Materials Literature
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<div class="htmlview paragraph">This paper summarizes results from a large study on the release of NO<sub>x</sub> from a lean NO<sub>x</sub> trap during rich purges. Under certain purge conditions, some NO<sub>x</sub> trap formulations have the propensity to release some of th…
The excimer fluorescence of a bis-pyrene molecule can be reversibly regulated by ultraviolet light, metal ions and visible light in the presence of spiropyran. Based on this result, a new molecular logic circuit is proposed.
The linewidth of longitudinal acoustic waves in densified silica glass is obtained by inelastic x-ray scattering. It increases with a high power alpha of the frequency up to a crossover where the waves experience strong scattering. We find that alpha is at least 4, and probably larger. Resonance and hybridization of a…
Acetylsalicylic acid reacts with gadolinium(III) ions to yield a new gadolinium complex (1) displaying a chain structure which has been determined by single crystal X-ray crystallography: monoclinic P21/n (no. 14), a = 13.5709(13), b = 6.7141(9), c = 22.7232(17) Å, β = 99.705(14)°, Z = 4. The thermal dependence of the…
Abstract The synthesis of a new bis(ether carboxylic acid), 2,2′‐bis(4‐carboxyphenoxy)‐9,9′‐spirobifluorene, in which two orthogonally arranged carboxyphenoxyfluorene entities are connected through an sp 3 carbon atom (the spiro center), is reported. The direct phosphorylation polycondensation of this diacid monomer w…
This work reports on the development and characterization of novel meltable polymers and composites based on casein and soybean proteins. The effects of inert (Al(2)O(3)) and bioactive (tricalcium phosphate) ceramic reinforcements over the mechanical performance, water absorption, and bioactivity behavior of the injec…
Recent photoemission spectra of the perovskite series CaxSr1-xVO3 revealed strong modifications associated with surface contributions. To study the effect of Coulomb correlations in the bulk and at the surface, the quasiparticle spectra are evaluated using the dynamical mean field theory. It is shown that as a result…
The interaction of C60 with single-wall carbon nanotubes (SWNTs) and graphite is studied experimentally by thermal desorption spectroscopy and theoretically by molecular-mechanics and molecular-dynamics calculations. The van der Waals parameters and force field for C60-graphene and C60-SWNT interactions are derived fr…
Using molecular dynamics simulations, we show that a simple model of a glassy material exhibits the shear localization phenomenon observed in many complex fluids. At low shear rates, the system separates into a fluidized shear band and an unsheared part. The two bands are characterized by a very different dynamics pro…
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The crystal structure, magnetization and electrical resistivity properties of the anion-deficient La 1− x Ba x MnO 3− x /2 (0 ≤ x ≤ 0.50) perovskite manganites without Mn 4+ ions have been investigated. It is established the reduced samples in the region 0 ≤ x ≤ 0.05 are O′-orthorhombic perovskites, in 0.10 ≤ x ≤ 0.25…
The temperature dependence of the superlattice reflections: a) F spots and b) alpha spots in a lead magnesium niobate (PMN) single crystals containing 0% and 6% of PbTiO3 (PT) has been studied using synchrotron x-ray scattering techniques. (No superlattice reflections were found in PMN doped with 32% PT). Analysis of…
The microscopic mechanism of the melting of a crystal is analyzed by the constant-pressure Monte Carlo simulation of a Lennard-Jones fcc system. Beyond a temperature of the order of 0.8 of the melting temperature, we found that the relevant excitations are lines of defects. Each of these lines has the structure of a r…
Temperature dependent studies of the 1/2(hk0) superlattice reflections αspots by synchrotron x-ray scattering measurements were performed in (PMN) and (PMN-xPT) with Ti doping x<0.32 single crystals. Separation of the αspots from the underlying diffuse scattering background allowed studying them as separate entities f…
The critical current density (Jc) of hot isostatic pressed (HIPed) MgB2 wires, measured by d.c. transport and magnetization, is compared with that of similar wires annealed at ambient pressure. The HIPed wires have a higher Jc than the annealed wires, especially at high temperatures and magnetic fields, and higher irr…
Reflection electron energy loss spectroscopy (EELS) in specular and off specular geometry has been employed to study the early stage of the copper phthalocyanine (CuPc) growth on Al (100) substrate. EEL spectroscopy has been a useful tool in order to study electronic structure of molecular films also in the submonolay…
Mn-Ce mixed-oxide catalyst yields nearly 100% NO conversion at 100-150 degrees C at a high space velocity of 42,000 h(-1). SO2 and H2O (at high concentrations) have only slight effects on the activity.
Temperature-dependent Brillouin scattering studies have been carried out on La_{0.77}Ca_{0.23}MnO_3 across the paramagnetic insulator - ferromagnetic metal (I-M) transition. The spectra show a surface Rayleigh wave (SRW) and a high velocity pseudo surface acoustic wave (HVPSAW) besides bulk acoustic waves (BAW). The B…
We argue that an ionic lattice surrounded by a Fermi liquid changes phase several times under pressure, oscillating between the symmetric phase and a low-symmetry dimerized structure, as a consequence of Friedel oscillations in the pair potential. Phase oscillations explain the tendency towards dimerization which has…
While attempting to find a suitable crosslinking reagent for biopolymers, a naturally occurring proanthocyanidin (PA) obtained from grape seeds was selected to fix biological tissues. The cytotoxicity and crosslinking rate, reflected by the in vitro and in vivo degradation of fixed matrices has been studied. The shrin…