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Digitization of Endocytic pH by Hybrid Ultra‐pH‐Sensitive Nanoprobes at Single‐Organelle Resolution

Yiguang Wang、Chensu Wang、Yang Li 等 10 位作者2016-11-04Advanced Materials

A multispectral hybrid nanotransistor consisting of modular fluorescent block copolymers with discrete and sharp pH transitions in one nanoparticluate system is presented. This nanotransistor probe allows digitized reporting of dynamic maturation at single-organelle resolution over time. This nanotechnology platform o…

Supramolecular Self-Assembly in MaterialsAdvanced biosensing and bioanalysis techniquesLipid Membrane Structure and Behavior

Gold aggregating gold: A novel nanoparticle biosensor approach for the direct quantification of hepatitis C virus RNA in clinical samples

Sherif M. Shawky、Ahmed Awad、Walaa R. Allam 等 5 位作者2016-11-04Biosensors and Bioelectronics

The affordable and reliable detection of Hepatitis C Virus (HCV) RNA is a cornerstone in the management and control of infection, affecting approximately 3% of the global population. However, the existing technologies are expensive, labor intensive and time consuming, posing significant limitations to their wide-scale…

Advanced biosensing and bioanalysis techniquesGold and Silver Nanoparticles Synthesis and ApplicationsNanocluster Synthesis and Applications

Adhesion mechanisms of curli subunit CsgA to abiotic surfaces

Elizabeth P. DeBenedictis、Jenny Liu、Sinan Keten2016-11-04Science Advances

Curli fibers are functional amyloids that play a key role in biofilm structure and adhesion to various surfaces. Strong bioinspired adhesives comprising curli fibers have recently been created; however, the mechanisms curli uses to attach onto abiotic surfaces are still uncharacterized. Toward a materials-by-design ap…

Biocrusts and Microbial EcologySilk-based biomaterials and applicationsDiatoms and Algae Research

Understanding the Antifungal Mechanism of Ag@ZnO Core-shell Nanocomposites against Candida krusei

Bhaskar Das、Md Imran Khan、R. Jayabalan 等 7 位作者2016-11-04Scientific Reports

In the present paper, facile synthesis of Ag@ZnO core-shell nanocomposites is reported where zinc oxide is coated on biogenic silver nanoparticles synthesized using Andrographis paniculata and Aloe vera leaf extract. Structural features of as synthesized nanocomposites are characterized by UV-visible spectroscopy, XRD…

Nanoparticles: synthesis and applicationsGraphene and Nanomaterials Applications

Preparation and properties of natural rubber reinforced with polydopamine-coating modified carbon nanotubes

Y-L. Lu、Junpeng Ma、T-Y. Xu 等 6 位作者2016-11-04eXPRESS Polymer Letters

Multi-walled carbon nanotubes (MWCNTs) were functionalized by polydopamine (PDA)-coating and mixed with natural rubber (NR) via latex compounding. Compared with pristine MWCNTs, the surface of MWCNT-PDA was covered by an amorphous and nanometer-scale PDA layer which had a large amount of oxygenic and nitric functional…

Polymer Nanocomposite Synthesis and IrradiationPolymer Nanocomposites and PropertiesCarbon Nanotubes in Composites

Prediction of interface structures and energies via virtual screening

Shin Kiyohara、Hiromi Oda、Tomohiro Miyata 等 4 位作者2016-11-04Science Advances

Interfaces markedly affect the properties of materials because of differences in their atomic configurations. Determining the atomic structure of the interface is therefore one of the most significant tasks in materials research. However, determining the interface structure usually requires extensive computation. If t…

Metal and Thin Film MechanicsMachine Learning in Materials ScienceMicrostructure and mechanical properties

Synthesis and characterization of new functionalized polymer-Fe3O4 nanocomposite particles

Agnieszka Bukowska、Wiktor Bukowski、Krzysztof Hus 等 5 位作者2016-11-04eXPRESS Polymer Letters

In this study, Fe 3 O 4 nanoparticles (NPs) were functionalized with copolymer or terpolymer bearing glycidyl methacrylate (GMA) moieties making them suitable for potential applications as drug delivery systems (DDS). For this purpose, the surface of magnetic nanoparticles was first coated with 3-(trimethoxysilyl) pro…

Iron oxide chemistry and applicationsNanoparticle-Based Drug DeliveryCharacterization and Applications of Magnetic Nanoparticles

Interplay of orbital effects and nanoscale strain in topological crystalline insulators

Daniel Walkup、Badih Assaf、Kane L Scipioni 等 9 位作者2016-11-04arXiv

Orbital degrees of freedom can have pronounced effects on the fundamental properties of electrons in solids. In addition to influencing bandwidths, gaps, correlation strength and dispersion, orbital effects have also been implicated in generating novel electronic and structural phases, such as Jahn-Teller effect and c…

