Materials Literature
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It has been shown in our previous publication (Blawzdziewicz,Cristini,Loewenberg,2003) that high-viscosity drops in two dimensional linear creeping flows with a nonzero vorticity component may have two stable stationary states. One state corresponds to a nearly spherical, compact drop stabilized primarily by rotation,…
Recent advances in the application of semiconductor nanocrystals, or quantumdots, as biochemical sensors are reviewed. Quantum dots have unique optical properties thatmake them promising alternatives to traditional dyes in many luminescence basedbioanalytical techniques. An overview of the more relevant progresses in…
Abstract The electrochemical polymerization of aqueous solution of aniline and HCl was carried out in a single compartment electrochemical cell. After 2 h of the polymerization reaction, polarity of the electrodes was reversed and kept for 1 h. By this process the conductivity of the polyaniline (PAni) formed was foun…
The ferroelectricity of the spiral magnets LiCu2O2 and LiCuVO4 was examined by calculating the electric polarizations of their spin spiral states on the basis of density-functional theory with spin-orbit coupling. Our work unambiguously reveals that spin-orbit coupling is responsible for the ferroelectricity with the…
Ceramic anodes for solid oxide fuel cells (SOFCs) were prepared by aqueous impregnation of nitrate salts to produce composites with (LSCM) in a 65% porous yttria-stabilized zirconia (YSZ) scaffold. Scanning electron micrographs indicate that the LSCM coats the YSZ pores following calcination at . Composites produced i…
We propose a model of carrier-mediated ferromagnetism in semiconductors that accounts for the temperature dependence of the carriers. The model permits analysis of the thermodynamic stability of competing magnetic states, opening the door to the construction of magnetic phase diagrams. As an example, we analyze the st…
The purpose of this paper is to review some elasticity effects in epitaxial growth. We start by a description of the main ingredients needed to describe elasticity effects (elastic interactions, surface stress, bulk and surface elasticity, thermodynamics of stressed solids). Then we describe how bulk and surface elast…
Magnetoelectric (ME) coupling of a cylindrical trilayered composite was studied in this paper. A Ni–lead zirconate titanate (PZT)-Ni trilayered cylindrical composite was synthesized by electro-deposition. The maximum ME voltage coefficient of the cylindrical ME composite is 35 V cm −1 Oe −1 , about three times higher…
Using a combined ultra-small-angle and small-angle scattering (CSAS) method of neutrons and X-rays, we investigated hierarchical structures of carbon black (CB) highly loaded in polyisoprene (PI) and poly(styrene- random -butadiene) copolymer (SBR) under mechanical field (defined respectively as CB/PI and CB/SBR) as w…
Time-correlated single photon counting methods are used with confocal microscopy and maximum likelihood estimation analysis to obtain fluorescence lifetime trajectories for single quantum dots with KHz update rates. This technique reveals that control of the solution environment can influence both radiative (k(rad)) a…
We determine the equation of state of stoichiometric FeO employing the diffusion Monte Carlo method. The fermionic nodes are fixed to those of a wave function having the form of a single Slater determinant. The calculated ambient pressure properties (lattice constant, bulk modulus and cohesive energy) agree very well…
This paper summarizes the current state of charge flipping, a recently developed algorithm of ab initio structure determination. Its operation is based on the perturbation of large plateaus of low electron density but not directly on atomicity. Such a working principle radically differs from that of classical direct m…
We study the dynamics of vortex-antivortex (VA) pairs in an infinitely thin ferromagnetic film with easy-plane anisotropy. These are localized excitations with finite energy that are characterized by a topological (skyrmion) number N = 0,+1,-1. Topologically trivial (N=0) VA pairs undergo Kelvin motion analogous to th…
In addition to mechanisms already proposed to account for the formation in manganites of a small-polaron superlattice above the Curie temperature Tc and to a metallic-like sea of large polarons below Tc, we now consider other observed colossal-resistance inducing fields, such as magnetic, electric, photon, or strain f…
The electronic structure and properties of PuO$_{2}$ and Pu$_{2}$O$_{3}$ have been studied from first principles by the all-electron projector-augmented-wave (PAW) method. The local density approximation (LDA)+$U$ and the generalized gradient approximation (GGA)+$U$ formalism have been used to account for the strong o…
The thermal conductivity of silicon nanowires (SiNWs) is investigated by molecular dynamics (MD) simulation. It is found that the thermal conductivity of SiNWs can be reduced exponentially by isotopic defects at room temperature. The thermal conductivity reaches the minimum, which is about 27% of that of pure 28Si NW,…
Advances made over the past decade in structure determination from powder diffraction data are reviewed with particular emphasis on algorithmic developments and the successes and limitations of the technique. While global optimization methods have been successful in the solution of molecular crystal structures, new me…
The oxidation of methane in an atmospheric-pressure flow reactor has been studied experimentally under highly diluted conditions in N 2 and CO 2, respectively. The stoichiometry was varied from fuel-lean to fuel-rich, and the temperatures covered the range 1200–1800 K. The results were interpreted in terms of a detail…
Structural rearrangements are an essential property of atomic and molecular glasses; they are critical in controlling resistance to flow and are central to the evolution of many properties of glasses, such as their heat capacity and dielectric constant. Despite their importance, these rearrangements cannot directly be…
Protein molecules have the ability to form a rich variety of natural and artificial structures and materials. We show that amyloid fibrils, ordered supramolecular nanostructures that are self-assembled from a wide range of polypeptide molecules, have rigidities varying over four orders of magnitude, and constitute a c…