Materials Literature
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Nucleation and growth mechanisms of short chains of carbon atoms on single-layer, hexagonal boron nitride (h-BN) and short BN chains on graphene are investigated using first-principles plane-wave calculations. Our analysis starts with the adsorption of a single carbon adatom and examines its migrations. Once a C${}_{2…
In the framework of algebraic topology the closed sequence of 4-dimensional polyhedra(algebraic polytopes) was defined. These polytopes were determined by the second coordination sphere of 8-dimensional lattice E8. The ordered non-crystalline structure is determined by a chain of constructions of algebraic topology: a…
Fine-grain graphite targets have been exposed to ITER divertor relevant plasmas in Pilot-PSI to address material migration issues in fusion devices. Optical emission spectroscopy and mass loss measurements have been employed to quantify gross chemical erosion and net erosion yields, respectively. Effects of the ion im…
We present a study of the thickness dependence of magnetism and electrical conductivity in ultrathin La0.67Sr0.33MnO3 films grown on SrTiO3 (110) substrates. We found a critical thickness of 10 unit cells below which the conductivity of the films disappeared and simultaneously the Curie temperature increased, indicati…
A two-dimensional atomic mass spring system is investigated for critical fracture loads and its crack path geometry. We rigorously prove that, in the discrete-to-continuum limit, the minimal energy of a crystal under uniaxial tension leads to a universal cleavage law and energy minimizers are either homogeneous elasti…
Nanoscale CeO₂ is increasingly used for industrial and commercial applications, including catalysis, UV-shielding and as an additive in various nanocomposites. Because of its increasing potential for consumer and occupational exposures, a comprehensive toxicological characterisation of this nanomaterial is needed. Pre…
Counter electrodes from polypyrrole (PPy) and polyaniline (PANi) nanostructures were fabricated by chemical and electrochemical approaches for dye-sensitized solar cell (DSSC) applications. It was found that double-layered PANi consisting of a nanoparticle layer and a nanofiber layer was formed by an electrodeposition…
The influence of poly(tetramethylene oxide) (PTMO) soft segment length on the phase-separated microstructure, state of hydrogen-bonded associations, and molecular dynamics was investigated in polyureas polymerized from the bulk. For higher PTMO molecular weights (1000 and 650 g/mol) hard segments self-assemble into ri…
The biological approach to synthesis of AuNPs is eco-friendly and an ideal method to develop environmentally sustainable nanoparticles alternative to existing methods. We have developed a simple, fast, clean, efficient, low-cost and eco-friendly single-step green chemistry approach for the synthesis of biocompatible g…
Dumbbell-like Pt(48)Pd(52)-Fe(3)O(4) nanoparticles are synthesized and functionalized with oleylamine-polyethyleneglycol to serve as an efficient catalyst for H(2)O(2) reduction and tetramethylbenzidine (TMB) oxidation in biological solutions. The Pt(48)Pd(52)-Fe(3)O(4)/TMB kit is even more active than the natural enz…
Abstract Heteroatom‐doped carbon (HDC) has attracted tremendous attention due to its promising application in energy conversion and storage. Herein, due to its abundance high rate of reproduction, the microorganism, Bacillus subtilis , is selected as a precursor. An effective ionothermal process is adopted to produce…
We herein report the first instance of aqueous-phase photosensitization of semiconductor photocatalysts (WO(3) loaded with Pt) through triplet-triplet annihilation (TTA)-based upconversion of sub-band-gap photons. The TTA-based upconversion (UC) was achieved in the aqueous phase by encapsulating the solvent phase cont…
Developing approaches to effectively induce and control the magnetic states is critical to the use of magnetic nanostructures in quantum information devices but is still challenging. Here we have demonstrated, by employing the density functional theory calculations, the existence of infinite magnetic sheets with struc…
We have recently synthesized atomically flat semiconductor colloidal nanoplatelets with quasi 2D geometry. Here, we show that core/shell nanoplatelets can be obtained with a 2D geometry that is conserved. The epitaxial growth of the shell semiconductor is performed at room temperature. We report the detailed synthesis…
Graphene lite: a density of (2.1 ± 0.3) mg cm(-3), the lowest to date for a graphene framework architecture, is achieved by preparing an ultralight, N-doped, 3D graphene framework (see photo of a block of the material balancing on a dandelion). Its adsorption capacity for oils and organic solvents is much higher than…
Ultrathin metasurfaces consisting of a monolayer of subwavelength plasmonic resonators are capable of generating local abrupt phase changes and can be used for controlling the wavefront of electromagnetic waves. The phase change occurs for transmitted or reflected wave components whose polarization is orthogonal to th…
Supercapacitors have attracted intense attention due to their great potential to meet the demand of both high energy density and power density in many advanced technologies. Various carbon-based nanocomposites are currently pursued as supercapacitor electrodes because of the synergistic effect between carbon (high pow…
Covalent organic frameworks (COFs) represent an exciting new type of porous organic materials, which are ingeniously constructed with organic building units via strong covalent bonds. The well-defined crystalline porous structures together with tailored functionalities have offered the COF materials superior potential…
Abstract A mixture of acrylated castor oil (ACO) with N ‐carbobenzyloxy‐ L ‐isoleucylaminooctadecane (CIA) or ( R )‐12‐hydroxystrearic acid (HSA) containing photo‐initiators was heated to 130°C and gradually cooled to room temperature to give bio‐based gelatinous material. The photo‐curing of the gel generated a cross…
New approaches for optical data storage (ODS) applications are needed to meet the future requirements of applications in multimedia, archiving, security, and many others. Commercial data storage technologies are moving to threedimensional (3D) materials, but the capacity is limited by the fabrication cost and the numb…