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On the solubility of rare earths in M-type SrFe12O19hexaferrite compounds

L. Lechevallier、J.M. Le Breton、A. Morel 等 4 位作者2008-04-03Journal of Physics Condensed Matter

Sr 1− x RE x Fe 12 O 19 and Sr 1− x RE x Fe 12− x Co x O 19 ( x = 0–0.4 and RE = Pr, Nd) M-type hexaferrite powders were produced by a conventional ceramic process. Structural investigations made by x-ray diffraction and Mössbauer spectrometry reveal that the solubility of the rare earth ion in the M-type phase depend…

Magnetic Properties and Synthesis of FerritesIron oxide chemistry and applicationsMultiferroics and related materials

Er3+and Yb3+concentration effect in the spectroscopic properties and energy transfer in Yb3+/Er3+codoped tellurite glasses

H. Desirena、E. De la Rosa、A Shulzgen 等 5 位作者2008-04-03Journal of Physics D Applied Physics

Spectroscopic properties of Yb3+/Er3+ codoped tellurite glasses as a function of Er3+ and Yb3+ concentration have been investigated. Under 970 nm excitation three strong up-conversion emission bands centred at 525, 546 and 656 nm were observed, and the characteristic near infrared emission band was centred at 1.53 µm.…

Solid State Laser TechnologiesLuminescence Properties of Advanced MaterialsGlass properties and applications

Direct Measurement of Strain-Induced Changes in the Band Structure of Carbon Nanotubes

Mingyuan Huang、Yang Wu、Bhupesh Chandra 等 7 位作者2008-04-03Physical Review Letters

The effect of uniaxial strain on the optical transition energies of single-walled carbon nanotubes with known chiral indices was measured by Rayleigh scattering spectroscopy. Existing theory accurately predicts the trends in the measured strain-induced shifts, but overestimates their magnitude. Modification of the ana…

Carbon Nanotubes in CompositesMechanical and Optical ResonatorsGraphene research and applications

Dye reorientation as a probe of stress-induced mobility in polymer glasses

Hau-Nan Lee、Keewook Paeng、Stephen F. Swallen 等 4 位作者2008-04-03The Journal of Chemical Physics

The reorientation of dye molecules can be used to monitor the segmental dynamics of a polymer melt. We utilize this technique to measure stress-induced mobility in a lightly cross-linked poly(methyl methacrylate) (PMMA) glass during tensile creep deformation. At 377 K (18 K below the glass transition temperature Tg),…

Liquid Crystal Research AdvancementsPolymer crystallization and propertiesMaterial Dynamics and Properties

Effect of Phonon-Phonon Interactions on Localization

Abhishek Dhar、Joel L. Lebowitz2008-04-03Physical Review Letters

We study the heat current J in a classical one-dimensional disordered chain with on-site pinning and with ends connected to stochastic thermal reservoirs at different temperatures. In the absence of anharmonicity all modes are localized and there is a gap in the spectrum. Consequently J decays exponentially with syste…

Advanced Thermodynamics and Statistical MechanicsQuantum many-body systemsThermal properties of materials

Viscous Friction in Foams and Concentrated Emulsions under Steady Shear

Nikolai D. Denkov、Slavka Tcholakova、Konstantin Golemanov 等 5 位作者2008-04-03Physical Review Letters

We present a model for the viscous friction in foams and concentrated emulsions, subject to steady shear flow. First, we calculate the energy dissipated due to viscous friction inside the films between two neighboring bubbles or drops, which slide along each other in the flow. Next, from this energy we calculate the m…

Rheology and Fluid Dynamics StudiesPickering emulsions and particle stabilizationHeat and Mass Transfer in Porous Media

TarO: a target optimisation system for structural biology

Ian M. Overton、C. A. Johannes van Niekerk、Lester G. Carter 等 11 位作者2008-04-03Nucleic Acids Research

TarO (http://www.compbio.dundee.ac.uk/taro) offers a single point of reference for key bioinformatics analyses relevant to selecting proteins or domains for study by structural biology techniques. The protein sequence is analysed by 17 algorithms and compared to 8 databases. TarO gathers putative homologues, including…

Advanced Proteomics Techniques and ApplicationsEnzyme Structure and FunctionGenomics and Phylogenetic Studies

Variably Isotactic Poly(hydroxybutyrate) from Racemic β‐Butyrolactone: Microstructure Control by Achiral Chromium(III) Salophen Complexes

Manuela Zintl、F. Molnár、Tobias Urban 等 6 位作者2008-04-03Angewandte Chemie International Edition

ROP artists: The ROP of racemic β-butyrolactone (BL) catalyzed by highly active chromium(III) salophen complexes 1 gives poly(hydroxybutyrate) (PHB) with high molecular weight and with isotacticities of 60–70 %. The product is a biodegradable polymer material with mechanical properties that can be varied from crystall…

Carbon dioxide utilization in catalysisOrganometallic Complex Synthesis and Catalysisbiodegradable polymer synthesis and properties

Guide to collagen characterization for biomaterial studies

Leah C. Abraham、Erin Zuena、Bernardo Pérez-Ramírez 等 4 位作者2008-04-03Journal of Biomedical Materials Research Part B Applied Biomaterials

