Materials Literature
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Spider silks are among the strongest and toughest known materials, but investigation of these remarkable properties has been confined largely to orb-weaving spiders. We investigated the mechanical performance of silk from the cobweb-weaving spider Latrodectus hesperus. Both silk from the scaffolding region of the web…
The Néel temperature of Ni0.5Zn0.5Fe2O4 spinel ferrite increases significantly from 538K in the bulk state to 592K when the grain size is reduced to 16nm by milling in a high-energy ball mill. This has been attributed to an increase in the AB superexchange interaction strength due to a possible enhancement in the magn…
High temperature ferromagnetism in thin films of dilute magnetic oxides is a widespread phenomenon, of which there appear to be two sources. One is the contribution of the 3d dopant ions themselves, the other is related to crystal defects in the interface region. The latter contributes a magnetic moment of 100–400μB p…
Current–voltage measurements of Au contacts deposited on ex situ cleaned, n-type ZnO(0001) [(0001¯)] surfaces showed reverse bias leakage current densities of ∼0.01(∼0.1)A∕cm2 at 4.6 (3.75) V reverse bias and ideality factors >2 (both surfaces) before sharp, permanent breakdown (soft breakdown). This behavior w…
Highly homogeneous and luminescent CdSe colloidal nanocrystals in the less common zinc blende crystal structure have been obtained at high temperature in a noncoordinating organic solvent. The key parameter appears to be the addition of a phosphonic acid to the trioctylphosphine-selenium complex before its injection i…
The local and intermediate structure of stoichiometric LaMnO3 has been studied in the pseudocubic and rhombohedral phases at high temperatures (300-1150 K). Neutron powder diffraction data were collected and a combined Rietveld and high real space resolution atomic pair distribution function analysis was carried out.…
A simple model of thermal conductivity, based on the harmonic theory of solids, is used to study the heat transfer in nanostructures. The thermal conductivity is obtained by summing the contribution of all the vibration modes of the system. All the vibrational properties (dispersion curves and relaxation time) that ar…
Through nonequilibrium rf magnetron cosputtering of ZnO and Cr metal on a-plane Al2O3 we find ferromagnetic ordering with a room-temperature saturation moment of 1.4μB per Cr ion at a doping concentration of ∼9.5 at. % after UHV postanneal. No secondary phases are detected in the films via x-ray diffraction (XRD). Inc…
Resonance Raman spectroscopy/microscopy was used to study individualized single-walled carbon nanotubes (SWNTs) both in aqueous suspensions as well as after spin-coating onto Si/SiO2 surfaces. Four different SWNT materials containing nanotubes with diameters ranging from 0.7 to 1.6 nm were used. Comparison with Raman…
The white-light long-lasting phosphor CaAl2O4:Dy3+ was prepared and investigated. The white-light afterglow spectra under the irradiation of 254 or 365nm are comprised of the blue light emission and the yellow light emission, originating from the transitions of F9∕24→H15∕26, F9∕24→H13∕26 in the 4f9 configuration of Dy…
A simple approximate expression in real and reciprocal spaces is given for the static exchange-correlation kernel of a uniform electron gas interacting with the long-range part only of the Coulomb interaction. This expression interpolates between the exact asymptotic behaviors of this kernel at small and large wave ve…
This paper derives expressions for the critical current at the onset of spin-transfer-torque (STT) instability in CPP-GMR read heads, as a function of the relative angle (theta) between the free and reference layer magnetizations. Including a general angular dependent STT coefficient B(q=cos(theta)) exclusive of the a…
We report on a atomistic theory of electronic structure and optical properties of a single InAs quantum dot grown on InP patterned substrate. The spatial positioning of individual dots using InP nano-templates results in a quantum dot embedded in InP pyramid. The strain distribution of a quantum dot in InP pyramid is…
We predict bistability in the Curie temperature-voltage characteristic of double barrier resonant-tunneling structures with dilute ferromagnetic semiconductor quantum wells. Our conclusions are based on simulations of electrostatics and ballistic quantum transport combined with a mean-field theory description of ferro…
We report an experimental and a theoretical study of the radial elasticity of multiwalled carbon nanotubes as a function of external radius. We use atomic force microscopy and apply small indentation amplitudes in order to stay in the linear elasticity regime. The number of layers for a given tube radius is inferred f…
Electrospinning is a simple and versatile technique of producing polymeric fibers ranging from submicron to micron in diameter. Incorporation of bioactive agents into the fibers could make a biofunctional tissue engineering scaffold. In this study, we investigated the feasibility of encapsulating human beta-nerve grow…
We report a first-principles study, which demonstrates that a single Ti atom coated on a single-walled nanotube (SWNT) binds up to four hydrogen molecules. The first H2 adsorption is dissociative with no energy barrier while the other three adsorptions are molecular with significantly elongated H-H bonds. At high Ti c…
Optical transitions in carbon nanotubes are of central importance for nanotube characterization. They also provide insight into the nature of excited states in these one-dimensional systems. Recent work suggests that light absorption produces strongly correlated electron-hole states in the form of excitons. However, i…
A theory of reversible susceptibility tensor based on magnetization vector dynamics, as described by the Landau–Lifshitz equation of motion, is given. It is shown that the reversible transverse susceptibility (RTS) is in fact the zero frequency limit of the ferromagnetic resonance (FMR). Thus, the methods which have b…
The quartz crystal microbalance (QCM) method was used to obtain precise information about the dissolution behavior of resist polymers. The time evolutions of the resonance frequency and the impedance during the dissolution were measured using the QCM method. The data were simulated using the transmission line method o…