalline materials deform in an intermittent way via dislocation-slip avalanches. Below a critical stress, the dislocations are jammed within their glide plane due to long-range elastic interactions and the material exhibits plastic response, while above this critical stress the dislocations are mobile (the unjamme…
Ultrafast laser-induced demagnetization of Gd(0001) has been investigated by magneto-induced optical second harmonic generation and the magneto-optical Kerr effect which facilitate a comparison of surface and bulk dynamics. We observe pronounced differences in the transient changes of the surface and bulk sensitive ma…
Room temperature Terahertz stimulated emission and population inversion in optically pumped graphene is reported. We experimentally observe fast relaxation and relatively slow recombination dynamics of photogenerated electrons/holes in an exfoliated graphene on SiO2/Si substrate under pumping with a 1550-nm, 80-fs pul…
Three-dimensional (3D) flowerlike hierarchical Fe(3)O(4)@Bi(2)O(3) core-shell architectures were synthesized by a simple and direct solvothermal route without any linker shell. The results indicated that the size of the 3D flowerlike hierarchical microspheres was about 420 nm and the shell was composed of several nano…
We design an anisotropic ultrathin metamaterial to allow perfect transmissions of electromagnetic (EM) waves for two incident polarizations within a common frequency interval. The transparencies are governed by different mechanisms, resulting in significant differences in transmission phase changes for two polarizatio…
Dehydrogenation chemistry with iron: The first examples of efficient iron-catalyzed dehydrocoupling/dehydrogenation of amine–boranes at ambient temperature have been reported. In the case of the primary amine–borane adduct MeNH2⋅BH3, both the polymer and/or N-alkyl borazine can be obtained (see scheme; 1=[{CpFe(CO)2}2…
This paper has been withdrawn by the authors.
A constitutive model based on the combination of damage mechanics and plasticity is developed to analyse concrete structures subjected to dynamic loading. The aim is to obtain a model, which requires input parameters with clear physical meanings. The model should describe the important characteristics of concrete subj…
We present a method for the calculation of electronic structure of systems that contain tens of thousands of atoms. The method is based on the division of the system into mutually overlapping fragments and the representation of the single-particle Hamiltonian in the basis of eigenstates of these fragments. In practice…
We report the first direct observation of a disordered vortex matter phase existing near the edge of a bulk type-II superconductor Nb using a novel position-sensitive neutron diffraction technique. This "edge-contaminated" vortex state was implicated in previous studies using transport techniques and was postulated to…
In this paper, we present three amorphous GaN models obtained from the first principles simulation. We find that a chemically ordered continuous random network is the ideal structure for a-GaN. If we exclude the tail states, we predict a 3.0eV optical gap for 64-atom model and 2.3eV for 250-atom models. We observe a h…
Newly developed fabrication technique of thermoresponsive surface using RAFT-mediated block copolymerization and photolithography achieved stripe-like micropatterning of poly(N-isopropylacrylamide) (PIPAAm) brush domains and poly(N-isopropylacrylamide)-b-poly(N-acryloylmorpholine) domains. Normal human dermal fibrobla…
Light-emitting diodes [LEDs] are of particular interest recently as their performance is approaching fluorescent/incandescent tubes. Moreover, their energy-saving property is attracting many researchers because of the huge energy crisis we are facing. Among all methods intending to enhance the efficiency and intensity…
We report a detailed high-resolution powder neutron diffraction investigation of the structural behavior of the multiferroic hexagonal polymorph of YMnO${}_{3}$ between room temperature and 1403 K. The study was aimed at resolving previous uncertainties regarding the nature of the paraelectric-ferroelectric transition…
High resolution angle-resolved photoemission measurements have been carried out to study the electronic structure and superconducting gap of the $({\mathrm{Tl}}_{0.58}{\mathrm{Rb}}_{0.42}){\mathrm{Fe}}_{1.72}{\mathrm{Se}}_{2}$ superconductor with a ${T}_{c}=32\text{ }\text{ }\mathrm{K}$. The Fermi surface topology con…
Charging clusters: A hybrid of polyoxometalate (POM) molecules individually adsorbed onto the surfaces of single-wall carbon nanotubes (SWNTs) can be used as a cathode-active material in rechargeable lithium batteries. This POM/SWNT battery exhibited a very high capacity (>300 Ah kg−1) with a short charging/dischargin…
Metastasis is a multistep process that culminates in the spread of cells from a primary tumor to a distant site or organs. For tumor cells to be able to metastasize, they have to locally invade through basement membrane into the lymphatic and the blood vasculatures. Eventually they extravasate from the blood and colon…
Atomistic molecular dynamics simulations of a composite consisting of an ungrafted or a grafted spherical silica nanoparticle embedded in a melt of 20-monomer atactic polystyrene chains have been performed. The structural properties of the polymer in the vicinity of a nanoparticle have been studied. The nanoparticle m…
A novel method of rare-earth cation-assisted ligand assembly has been developed to provide upconversion nanophosphors with T(1)-enhanced magnetic resonance (MR), radioactivity, and targeted recognition properties, making these nanoparticles potential candidates for multimodal bioimaging. The process of modifying the s…
In this Article, we present our findings on the formation of metal sulfide nanocrystals from sulfur-alkylamine solutions. By pulsed field gradient diffusion NMR along with the standard toolbox of 1D and 2D NMR, we determined that sulfur-amine solutions used as a sulfur precursor exist as alkylammonium polysulfides at…