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Crystal structure and magnetic properties of K5.5Na1.5[PW10Cu2(H2O)2O38].13H2O. Substituted Keggin heteropolytungstates of the type PW10Cu2 containing exchange-coupled copper pairs

Carlos J. Gómez‐García、Eugenio Coronado、Pedro Gómez‐Romero 等 4 位作者1993-01-01Inorganic Chemistry

We report the structural and magnetic characterization of the crystalline product obtained from a solution containing Δ-(PW9O34)9- and Cu2+ ions (molar ratio 1/2) after standing a long period of time at room temperature. Three complementary techniques were used: X-ray diffraction, magnetic susceptibility measurements,…

Metal-Organic Frameworks: Synthesis and ApplicationsPolyoxometalates: Synthesis and ApplicationsNanocluster Synthesis and Applications

Transformation Textures in Zirconia

Keith J. Bowman、I‐Wei Chen1993-01-01Journal of the American Ceramic Society

The large shear component of the tetragonal‐to‐monoclinic transformation in zirconia causes a stress‐induced preferred orientation of the tetragonal and monoclinic variants. The resultant texture, which is dependent on the loading condition, has been analyzed in terms of stress assistance to transformation and experim…

Advanced ceramic materials synthesisMicrostructure and mechanical propertiesAdvanced materials and composites

Investigation of the surface activity of corrosion inhibitors by XPS and time‐of‐flight SIMS

Andrew J. Swift、Alan J. Paul、John C. Vickerman1993-01-01Surface and Interface Analysis

Abstract X‐ray photoelectron spectroscopy (XPS), time‐of‐flight secondary ion mass spectrometry (ToF‐SIMS) and infrared spectroscopy (IR) have been used to study the interaction of two corrosion inhibitor blends of unknown composition with an iron surface. The analysis has precisely identified quaternary ammonium and…

Corrosion Behavior and InhibitionElectron and X-Ray Spectroscopy TechniquesIon-surface interactions and analysis

Laser manipulation and assembling of polymer latex particles in solution

Hiroaki Misawa、Keiji Sasaki、Masanori Koshioka 等 5 位作者1993-01-01Macromolecules

ADVERTISEMENT RETURN TO ISSUEPREVArticleNEXTLaser manipulation and assembling of polymer latex particles in solutionHiroaki Misawa, Keiji Sasaki, Masanori Koshioka, Noboru Kitamura, and Hiroshi MasuharaCite this: Macromolecules 1993, 26, 2, 282–286Publication Date (Print):January 1, 1993Publication History Published o…

Diatoms and Algae Research

Phase states: an analytic approach in the unit disc

A. Vourdas1993-01-01Physica Scripta

Phase states are defined as eigenkets of the "exponential of the phase" operator E − . It is shown that they are SU(1, 1) Perelomov coherent states corresponding to the k = ½ representation. The properties of these states are discussed and used for the calculation of the phase distribution of coherent, squeezed and ph…

Quantum optics and atomic interactionsSolid-state spectroscopy and crystallographyOptical and Acousto-Optic Technologies

Relationship between segmental and chain dynamics in polymer melts as studied by dielectric spectroscopy

Andreas Schönhals、E. Schlosser1993-01-01Physica Scripta

Broadband dielectric spectroscopy in the frequency range from 10 −5 Hz to 10 6 Hz is employed to study the relation between α-relaxation and normal mode process for oligomeric polyisoprene and polypropylene glycol samples of different molecular weight. It is shown that relaxation time of the α-relaxation has a much st…

Polymer crystallization and propertiesMaterial Dynamics and PropertiesRheology and Fluid Dynamics Studies

The Development of Bearing Steels for Long Life Rolling Bearings Under Clean Lubrication and Contaminated Lubrication

K Furumura、Yasuo Murakami、T Abe1993-01-01OpenAlex

Nearly ten years have passed since the LF-RH-CC process was adopted in the production of bearing steels. This process has become a common system for steelmakers, regardless of using EFs or BOFs as melting furnaces. The current cleanliness level of bearing steels shows a remarkable improvement when compared to that of…

Gear and Bearing Dynamics AnalysisTribology and Lubrication EngineeringMetal Alloys Wear and Properties

