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Evidence of photo- and electrodarkening of (CdSe)ZnS quantum dot composites

J. Rodríguez‐Viejo、Hedi Mattoussi、Johanna Heine 等 7 位作者2000-06-15Journal of Applied Physics

We present a study of the kinetics of photoluminescence (PL) and cathodoluminescence (CL) degradation of semiconductor quantum dot composites, formed by highly luminescent (CdSe)ZnS core-shell nanocrystals embedded in a ZnS matrix. The photoluminescence and cathodoluminescence spectra indicate that both emissions orig…

Perovskite Materials and ApplicationsQuantum Dots Synthesis And PropertiesChalcogenide Semiconductor Thin Films

The Archaeon Sulfolobus solfataricus Contains a Membrane-Associated Protein Kinase Activity That Preferentially Phosphorylates Threonine Residues In Vitro

Brian H. Lower、Kenneth M. Bischoff、Peter J. Kennelly2000-06-15Journal of Bacteriology

The extreme acidothermophilic archaeon Sulfolobus solfataricus harbors a membrane-associated protein kinase activity. Its solubilization and stabilization required detergents, suggesting that this activity resides within an integral membrane protein. The archaeal protein kinase utilized purine nucleotides as phosphory…

Bacterial Genetics and BiotechnologyCellular transport and secretionEnzyme Structure and Function

Double-helical network in amylose as seen by slow calorimetry and FTIR

Paul Bernazzani、Camille Chapados、G. Delmas2000-06-15Journal of Polymer Science Part B Polymer Physics

The phase content and crystallinity of initially amorphous amylose–water mixtures (70/30 W/W) have been changed by slow cycles of dissolution and recrystallization from Tmax with 50 °C < Tmax < 120 °C. Analysis of the treatment-induced changes is made by X-ray diffraction, FTIR, fast T-ramp DSC and slow calorimetry. O…

Food composition and propertiesbiodegradable polymer synthesis and propertiesPolysaccharides Composition and Applications

Metal-insulator transition, gap opening due to the combined orbital-spin ordering, and spin-triplet superconductivity

Andrzej Klejnberg、J. Spałek2000-06-15Physical review. B, Condensed matter

We consider a metal-insulator transition for the quarter-filled doubly degenerate band of correlated electrons, as well as the onset of the itinerant orbitally ordered phase combined with the saturated ferromagnetism near that limit. The insulating state is instable with respect to either spin-triplet superconductivit…

Magnetic and transport properties of perovskites and related materialsRare-earth and actinide compoundsAdvanced Condensed Matter Physics

Exciton states and optical spectra in CdSe nanocrystallite quantum dots

Jingbo Li、Jian‐Bai Xia2000-06-15Physical review. B, Condensed matter

By using the hole effective-mass Hamiltonian for semiconductors with the wurtzite structure, we have studied the exciton states and optical spectra in CdSe nanocrystallite quantum dots. The intrinsic asymmetry of the hexagonal lattice structure and the effect of spin-orbital coupling (SOC) on the hole states are inves…

Semiconductor Quantum Structures and DevicesQuantum Dots Synthesis And PropertiesChalcogenide Semiconductor Thin Films

Non-monotonous crossover between capillary condensation and interface localisation/delocalisation transition in binary polymer blends

Marcus Müller、Kurt Binder、Ezequiel V. Albano2000-06-15Europhysics Letters (EPL)

Within self-consistent field theory we study the phase behaviour of a symmetric binary AB polymer blend confined into a thin film. The film surfaces interact with the monomers via short-range potentials. One surface attracts the A component and the corresponding semi-infinite system exhibits a first-order wetting tran…

Rheology and Fluid Dynamics StudiesBlock Copolymer Self-AssemblyFluid Dynamics and Thin Films

Structure Formation of Isotactic Polypropylene from the Glass

Yoshihisa Miyamoto、Koji Fukao、Tomoko Yoshida 等 5 位作者2000-06-15Journal of the Physical Society of Japan

The structure formation process of isotactic polypropylene (itPP) from the glass into the “smectic” mesophase has been studied by small-angle x-ray scattering, wide-angle x-ray scattering and differential scanning calorimetry. The structure of the smectic phase was unaltered during the transition process, which indica…

Polymer crystallization and propertiesPolymer Nanocomposites and Propertiesbiodegradable polymer synthesis and properties

