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Synthesis of NiGa Layered Double Hydroxides. A Combined Extended X-ray Absorption Fine Structure, Small-Angle X-ray Scattering, and Transmission Electron Microscopy Study. 1. Hydrolysis in the Pure Ni2+ System

Guillaume Defontaine、Laurent J. Michot、Isabelle Bihannic 等 5 位作者2003-11-08Langmuir

Takovites are nickel-based layered double hydroxides (LDHs) with a general formula that can be written as Ni 1 - x Al x (OH) 2, A z - x / z, y H 2 O, where A is a compensating interlayer anion. As in some other LDH samples, the positive charge of the layer can be adjusted upon synthesis and various anions can be excha…

Supercapacitor Materials and FabricationLayered Double Hydroxides Synthesis and ApplicationsInorganic Chemistry and Materials

Molecular Tectonics. Dendritic Construction of Porous Hydrogen-Bonded Networks

D. Laliberté、Thierry Maris、Ariane Sirois 等 4 位作者2003-11-08Organic Letters

Molecules that associate to form porous networks can be made by attaching multiple hydrogen-bonding sites to suitable cores. Pentaerythrityl tetraphenyl ether, a four-armed core, is the progenitor of dendritic derivatives with more arms, including dipentaerythrityl hexaphenyl ether 7. An advantage of such dendritic de…

Advanced Polymer Synthesis and CharacterizationLuminescence and Fluorescent MaterialsDendrimers and Hyperbranched Polymers

Formation and Optical Properties of Cylindrical Gold Nanoshells on Silica and Titania Nanorods

Steven J. Limmer、Tammy P. Chou、Guozhong Cao2003-11-08The Journal of Physical Chemistry B

Metal−insulator core−shell structures have been demonstrated to have interesting and tunable optical properties. Systems previously investigated include silica-capped gold particles and gold shells surrounding silica particles. However, many of the systems studied so far have been spherical (or zero-dimensional). Thus…

Gold and Silver Nanoparticles Synthesis and ApplicationsQuantum Dots Synthesis And PropertiesNanocluster Synthesis and Applications

A ferroelectric barium titanate, BaTi2O5

Teiichi Kimura、Takashi Goto、Hisanori Yamane 等 6 位作者2003-11-08Acta Crystallographica Section C Crystal Structure Communications

The crystal structure of monobarium dititanium pentaoxide, BaTi(2)O(5), synthesized by a floating-zone method, was studied by X-ray diffraction. Previous reports describe the structure as being in the monoclinic centrosymmetric space group C2/m. We have recently found that this material exhibits ferroelectricity, and…

Ferroelectric and Piezoelectric MaterialsGlass properties and applicationsSolid-state spectroscopy and crystallography

Nanocrystalline Mesoporous Tin Dioxide Prepared by the Sol−Gel Route from a Dialkoxydi(β-Diketonato)tin Complex

Thierry Toupance、Odile Babot、B. Jousseaume 等 4 位作者2003-11-08Chemistry of Materials

Nanocrystalline mesoporous tin dioxide materials have been obtained through the controlled hydrolysis of bis(2-methylbutan-2-oxy)di(pentan-2,4-dionato)tin followed by a thermal treatment at 400−550 °C. These materials have been carefully characterized by elemental analysis, FTIR, TGA-MS, XRD, MET, N 2 adsorption, and…

Mesoporous Materials and CatalysisPorphyrin and Phthalocyanine ChemistryTransition Metal Oxide Nanomaterials

Correlation between Magnetic Properties and Mn/Co Atomic Order in LaMn0.5Co0.5O3+δ: I. Second-Order Nature in Mn/Co Atomic Ordering and Valence State

Tôru Kyômen、Ryutaro Yamazaki、Mitsuru Itoh2003-11-08Chemistry of Materials

The relaxation phenomenon around 1300 K in LaMn 0.5 Co 0.5 O 3+ δ and their valence states of Mn and Co atoms were investigated by TG-DTA, powder X-ray diffraction, magnetic susceptibility, and XANES of two samples cooled at 10 Kh - 1 in the range 1673−973 K and quenched from 1673 K. DTA clarified that the relaxation…

Magnetic and transport properties of perovskites and related materialsAdvanced Condensed Matter PhysicsElectronic and Structural Properties of Oxides

Synthesis and Self-Assembly of Supramolecular Dendritic “Bow-Ties”: Effect of Peripheral Functionality on Association Constants

Elizabeth R. Gillies、Jean M. J. Fréchet2003-11-08The Journal of Organic Chemistry

