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Coupled Electron‐Proton Transport in Electropolymerized Methylene Blue and the Influences of Its Protonation Level on the Rate of Electron Exchange with β‐Nicotinamide Adenine Dinucleotide

Teruhisa Komura、G.Y. Niu、Takahiro Yamaguchi 等 5 位作者2004-09-28Electroanalysis

Abstract This paper describes electrochemical characteristics of poly(methylene blue) electrolytically deposited on glassy carbon and examines the electrocatalytic activity of the polymer toward oxidation of the coenzyme NADH. Redox‐active properties of the cationic polyelectrolyte arose from both electron self‐exchan…

Electrochemical sensors and biosensorsConducting polymers and applicationsAnalytical Chemistry and Sensors

A 0.18 μm 3.0 V 64 Mb non-volatile phase-transition random-access memory (PRAM)

Woo Yeong Cho、Beak-Hyung Cho、Byung-Gil Choi 等 15 位作者2004-09-28OpenAlex

A non-volatile 64 Mb phase-transition RAM is developed by fully integrating a chalcogenide alloy GST (Ge/sub 2/Sb/sub 2/Te/sub 5/) into 0.18 /spl mu/m CMOS technology. This alloy is programmed by resistive heating. To optimize SET/RESET distribution, a 512 kb sub-core architecture, featuring meshed ground line, is pro…

Optical Network TechnologiesPhotonic and Optical DevicesPhase-change materials and chalcogenides

New Organosilyl Derivatives of the Dawson Polyoxometalate [α2‐P2W17O61(RSi)2O]6−: Synthesis and Mass Spectrometric Investigation

Cédric R. Mayer、Catherine Roch‐Marchal、Hélène Lavanant 等 7 位作者2004-09-28Chemistry - A European Journal

In the field of functionalized polyoxometalates, organosilyl derivatives of polyoxotungstate constitute a special class of hybrid organic-inorganic system. The first organosilyl derivative of the monovacant Dawson heteropolyoxotungstate [alpha2-P2W17O61]10- was obtained by three different methods. The use of two organ…

Metal-Organic Frameworks: Synthesis and ApplicationsPolyoxometalates: Synthesis and ApplicationsAdvanced Nanomaterials in Catalysis

Salt-Induced Multilayer Growth: Correlation with Phase Separation in Solution

Vladimir A. Izumrudov、Eugenia Kharlampieva、Svetlana A. Sukhishvili2004-09-28Macromolecules

We report salt-induced phase separation of polyelectrolyte complexes in solution correlates with deposition of polymer multilayers at a surface. Multilayer growth was followed in situ using FTIR-ATR (Fourier transform infrared spectroscopy by attenuated total reflection). The polymer system was quaternized poly(4-viny…

Polymer Surface Interaction StudiesForce Microscopy Techniques and ApplicationsAdhesion, Friction, and Surface Interactions

Nonlinear elastic properties of decagonal quasicrystals

Xiang Zhou、Chengzheng Hu、Ping Gong 等 4 位作者2004-09-28Physical Review B

Quasicrystals have both positional and orientational long-range order. Thus, they are essentially anisotropic. However, both theory and experiment show that ordinary linear elastic property (linear phonon elasticity) is isotropic for quasicrystals. To detect the quasicrystal anisotropy the nonlinear elasticity should…

Quasicrystal Structures and PropertiesMineralogy and Gemology Studies

Nanostructured Materials

Cury Suryanarayana2004-09-28OpenAlex

Nanocrystalline materials are single-or multiphase polycrystalline solids with a grain size of the order of a few nanometers (1 nm = 109 m = 10 A˚), typically 1-100 nm in at least one dimension. Since the grain sizes are so small, a significant volume of the microstructure in nanocrystalline materials is composed of in…

Nanoporous metals and alloysNanotechnology research and applicationsElectrophoretic Deposition in Materials Science