Magnetic properties of BaFe12−2xZnxZrxO19 particles

F. L. Wei、Hanyan Fang、C. K. Ong 等 5 位作者2000-06-15Journal of Applied Physics

ZnZr doped barium ferrite single domain particles BaFe12−2xZnxZrxO19 with 0⩽x⩽0.8 were prepared by the chemical coprecipitation method. With increasing doping concentration x, the magnetocrystalline anisotropy and thus the coercivity was drastically decreased. This was mainly due to the substitution of Fe3+ ions in th…

Magnetic properties of thin filmsMultiferroics and related materialsMagnetic Properties and Synthesis of Ferrites

Spiralling optical morphologies in spherulites of poly(hydroxybutyrate)

Jamie K. Hobbs、D. R. Binger、A. Keller 等 4 位作者2000-06-15Journal of Polymer Science Part B Polymer Physics

Some rather unusual optical morphologies in thin films of poly(hydroxybutyrate) in which a temperature gradient is imposed across the thickness of the film are reported. Spherulites in which the Maltese cross degenerates into a continuous spiral grow under these conditions, and the direction of the rotation of the spi…

Polymer crystallization and propertiesbiodegradable polymer synthesis and propertiesPolymer composites and self-healing

In situTEM evaluation of the growth kinetics of Au particles on highly oriented pyrolithic graphite at elevated temperatures

R. Antón、P. Kreutzer2000-06-15Physical review. B, Condensed matter

Gold particles were vapor deposited onto thin substrates of highly oriented graphite at temperatures from 250 to 350 \ifmmode^\circ\else\textdegree\fi{}C inside a transmission electron microscope. The growth kinetics of individual particles were recorded in real time. Mostly well faceted, flat crystallites grew in epi…

Electron and X-Ray Spectroscopy Techniquesnanoparticles nucleation surface interactionsSurface and Thin Film Phenomena

Regulation of biodegradability and drug release behavior of aliphatic polyesters by blending

Youqing Shen、Weilin Sun、K. J. Zhu 等 4 位作者2000-06-15Journal of Biomedical Materials Research

Polyester blending of poly(epsilon-caprolactone) (PCL) with poly(D, L-lactide) (PLA) and their random copolymers (R(CL/LA)) was found to be a convenient approach to regulate the degradation and drug release behaviors of the polyesters. The blend composition and compatibility both affected its degradation and drug rele…

Advanced Polymer Synthesis and Characterizationbiodegradable polymer synthesis and propertiesPolymer Surface Interaction Studies

Observation of developmental processes in loosely attached diatom (Bacillariophyceae) communities

Akihiro Tuji2000-06-15Phycological Research

SUMMARY The succession of attached algal communities was studied in Lake Biwa and the Omiya River. After the ‘climax’ which was characterized by large numbers of Cymbella turgidula Grunow and Gomphoneis quadripunctatum (Ostrup) P. Dawson, the community was dominated by species attached directly to stalks or tangled am…

Marine and coastal ecosystemsAquatic Ecosystems and Phytoplankton DynamicsDiatoms and Algae Research

Novel polyesters with amino-sulfone azobenzene chromophores in the main chain

Zusheng Xu、V. Drnoyan、Almeria Natansohn 等 4 位作者2000-06-15Journal of Polymer Science Part A Polymer Chemistry

The synthesis and optical properties of a series of amorphous polyesters with amino-sulfone azobenzene chromophores in the main chain are presented. The condensation of alkyl diacid chlorides with 4-[(2-hydroxyethyl)ethylamino]-4′-(2-hydroxyethylsulfonyl)azobenzene (7) gave polymers that showed low and unstable photoi…

Photonic and Optical DevicesLiquid Crystal Research AdvancementsSynthesis and properties of polymers

Homoepitaxial growth mechanism of ZnO(0001): Molecular-dynamics simulations

Momoji Kubo、Yasunori Oumi、Hiromitsu Takaba 等 8 位作者2000-06-15Physical review. B, Condensed matter

We clarified here an epitaxial growth mechanism of ZnO(0001) surface on an atomic scale, by using molecular-dynamics crystal-growth simulations. It was observed that the crystal growth starts at the step of ZnO(0001), but not at the terrace of ZnO(0001). This phenomenon is clearly justified from the coordination numbe…

ZnO doping and propertiesCopper-based nanomaterials and applicationsGa2O3 and related materials