The structure and remodeling of collagen in vivo is critical to the pathology and healing of many human diseases, as well as to normal tissue development and regeneration. In addition, collagen matrices in the form of fibers, coatings, and films are used extensively in biomaterial and biomedical applications. The spec…

Collagen: Extraction and CharacterizationBone Tissue Engineering MaterialsSilk-based biomaterials and applications

Characteristics of hydrogen co-doped ZnO : Al thin films

S H Lee、T S Lee、K S Lee 等 6 位作者2008-04-03Journal of Physics D Applied Physics

ZnO films co-doped with H and Al (HAZO) were prepared by sputtering ZnO targets containing 1 wt% Al 2 O 3 on Corning glass at a substrate temperature of 150 °C with Ar and H 2 /Ar gas mixtures. The effects of hydrogen addition to Al-doped ZnO (AZO) films with low Al content on the electrical, the optical and the struc…

Copper-based nanomaterials and applicationsGas Sensing Nanomaterials and SensorsZnO doping and properties

Designs for optical cloaking with high-order transformations

Wenshan Cai、Uday K. Chettiar、Alexander V. Kildishev 等 4 位作者2008-04-03Optics Express

Recent advances in metamaterial research have provided us a blueprint for realistic cloaking capabilities, and it is crucial to develop practical designs to convert concepts into real-life devices. We present two structures for optical cloaking based on high-order transformations for TM and TE polarizations respective…

Advanced Antenna and Metasurface TechnologiesOrbital Angular Momentum in OpticsMetamaterials and Metasurfaces Applications

Floating Tip Nanolithography

Alexander A Milner、Kaiyin Zhang、Yehiam Prior2008-04-03arXiv

We demonstrate noncontact, high quality surface modification with spatial resolution of ~20 nm. The nanowriting is based on the interaction between the surface and the tip of an Atomic force microscope illuminated by a focused laser beam and hovering 1-4 nanometers above the surface without touching it. The floating t…

Materials Science

Charge fluctuations and feedback effect in shot noise in a Y-terminal system

Bogdan R. Bulka2008-04-03arXiv

We investigate a dynamical Coulomb blockade effect and its role in the enhancement of current-current correlations in a three-terminal device with a multilevel splitter, as well as with two quantum dots. Spectral decomposition analysis shows that in the Y-terminal system with a two level ideal splitter, charge fluctua…

Materials Science

Molar volume of solid isotopic helium mixtures

Carlos P. Herrero2008-04-03arXiv

Solid isotopic helium mixtures have been studied by path-integral Monte Carlo simulations in the isothermal-isobaric ensemble. This method allowed us to study the molar volume as a function of temperature, pressure, and isotopic composition. At 25 K and 0.2 GPa, the relative difference between molar volumes of isotopi…

Materials Science

A microscopic modeling of phonon dynamics and charge response in NdCuO

Thomas Bauer、Claus Falter2008-04-03arXiv

A description of phonon dynamics and charge response of the $n$-doped high-temperature superconductor (HTSC) NdCuO is presented based upon a microscopic modeling of the electronic density response. This is accomplished starting from the insulating state via the underdoped strange metallic to the more conventional meta…

SuperconductivityMaterials Science

Thermal rectifiers from deformed carbon nanohorns

Gang Wu、Baowen Li2008-04-03Journal of Physics Condensed Matter

We study thermal rectification in single-walled carbon nanohorns (SWNHs) by using a non-equilibrium molecular dynamics (MD) method. It is found that the horns with the bigger top angles show larger asymmetric heat transport due to the larger structural gradient distribution. This kind of gradient behavior can be furth…

Nanopore and Nanochannel Transport StudiesCarbon Nanotubes in CompositesThermal properties of materials

Polarization Saturation in Strained Ferroelectrics

Yanpeng Yao、Huaxiang Fu2008-04-03arXiv

Using density-functional calculations we study the structure and polarization response of tetragonal PbTiO3, BaTiO3 and SrTiO3 in a strain regime that is previously overlooked. Different from common expectations, we find that the polarizations in all three substances saturate at large strains, demonstrating a universa…

Materials Science

Spin dependent impurity effects in the 2D frustrated magnetism of NiGa$_2$S$_4$

Yusuke Nambu、Satoru Nakatsuji、Yoshiteru Maeno 等 5 位作者2008-04-03arXiv

Impurity effects on the triangular antiferromagnets Ni$_{1-x}M_x$Ga$_2$S$_4$ ($M=$ Mn, Fe, Co and Zn) are studied. The 2D frozen spin-disordered state of NiGa$_2$S$_4$ is stable against the substitution of Zn$^{2+}$ ($S=0$) and Heisenberg Fe$^{2+}$ ($S=2$) spins, and exhibits a $T^2$-dependent magnetic specific heat,…

Materials ScienceStrongly Correlated Electrons

Yeast Cells with an Artificial Mineral Shell: Protection and Modification of Living Cells by Biomimetic Mineralization

Ben Wang、Peng Liu、Wenge Jiang 等 6 位作者2008-04-03Angewandte Chemie International Edition

Inspired by eggshells in nature, living yeast cells were conferred with an artificial mineral coat by using a combination of the layer-by-layer (LBL) treatment with functional polymers and in situ biomimetic mineralization. The resulting hard inorganic shells have a tremendous effect on the storage, protection, delive…

Polymer Surface Interaction StudiesBone Tissue Engineering Materialsbiodegradable polymer synthesis and properties