Materials Literature
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We use the 1-bond -> 2-phonon percolation doublet of zincblende alloys as a mesoscope for an unusual insight into their phonon behavior under pressure. We focus on (Zn,Be)Se and show by Raman scattering that the original Be-Se doublet at ambient pressure, of the stretching-bending type, turns into a pure-bending singl…
We present theoretical evidence for local magnetic moments on Ti3+ ions in oxygen-deficient anatase and rutile TiO2 observed in a recent experiment [S. Zhou, et al., Phys. Rev. B 79, 113201 (2009)]. Results of our first-principles GGA+U calculations reveal that an oxygen vacancy converts two Ti4+ ions to two Ti3+ ions…
We have implemented a virtual Young's double slit experiment for hard X-ray photons with micro-fabricated bi-prisms. We observe fringe patterns with a scintillator, and quantify interferograms by detecting X-ray fluorescence from a scanned 30nm Cr metal film. The observed intensities are best modeled with a near-field…
Changing the morphology of the growing surface and the nature of residual impurities in (Ge,Mn) layers - by using different substrates - dramatically changes the morphology of the ferromagnetic Mn-rich inclusions and the magnetotransport properties. We obtained p-type layers with nanocolumns, either parallel or entang…
Recently spin-transistors receive considerable attention as a highly-functional building block of future integrated circuits. In order to realize spin-transistors, it is essential that technology of efficient spin injection/detection for semiconductor channel is established. However, this is not so easy challenge owin…
Different thicknesses of cobalt thin films were growth by magnetron sputtering deposition techniques. The films thicknesses were determinated with X ray Photoelectron Spectroscopy (XPS) and Quartz Crystal Monitoring (QCM). XPS is also used to determinate the films quality. The films magnetic properties were determinat…
Magnetoelectric phase diagrams of the perovskite manganites, Eu1-xYxMnO3 and Gd1-xTbxMnO3, are theoretically studied. We first construct a microscopic model, and then analyze the model using the Monte-Carlo method. We reproduce the diagrams, which contain two different multiferroic states, i.e., the ab-plane spin cycl…
Inorganic–organic composite films for rewritable optical storage are fabricated base on the reversible luminescence modulation of ordered upconversion nanopatterns via a photochromic diarylethene. The near-IR excitation for reading the upconversion emission does not affect the recorded data bits. Moreover, the spatial…
We demonstrate circular dichroism (CD) in the second harmonic generation (SHG) signal from chiral assemblies of G-shaped nanostructures made of gold. The arrangement of the G shapes is crucial since upon reordering them the SHG-CD effect disappears. Microscopy reveals SHG "hotspots" assemblies, which originate in enan…
Diamond nanoparticles (nanodiamonds) have been recently proposed as new labels for cellular imaging. For small nanodiamonds (size <40 nm), resonant laser scattering and Raman scattering cross sections are too small to allow single nanoparticle observation. Nanodiamonds can, however, be rendered photoluminescent with a…
We show that nanocrystals (NCs) with well-established synthetic protocols for high shape and size monodispersity can be used as templates to independently control the NC composition through successive cation exchange reactions. Chemical transformations like cation exchange reactions overcome a limitation in traditiona…
Synthetic meso-substituted porphyrins offer significant attractions compared with naturally occurring beta-substituted porphyrins. The attractions include the rectilinear arrangement of the four meso substituents and potential synthetic amenability from pyrrole and simple acyl reactants, thereby avoiding the cumbersom…
Driven by the depletion of crude oil, the direct oxidation of methane to methanol has been of considerable interest. Promising low-temperature activity of an oxygen-activated zeolite, Cu-ZSM-5, has recently been reported in this selective oxidation and the active site in this reaction correlates with an absorption fea…
We present first-principles calculations of many-electron effects on the optical response of graphene, bilayer graphene, and graphite employing the GW-Bethe Salpeter equation approach. We find that resonant excitons are formed in these two-dimensional semimetals. The resonant excitons give rise to a prominent peak in…
Using first-principles plane-wave calculations, we investigate two-dimensional (2D) honeycomb structure of group-IV elements and their binary compounds as well as the compounds of group III-V elements. Based on structure optimization and phonon-mode calculations, we determine that 22 different honeycomb materials are…
Herein we cover the key concepts in the field of thermoelectric materials research, present the current understanding, and show the latest developments. Current research is aimed at increasing the thermoelectric figure of merit (ZT) by maximizing the power factor and/or minimizing the thermal conductivity. Attempts at…
The structure of LP2179, a member of the PF08866 (DUF1831) family, suggests a novel α+β fold comprising two β-sheets packed against a single helix. A remote structural similarity to two other uncharacterized protein families specific to the Bacillus genus (PF08868 and PF08968), as well as to prokaryotic S-adenosylmeth…
Abstract The sub‐ T m exotherms in polyamide 6 (PA6) have been carefully re‐examined by differential scanning calorimetry and X‐ray diffraction, considering the effects of processing and thermal history, addition of water and clay. The results obtained cast doubt on Khanna's proposal that sub‐ T m exotherm in PA6 come…
Abstract Stochastic sub‐wavelength structures with lateral sizes of below 100 nm and heights of about 250 nm were produced on polymer surfaces by plasma treatment. From these master samples, an embossing nickel tool was manufactured, which, in turn, was used to replicate the master surface form by hot embossing in pla…
One-dimensional zinc-blende CdTe nanocrystals were successfully synthesized by a green and ambient pressure aqueous solution synthesis at relatively low temperature. The synthesized nanocrystallites were characterized by X-ray diffraction (XRD), transmission electron microscopy (TEM), high-resolution TEM (HRTEM), and…