Electronic specific heat at the boundary region of the metal-insulator transition in the two-dimensional electronic system ofκ−(BEDT−TTF)2Cu[N(CN)2]Br

Yasuhiro Nakazawa、Hiromi Taniguchi、Atsushi Kawamoto 等 4 位作者2000-06-15Physical review. B, Condensed matter

The electronic specific heat of partially deuterated organic conductors $\ensuremath{\kappa}\ensuremath{-}{(\mathrm{B}\mathrm{E}\mathrm{D}\mathrm{T}\ensuremath{-}\mathrm{T}\mathrm{T}\mathrm{F})}_{2}{\mathrm{Cu}[\mathrm{N}(\mathrm{CN})}_{2}]\mathrm{B}\mathrm{r},$ [where BEDT-TTF denotes bis(ethylenedithio)tetrathiafulv…

Physics of Superconductivity and MagnetismMagnetism in coordination complexesOrganic and Molecular Conductors Research

Theory for Photoinduced Ionic-Neutral Structural Phase Transition in Quasi One-Dimensional Organic Molecular Crystal TTF-CA

Ping Huai、Hang Zheng、Keiichirō Nasu2000-06-15Journal of the Physical Society of Japan

Using a quasi one-dimensional extended Peierls-Hubbard model, we theoretically study the photoinduced ionic-neutral structural phase transition in an organic molecular chain crystal TTF-CA, by means of the adiabatic approximation and the mean-field theory. This model includes strong intra-chain Coulomb interactions wh…

Organic Light-Emitting Diodes ResearchMagnetism in coordination complexesOrganic and Molecular Conductors Research

Optical spectra and electronic structures of lead halides

M. Fujita、Minoru Itoh、Yoshitoshi Bokumoto 等 6 位作者2000-06-15Physical review. B, Condensed matter

Polarized reflectivity spectra of single crystals of $\ensuremath{\alpha}\ensuremath{-}{\mathrm{PbF}}_{2},$ $\ensuremath{\beta}\ensuremath{-}{\mathrm{PbF}}_{2},$ ${\mathrm{PbCl}}_{2},$ and ${\mathrm{PbBr}}_{2}$ have been measured at 10 K in the energy range up to 30 eV using synchrotron radiation as a light source. Th…

Luminescence Properties of Advanced MaterialsSolid-state spectroscopy and crystallographyInorganic Fluorides and Related Compounds

Interchain conductivity of coupled Luttinger liquids and organic conductors

Antoine Georges、Thierry Giamarchi、Nancy Sandler2000-06-15Physical review. B, Condensed matter

We reconsider the theory of dc and ac interchain conductivity in quasi-one dimensional systems. Our results are in good agreement with the measured c-axis optical conductivity of ${(\mathrm{TMTSF})}_{2}{\mathrm{ClO}}_{4}$ and suggest that the c-axis dc conductivity of ${(\mathrm{TMTSF})}_{2}{\mathrm{PF}}_{6}$ in the $…

Physics of Superconductivity and MagnetismQuantum and electron transport phenomenaOrganic and Molecular Conductors Research

Chemical functionalization of carbon nanotubes through energetic radical collisions

Boris Ni、Susan B. Sinnott2000-06-15Physical review. B, Condensed matter

Classical molecular dynamics simulations are used to model the bombardment of a bundle of single walled carbon nanotubes by ${\mathrm{CH}}_{3}$ radicals impacting with incident energies of 10, 45, and 80 eV. The simulations show that there is a high probability of adhesion of either the radicals or their fragments to…

Carbon Nanotubes in CompositesIon-surface interactions and analysisGraphite, nuclear technology, radiation studies

Site-selective yellow to violet and near-infrared to green upconversion inBaLu2F8:Nd3+

Oliver S. Wenger、Daniel R. Gamelin、Hans U. Güdel 等 5 位作者2000-06-15Physical review. B, Condensed matter

Single crystals of ${\mathrm{BaLu}}_{2}{\mathrm{F}}_{8}$ doped with 0.6% ${\mathrm{Nd}}^{3+}$ were studied by high-resolution optical absorption, luminescence, and excitation spectroscopy in the 15--300 K temperature range. The two crystallographically distinct sites for the dopant ions present in this host are identi…

Luminescence Properties of Advanced MaterialsMagnetism in coordination complexesInorganic Fluorides and Related Compounds