Thermal conductance enhancement of particle-filled thermal interface materials using carbon nanotube inclusions

Xuejiao Hu、Linan Jiang、Kenneth E. Goodson2004-09-28OpenAlex

Thermal interface materials (TIMs) are widely used in high power integrated circuits. This work introduces multi-walled carbon nanotubes (CNTs) into a silicone composite filled with metal particles, resulting in a TIM with higher thermal conductivity. Anomalous increase in thermal conductivity is found starting at a C…

Nanofluid Flow and Heat TransferHeat Transfer and OptimizationThermal properties of materials

Morphological Evolution of Inorganic Crystal into Zigzag and Helical Architectures with an Exquisite Association of Polymer: A Novel Approach for Morphological Complexity

Yuya Oaki、Hiroaki Imai2004-09-28Langmuir

The morphology of potassium sulfate (K(2)SO(4)) crystals grown in a viscous polymer solution of poly(acrylic acid) (PAA) was remarkably changed from the tilted columnar assembly into zigzag and helical architectures with increasing PAA concentration. The habit modification of orthorhombic K(2)SO(4) with adsorption of…

Surfactants and Colloidal SystemsPolymer composites and self-healingCalcium Carbonate Crystallization and Inhibition

Heat transport in ultrathin dielectric membranes and bridges

Thomas Kühn、Dragoş-Victor Anghel、J. P. Pekola 等 5 位作者2004-09-28Physical Review B

Phonon modes and their dispersion relations in ultrathin homogeneous dielectric membranes are calculated using elasticity theory. The approach differs from the previous ones by a rigorous account of the effect of the film surfaces on the modes with different polarizations. We compute the heat capacity of membranes and…

Thermal properties of materialsSuperconducting and THz Device TechnologyThermal Radiation and Cooling Technologies

DFT Study on the Five Isomers of PW12O403-: Relative Stabilization upon Reduction

Xavier López、Josep M. Poblet2004-09-28Inorganic Chemistry

The electronic characteristics and the redox properties of each isomer of PW(12)O(40)(3)(-) depend on the arrangement adopted by the metal-oxide framework. At the DFT/BP86 level, we computed the structures of the five isomers of PW(12)O(40)(3)(-) in oxidized form. The energy scale fits the experimental findings as wel…

Metal-Organic Frameworks: Synthesis and ApplicationsMagnetism in coordination complexesPolyoxometalates: Synthesis and Applications

Effects of Peripheral Substituents and Axial Ligands on the Electronic Structure and Properties of Iron Phthalocyanine

Meng‐Sheng Liao、Tapas Kar、Sergiu M. Gorun 等 4 位作者2004-09-28Inorganic Chemistry

The effects of peripheral substituents and axial ligands on the electronic structure and properties of iron phthalocyanine, H(16)PcFe, have been investigated using a DFT method. Substitution by electron-withdrawing fluorinated groups alters the ground state of H(16)PcFe and gives rise to large changes in the ionizatio…

Magnetism in coordination complexesPorphyrin and Phthalocyanine ChemistryPhotochemistry and Electron Transfer Studies

Adhesion of Polyether-Modified Poly(acrylic acid) to Mucin

John Cleary、Lev Bromberg、Edmond Magner2004-09-28Langmuir

Pluronic-PAA, a thermogelling copolymer composed of side chains of poly(acrylic acid) (PAA) grafted onto a backbone of Pluronic copolymer, is of interest as a vehicle for the controlled release of compounds. An important feature of such a vehicle is its bioadhesive/mucoadhesive properties, which in the case of Pluroni…

Hydrogels: synthesis, properties, applicationsbiodegradable polymer synthesis and propertiesPolymer Surface Interaction Studies

Resonant Raman spectroscopy of nanotubes

C. Thomsen、Stephanie Reich、Janina Maultzsch2004-09-28Philosophical Transactions of the Royal Society A Mathematical Physical and Engineering Sciences