Self-assembled polyester dendritic bow-ties with various peripheral groups were prepared, and their association constants were measured by (1)H NMR in CDCl(3). The two complementary dendrons were prepared by attachment of either a bis(adamantylurea) or a glycinylurea to the focal point of the dendron. The parent self-…

Advanced Polymer Synthesis and CharacterizationDendrimers and Hyperbranched PolymersSynthesis and properties of polymers

The 5-V Window of Polarizability of Fluorinated Diamond Electrodes in Aqueous Solutions

Sergio Ferro、Achille De Battisti2003-11-08Analytical Chemistry

Heavily doped diamond films are quite actively studied for their promising applications in industrial as well as in fundamental electrochemistry (both for physicochemical studies and in the field of electroanalysis), because of their very high stability toward chemical and electrochemical oxidative attacks. Fluorinate…

Diamond and Carbon-based Materials ResearchMolecular Junctions and NanostructuresAnalytical Chemistry and Sensors

Synthesis and Characterization of Phenylphosphine Oxide Containing Perfluorocyclobutyl Aromatic Ether Polymers for Potential Space Applications

Jianyong Jin、Dennis W. Smith、Chris M. Topping 等 9 位作者2003-11-08Macromolecules

A novel class of phenylphosphine oxide (PPO) containing perfluorocyclobutyl (PFCB) polymers has been developed for potential use as multifunctional materials in space environments. The reaction of p -BrArOCF CF 2 (for Ar = phenyl and biphenyl) with tert -butyllithium affords the lithium reagent smoothly below −20 °C.…

Synthesis and characterization of novel inorganic/organometallic compoundsSynthesis and properties of polymersSilicone and Siloxane Chemistry

Ab Initio Computational Crystallography of 2:1 Clay Minerals: 1. Pyrophyllite-1Tc

Keith Refson、Sungho Park、Garrison Sposito2003-11-08The Journal of Physical Chemistry B

The interpretation of diffraction and spectroscopic data on clay minerals can be facilitated by first-principles quantum mechanical simulations based on density functional theory (DFT), which now has achieved sufficient accuracy to predict crystallographic properties of these minerals without recourse to empirical par…

High-pressure geophysics and materialsSoil and Unsaturated FlowClay minerals and soil interactions

Synthesis of Mesoporous Silica from Commercial Poly(ethylene oxide)/Poly(butylene oxide) Copolymers: Toward the Rational Design of Ordered Mesoporous Materials

Chengzhong Yu、Jie Fan、Bozhi Tian 等 5 位作者2003-11-08The Journal of Physical Chemistry B

Five commercial poly(ethylene oxide)/poly(butylene oxide) (PEO/PBO) triblock copolymer surfactants were utilized as structure-directing agents to synthesize mesoporous silica under acidic conditions. The structures of these materials were characterized by using powder X-ray diffraction (XRD), nitrogen adsorption analy…

Zeolite Catalysis and SynthesisMesoporous Materials and CatalysisPolyoxometalates: Synthesis and Applications

Mild, Solvent-Free ω-Hydroxy Acid Polycondensations Catalyzed by Candida antarctica Lipase B

Anil Mahapatro、Ajay Kumar、Richard A. Gross2003-11-08Biomacromolecules

Immobilized Candida antarctica Lipase B (Novozyme-435) was studied for bulk polyesterifications of linear aliphatic hydroxyacids of variable chain length. The products formed were not fractionated by precipitation. The relative reactivity of the hydroxyacids was l6-hydroxyhexadecanoic acid approximately 12-hydroxydode…

Enzyme Catalysis and ImmobilizationAdvanced Polymer Synthesis and Characterizationbiodegradable polymer synthesis and properties

Addition of Carbon Radicals Generated from Organic Peroxides to Single Wall Carbon Nanotubes

Polona Umek、Jin Won Seo、Klára Hernádi 等 7 位作者2003-11-08Chemistry of Materials

Single wall carbon nanotubes (SWNT) were functionalized via addition of carbon radicals, which were generated by thermal decomposition of diacyl and dibenzoyl peroxides. Reaction products were investigated with TEM, Raman scattering, TGA, UV−Visible spectroscopy, FTIR, and 1 H NMR. In Raman spectra of functionalized S…

Carbon Nanotubes in CompositesGraphene research and applicationsFullerene Chemistry and Applications

Ultra-Water-Repellent Poly(ethylene terephthalate) Substrates

Katsuya Teshima、Hiroyuki Sugimura、Yasushi Inoue 等 5 位作者2003-11-08Langmuir

ADVERTISEMENT RETURN TO ISSUEPREVNoteUltra-Water-Repellent Poly(ethylene terephthalate) SubstratesKatsuya Teshima, Hiroyuki Sugimura, Yasushi Inoue, Osamu Takai, and Atsushi TakanoView Author Information Department of Materials Processing Engineering, Graduate School of Engineering, Nagoya University, Nagoya 464-8603,…

