Materials Literature
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The recent advances in the syntheses of mesostructured porous silicates (MCM-41 and SBA-15) allow us to study liquids confined in highly regular geometry. Hence, one might get to a better understanding of the structure and the dynamics of confined fluids. In this paper, we address the problem of the interpretation of…
A comparison is made of the dynamics observed over wide ranges of time and temperature between five supercooled liquids and four isotropic phase liquid crystals that have been previously studied separately. Optical-heterodyne-detected optical Kerr effect (OHD–OKE) measurements were employed to obtain the orientational…
Theoretical study based on a first-principles band structure calculation is carried out for new room-temperature ferromagnets, zinc blende CrSb and CrAs. It is found from the total-energy calculation that the ferromagnetic state is energetically favorable for both materials. By using the value of the difference in tot…
Abstract Two routes have been developed inorder to prepare an inclusion complex of polyaniline (PANI) and β‐cyclodextrin (βCyD). The first route was to in situ polymerize N ‐phenyl‐1,4‐phenylenediamine (PPD) which was encapsulated in βCyD in advance. The formation of an inclusion complex was confirmed by UV‐vis, circu…
The paper proposes the use of a Lorentzian function to describe the irreversible component of the magnetization of soft materials with hysteresis using the Everett’s integral. We will derive an analytical formula to compute the irreversible magnetization, and compute the reversible component by the measurements of the…
Mechanical alloying of Mn-Al and Mn-Al-C powder mixtures resulted in the formation of α-Mn solid solution. Heat treatment of these mechanically alloyed powders resulted in the formation of the metastable τ phase. The mechanically alloyed powders annealed at relatively low temperatures (500–700 °C) showed small saturat…
The magnetic properties of laminated electrical steels are degraded by punching because of plasticity localized along the cutting edge, but also because of residual stresses, which may spread over the whole lamination. In this article, long-range residual stresses are analyzed via a simplified mechanical analysis. The…
Hexagonal manganites REMnO3 consist of layers of two-dimensional connected distorted MnO5 bipyramids separated by distorted layers of RE, leading to frustrated Mn3+–O2−–Mn3+ in-plane exchange paths (superexchange) and Mn3+–O2−–O2−–Mn3+ interplane exchange paths (super-superexchange). We report single-crystal diffracti…
A model has been developed that describes the interrelating effects of plastic deformation and applied stress on hysteresis loops based on the theory of ferromagnetic hysteresis. In the current model the strength of pinning sites for domain walls is characterized by the pinning coefficient keff given by keff=k0+k′σ. T…
We have studied the magnetic moments and magnetic anisotropy energy (MAE) of YCo5 and SmCo5 using full-potential linear augmented plane wave (LAPW) electronic structure calculations. Most previous calculations of the MAE for YCo5, using local density approximation (LDA) for the exchange-correlation potential, have fou…
The dynamic magnetomechanical properties of a Terfenol-D/epoxy 1–3 magnetostrictive particulate composite fabricated using 49% volume fraction of needle-shaped, [112]-oriented Terfenol-D particles were investigated as a function of magnetic bias field (HBias). A nonoriented composite with 51% volume fraction of irregu…
Stress is one of the principal external factors affecting the magnetization of materials. The magnetomechanical effect, that is, the change of magnetization of a magnetic material resulting from the application of stress, has attracted attention because of its scientific complexity. An improved model equation for inte…
Colossal magnetoresistance (CMR) composite materials have been synthesized to explore the possibility of improving magneto-transport and structural properties in CMR systems. In this work we describe (La1−xCaxMnO3)1−y (LCMO) (ZrO2)y (x≈0.3 and 0.0⩽y⩽0.40 mole %) composites that have been synthesized using a modified (…
Cu-alloy films are being explored for integrated circuits, for creating low-resistivity interconnects with stabilized metal/dielectric interfaces via solute segregation, and for interfacial reactions. Here, we describe the pathways of microstructure evolution in supersaturated Cu– 5–12 at. % Mg films, and phase format…
We report on the electronic, transport, and magnetic properties of the Ce-doped manganite, La1−xCexMnO3. This material is remarkably similar to the heavily investigated hole doped manganite La1−xCaxMnO3; e.g., both materials show Curie temperatures of TC∼250 K for x=0.3. The main difference which makes the Ce-doped ma…
In this article we report a chemical synthetic means for generating a high Ku magnetic material—narrowly dispersed nanoparticles of SmCo5. Using Co2(CO)8 and Sm(acac)3 as the precursors under air-free conditions, we produced SmCo5 nanoparticles according to the procedure reported by Sun et al. [Science 287, 1981 (2000…
The magnetic and magnetotransport properties of nanoparticulate magnetite with different grain sizes are investigated using x-ray diffraction, microscopy, magnetometry, and magnetoresistance measurements. The magnetization varies significantly with grain size and is sensitive to preparation conditions. The reduction i…
The evolution of the microstructure, microchemistry, and magnetic properties during slow cooling of melt-spun Sm(Co,Fe,Cu,Zr)z magnets was investigated. It was found that uniform cellular and lamellar structures are formed upon isothermal aging the as-spun ribbons at 850 °C for 3 h, without subsequent slow cooling. No…
Fe 3 O 4 thin films have been directly sputter deposited from a target consisting of a mixture of Fe3O4 and Fe2O3 onto Si and glass substrates. The magnetic properties and microstructures of the films have been characterized and correlated. The columnar growth of the Fe3O4 grains was found to be initialized from the s…
We investigate and discuss the interaction of a hydrogen atom (H) with graphene based on the density functional theory (DFT). Our calculation results show that reconstructions of carbon atoms play an important role in the H adsorption on graphene. When constituent carbon atoms are held rigid, endothermic H adsorption…