Synthesis and crystal and molecular structure of (Et 4 N) 2 [Mn 10 O 2 Cl 8 {(OCH 2 ) 3 CMe} 6 ]·4MeOH·2H 2 O, a Mn II,III mixed-valence cluster with the decametallate core geometry

Michael Cavaluzzo、Qin Chen、Jon Zubieta1993-01-01Journal of the Chemical Society Chemical Communications

The reaction of (Et4N)2MnCl4 with MeC(CH2OH)3 in acetonitrile in the presence of atmospheric oxygen yields the oxoalkoxomanganese cluster (Et4N)2[Mn10O2Cl8{(OCH2)3CMe}6]·4MeOH·2H2O, a MnII,III mixed valence species exhibiting the decametallate core geometry, {M10O2L26}.

Metal-Organic Frameworks: Synthesis and ApplicationsMagnetism in coordination complexesPolyoxometalates: Synthesis and Applications

Measurement of Fabric Roughness by a Non- contact Method

R. B. Ramgulam、J. Amirbayat、I. Porat1993-01-01Journal of the Textile Institute

The paper describes the method of using a laser sensor for the measurement of surface roughness and compares the results with those obtained by conventional contact methods. It goes further to study the anisotropy of roughness in ten plain woven fabrics.

Textile materials and evaluationsIndustrial Vision Systems and Defect DetectionSurface Roughness and Optical Measurements

Control of nucleation in the crystallization of lysozyme

Naomi E. Chayen、Jonathan Radcliffe、D. M. Blow1993-01-01Protein Science

This work investigates the influence of storage of lysozyme in solution on its crystallization. The crystallization of hen egg-white lysozyme exhibits a storage effect (aging) that depends on the length of time the lysozyme solution is stored, after dissolving from freeze-dried powder, before being brought to crystall…

Proteins in Food SystemsEnzyme Structure and FunctionCrystallization and Solubility Studies

Ionic dynamics in the rotator phase of n-alkylammonium chlorides (C 6 –C 10 ), studied by 1 H nuclear magnetic resonance, electrical conductivity and thermal measurements

Shigehiko Iwai、Mineyuki Hattori、Daiyû Nakamura 等 4 位作者1993-01-01Journal of the Chemical Society Faraday Transactions

1 H NMR, electrical conductivity and thermal measurements have been performed on the rotator phase of n-alkylammonium chlorides CnH2n+1 NH3Cl (n= 6–10). Rapid two-dimensional self-diffusion and uniaxial rotation of the long rod-like cations were observed in all salts studied by measuring 1H NMR spin–lattice relaxation…

Liquid Crystal Research AdvancementsMaterial Dynamics and PropertiesSolid-state spectroscopy and crystallography

Effect of reactive additives on the performance of cellulose fiber-filled polypropylene composites

Mohini Sain、B. V. Kokta、D. Maldas1993-01-01Journal of Adhesion Science and Technology

The role of boron compounds on the flame retardance characteristics of unmodified as well as surface-modified wood fiber-filled polypropylene composites is discussed. The effect of three different additives, m-phenylene bismaleimide (BMI), BMI-modified polypropylene (BPP), and a mixture of borax and boric acid, on the…

Polymer Nanocomposites and PropertiesNatural Fiber Reinforced CompositesFlame retardant materials and properties

Grafted polymer layers with chain exchange: A Monte Carlo simulation

Pik‐Yin Lai1993-01-01The Journal of Chemical Physics

By introducing a head-group energy of adsorption with the grafting surface, we simulate the grafted polymer layer including chain exchange with the bulk solution using the bond-fluctuation model. The kinetics of adsorption is relatively rapid in short times and becomes much slower in later time as the layer is formed.…

Surface Modification and SuperhydrophobicityPolymer Surface Interaction StudiesMolecular Junctions and Nanostructures

Effect of impurities on cluster growth and nucleation

Rajiv M. Ginde、Allan S. Myerson1993-01-01Journal of Crystal Growth

Previous measurements of concentration gradients formed in long columns of supersaturated glycine solutions [1] indicate that small amounts of impurities, such as valine, can lead to an increase in the magnitude of the gradient. This might indicate that the impurity enhances the degree of cluster formation. The concen…