Mesoscale and Nanoscale PhysicsMaterials Science

Proximity effects in cold atom artificial graphene

Tobias Grass、Ravindra W. Chhajlany、Leticia Tarruell 等 5 位作者2016-11-04arXiv

Cold atoms in an optical lattice with brick-wall geometry have been used to mimic graphene, a two-dimensional material with characteristic Dirac excitations. Here we propose to bring such artificial graphene into the proximity of a second atomic layer with a square lattice geometry. For non-interacting fermions, we fi…

quant-phcond-mat.quant-gasStrongly Correlated ElectronsMaterials Sciencephysics.atom-ph

The flow and evolution of ice-sucrose crystal mushes

Andrew Gilbert、Felix Oppong、Robert Farr2016-11-04arXiv

We study the rheology of suspensions of ice crystals at moderate to high volume fractions in a sucrose solution in which they are partially soluble; a model system for a wide class of crystal mushes or slurries. Under step changes in shear rate, the viscosity changes to a new `relaxed' value over several minutes, in a…

Materials ScienceSoft Condensed Matter

Critical enhancement of thermopower in a chemically tuned polar semimetal MoTe 2

H. Sakai、Koji Ikeura、M. S. Bahramy 等 8 位作者2016-11-04Science Advances

with a chemically tunable polar transition. It is unveiled from the first-principles calculations and magnetotransport measurements that charge transport with a strongly energy-dependent scattering rate critically evolves toward the boundary to the nonpolar phase, resulting in large cryogenic thermopower. Such a signi…

Advanced Thermoelectric Materials and Devices2D Materials and ApplicationsMXene and MAX Phase Materials

Mode-decomposition based on crystallographic symmetry in the band-unfolding method

Yuji Ikeda、Abel Carreras、Atsuto Seko 等 5 位作者2016-11-04arXiv

The band-unfolding method is widely used to calculate the effective band structures of a disordered system from its supercell model. The unfolded band structures show the crystallographic symmetry of the underlying structure, where the difference of chemical components and the local atomic relaxation are ignored. It h…

Materials Science

Stability of rhombohedral phases in vanadium at high-pressure and high-temperature: first-principles investigations

Yi X. Wang、Q. Wu、Xiang R. Chen 等 4 位作者2016-11-04arXiv

The pressure-induced transition of vanadium from BCC to rhombohedral structures is unique and intriguing among transition metals. In this work, the stability of these phases is revisited by using density functional theory. At finite temperatures, a novel transition of rhombohedral phases back to BCC phase induced by t…

Strongly Correlated ElectronsMaterials Sciencephysics.comp-ph

Hourglass Fermion Surface States in Stacked Topological Insulators with Nonsymmorphic Symmetry

Motohiko Ezawa2016-11-04arXiv

Recently a nonsymmorphic topological insulator was predicted, where the characteristic feature is the emergence of a "hourglass fermion" surface state protected by the nonsymmorphic symmetry. Such a state has already been observed experimentally. We propose a simple model possessing the hourglass fermion surface state…

Materials ScienceMesoscale and Nanoscale Physics

New insights on the formation of supersaturated solid solutions in the Cu Cr system deformed by high pressure torsion

Andrea Bachmaier、Georg Benedikt Rathmayr、Daniel Apel 等 6 位作者2016-11-04arXiv

In the Cu Cr system, the formation of supersaturated solid solutions can be obtained by severe plastic deformation. Energy dispersive synchrotron diffraction measurements on as deformed Cu Cr samples as a function of the applied strain during deformation confirm the formation of supersaturated solid solutions in this…

Materials Science

Phase separation of a supersaturated nanocrystalline Cu Co alloy and its influence on thermal stability

Andrea Bachmaier、Marina Pfaff、Moritz Stolpe 等 5 位作者2016-11-04arXiv

The thermal decomposition behavior, the microstructural evolution and its influence on the mechanical properties of a supersaturated Cu Co solid solution with ~100 nm average grain size prepared by severe plastic deformation is investigated under non-isothermal and isothermal annealing conditions. Pure fine grained Cu…

Materials Science

Molecular dynamics simulation of twin boundary effect on deformation of Cu nanopillars

G. Sainath、B. K. Choudhary2016-11-04arXiv

Molecular dynamics simulations performed on <110> Cu nanopillars revealed significant difference in deformation behavior of nanopillars with and without twin boundary. The plastic deformation in single crystal Cu nanopillar without twin boundary was dominated by twinning, whereas the introduction of twin boundary chan…

Materials Science