Surface Modification and SuperhydrophobicityPolymer crystallization and propertiesFiber-reinforced polymer composites

Switching of Spin States Triggered by a Phase Transition: Spin-Crossover Properties of Self-Assembled Iron(II) Complexes with Alkyl-Tethered Triazole Ligands

Tsuyohiko Fujigaya、Donglin Jiang、Takuzo Aida2003-11-08Journal of the American Chemical Society

Iron(II) complexes of triazole derivatives having two C12 and C16 long alkyl chains, (C12trz)FeII and (C16trz)FeII, serve as novel spin-crossover materials, which display a spin-state transition in response to a phase transition. In contrast, a triazole complex with two C8 alkyl chains ((C8trz)FeII) exhibits only a po…

Magnetism in coordination complexesLanthanide and Transition Metal ComplexesElectron Spin Resonance Studies

Interlayer Interaction of Two-Dimensional Layered Spin Crossover Complexes [FeIIH3LMe][FeIILMe]X (X-= ClO4-, BF4-, PF6-, AsF6-, and SbF6-; H3LMe= Tris[2-(((2-methylimidazol-4-yl)methylidene)amino)ethyl]amine)

Masahiro Yamada、M. Ooidemizu、Yuichi Ikuta 等 9 位作者2003-11-08Inorganic Chemistry

A series of two-dimensional (2D) spin crossover complexes, [FeIIH3L(Me)][FeIIL(Me)]X (X-=ClO4-, BF4-, PF6-, AsF6-, SbF6-) 1-5, have been synthesized, where H3L(Me) denotes an hexadentate N6 tripodlike ligand containing three imidazole groups, tris[2-(((2-methylimidazol-4-yl)methylidene)amino)ethyl]amine. Compounds 1-5…

Magnetism in coordination complexesMetal-Catalyzed Oxygenation MechanismsOrganic and Molecular Conductors Research

Biosynthesis of CaCO3 Crystals of Complex Morphology Using a Fungus and an Actinomycete

Debabrata Rautaray、Absar Ahmad、Murali Sastry2003-11-08Journal of the American Chemical Society

The biosynthesis of CaCO3 by reaction of aqueous Ca2+ ions with a fungus, Fusarium sp., and an actinomycete, Rhodococcus sp. (both plant organisms), is described. In the case of the fungus, cruciform-shaped calcite crystals are obtained (SEM picture A) while the actinomycete yielded the unstable polymorph of CaCO3, va…

Paleontology and Stratigraphy of FossilsCalcium Carbonate Crystallization and InhibitionMarine Sponges and Natural Products

Optimization of Single-Walled Carbon Nanotube Arrays for Methane Storage at Room Temperature

Dapeng Cao、Xianren Zhang、Jian‐Feng Chen 等 5 位作者2003-11-08The Journal of Physical Chemistry B

The adsorption storage of methane on triangular arrays of single-walled carbon nanotubes (SWNT) at room temperature was investigated by the grand canonical Monte Carlo (GCMC) method. In the simulation, carbon atoms on the tubular wall were structured according to the ( m, m ) armchair arrangement, and the site-to-site…

Carbon Nanotubes in CompositesGraphene research and applicationsZeolite Catalysis and Synthesis

Electrochemical Incineration of Organic Pollutants on Boron-Doped Diamond Electrode. Evidence for Direct Electrochemical Oxidation Pathway

Jinfang Zhi、Haibin Wang、T. Nakashima 等 5 位作者2003-11-08The Journal of Physical Chemistry B

The electrochemical incineration of organic pollutants on a boron-doped diamond (BDD) thin film electrode was examined by bulk electrolysis, and the mechanism of oxidation was investigated. A comparative study with other electrodes such as Pt and glassy carbon (GC) electrodes revealed the superiority of the BDD over t…

Advanced Photocatalysis TechniquesAdvanced oxidation water treatmentCovalent Organic Framework Applications

Coumarin-4-ylmethoxycarbonyls as Phototriggers for Alcohols and Phenols

Akinobu Z. Suzuki、Takayoshi Watanabe、Mika Kawamoto 等 8 位作者2003-11-08Organic Letters

Caged compounds can be used to regulate the spatial and temporal dynamics of signaling molecules in live cells. Photochemical properties of coumarin-4-ylmethoxy carbonates (1a-d) are investigated to construct caged compounds of hydroxy-containing molecules. All the compounds possess desired properties as phototriggers…

Radical Photochemical ReactionsPhotochromic and Fluorescence ChemistryFree Radicals and Antioxidants