Spectroscopy and Quantum Chemical StudiesCrystallization and Solubility Studiesnanoparticles nucleation surface interactions

Preparation of alumina-pillared acid-activated clays and their use as chlorophyll adsorbents

Robert Mokaya、William Jones、Mary E. Davies 等 4 位作者1993-01-01Journal of Materials Chemistry

Acid-activated clays (montmorillonites) have been cation-exchanged with aluminium chloride pentahydroxide dihydrate (aluminium chlorhydrate, ACH) solutions of different concentrations to yield expanded materials. Various Al:clay (a/c) ratios have been used. The effect of changing the degree of polymerisation of the pi…

Mesoporous Materials and CatalysisClay minerals and soil interactionsLayered Double Hydroxides Synthesis and Applications

Novel differential scanning calorimetric studies of supercooled organic liquids

S. Srinivasa Murthy、Gangasharan、Santanu Kumar Nayak1993-01-01Journal of the Chemical Society Faraday Transactions

The glass-forming tendency of a large number of organic liquids of varying molecular shapes has been examined using differential scanning calorimetry (DSC) and a sharp distinction between spherical and non-spherical molecular liquids as regards their glass-forming efficiency is observed. Calorimetric evidence has been…

Material Dynamics and PropertiesGlass properties and applicationsPhase-change materials and chalcogenides

Structure and electronic transport properties of the Misfit layer compound (LaSe)1.14(NbSe2)2, „LaNb2Se5”

R. Roesky、A. Meerschaut、J. Rouxel 等 4 位作者1993-01-01Zeitschrift für anorganische und allgemeine Chemie

Abstract The new misfit layer compound (LaSe) 1.14 (NbSe 2 ) 2 has been synthesized from the elements at 1050‐ and its structure has been determined by a composite approach. The structure has an alternating stacking sequence of [LaSe] and two [NbSe 2 ] layers along the c direction. The misfit of the two different laye…

Rare-earth and actinide compoundsIron-based superconductors researchInorganic Chemistry and Materials

Diffuse reflectance Fourier-transform infrared study of the plasma-fluorination of diamond surfaces using a microwave discharge in CF4

Toshihiro Ando、Junzo Tanaka、Motohiko Ishii 等 7 位作者1993-01-01Journal of the Chemical Society Faraday Transactions

Species chemisorbed on diamond surfaces, which had been treated under CF4-plasma conditions, have been investigated by diffuse reflectance Fourier-transform infrared spectroscopy. Both oxidized and hydrogenated diamond surfaces were fluorinated at temperatures in the range 300–1000 °C. The C—F bond was observed on the…

Metal and Thin Film MechanicsDiamond and Carbon-based Materials ResearchPlasma Diagnostics and Applications

Surface models for γ-Al 2 O 3 from molecular dynamics simulations

Luis Javier Álvarez、Javier Fdez. Sanz、M. J. Capitán 等 5 位作者1993-01-01Journal of the Chemical Society Faraday Transactions

Molecular dynamics simulations for γ-Al2O3 and La3+-doped γ-Al2O3 crystals have been performed. From bulk simulations a description of the crystal-terminating layers in both doped and pure alumina solids is reported. The molecular dynamics simulations allow us to describe systematically for the first time the surface…

Advanced ceramic materials synthesisGlass properties and applicationsX-ray Diffraction in Crystallography

X-ray diffraction, high-resolution transmission electron microscopy and Fourier-transform infrared study of Ca-doped Al2O3

C. Morterra、Giuliana Magnacca、G. Cerrato 等 6 位作者1993-01-01Journal of the Chemical Society Faraday Transactions

Three alumina preparations, doped with ca. 3% CaO and corresponding to the γ-, δ,θ- and α-Al2O3 phases, respectively, have been studied by XRD, TEM and FTIR spectroscopy. Owing to the presence of Ca, no bulk phase stabilization/destabilization effects were observed, but the particle morphology of the γ- and α-phases w…

Advanced ceramic materials synthesisMicrowave Dielectric Ceramics SynthesisMagnesium Oxide Properties and Applications