Single and double resonances in Raman scattering are introduced and six criteria for the observation and identification of double resonances stated. The experimental situation in carbon nanotubes is reviewed in view of these criteria. The evidence for the D mode and the high-energy mode is found to be overwhelming for…

Carbon Nanotubes in CompositesDiamond and Carbon-based Materials ResearchIon-surface interactions and analysis

Evolution of Nanocrystallinity in Periodic Mesoporous Anatase Thin Films

Sung Yeun Choi、Marc Mamak、Scott A. Speakman 等 5 位作者2004-09-28Small

Herein we report the first kinetic study of the intrachannel wall phase-transition of amorphous titania to nanocrystalline anatase for periodic mesoporous titania thin films, monitored by time-resolved in situ high-temperature X-ray diffraction. Structural transformations associated with the phase transition are furth…

Mesoporous Materials and CatalysisPolyoxometalates: Synthesis and ApplicationsLayered Double Hydroxides Synthesis and Applications

A Novel Approach to High Performance Elastomer by Using Clay

Jun Ma、Ping Xiang、Yiu‐Wing Mai 等 4 位作者2004-09-28Macromolecular Rapid Communications

Abstract Summary: A novel method was developed to prepare an exfoliated styrene butadiene rubber (SBR)/clay nanocomposite with a strong interface between the clay layers and the rubber. An exfoliation mechanism was proposed and verified based on X‐ray diffraction (XRD)/transmission electron microscopy (TEM) analyses o…

Structural Behavior of Reinforced ConcretePolymer Nanocomposites and PropertiesPolymer Nanocomposite Synthesis and Irradiation

Topographical Parameters for Specifying a Three-Dimensional Surface

Jouko Peltonen、Mikael Järn、Sami Areva 等 5 位作者2004-09-28Langmuir

The importance of different surface geometries and thereby the need for versatile surface identification by describing a number of different surface features is emphasized. A set of topographical parameters for the description of the amplitude and spatial and hybrid properties of surfaces was utilized for a versatile…

Surface Modification and SuperhydrophobicityAdhesion, Friction, and Surface InteractionsSurface Roughness and Optical Measurements

Layered Organosilicate Nanoparticles with Liquidlike Behavior

Athanasios B. Bourlinos、Subhendu Ray Chowdhury、David D. Jiang 等 7 位作者2004-09-28Small

A clear alternative: Hydrolytic polymerization and assembly of octadecyltrichlorosilane in toluene leads to meltable, structurally stable layered hybrids that are dispersible in common organic solvents (see picture). Such hybrid nanoparticle materials offer great potential as plasticizers and lubricating media.

Polymer Nanocomposites and PropertiesLayered Double Hydroxides Synthesis and ApplicationsSilicone and Siloxane Chemistry

Core energy and Peierls stress of a screw dislocation in bcc molybdenum: A periodic-cell tight-binding study

Ju Li、Cai‐Zhuang Wang、Jinpeng Chang 等 7 位作者2004-09-28Physical Review B

Using a formulation based on anisotropic elasticity we determine the core energy and Peierls stress of the ${a}_{0}∕2[111]$ screw dislocation in bcc molybdenum at $T=0$. We show that a proper definition of the core energy necessarily involves choosing a reference direction $\stackrel{\ifmmode \hat{}\else \^{}\fi{}}{\m…

Microstructure and mechanical propertiesMagnesium Alloys: Properties and ApplicationsFusion materials and technologies

Kinetic Study of a Direct Water Synthesis over Silica-Supported Gold Nanoparticles

David G. Barton、Simon G. Podkolzin2004-09-28The Journal of Physical Chemistry B

The reaction mechanism of water formation from H2 and O2 was studied over a series of silica-supported gold nanoparticles. The metal particle size distributions were estimated with TEM and XRD measurements. Hydrogen and oxygen adsorption calorimetry was used to probe the nature and properties of surface species formed…

Electrocatalysts for Energy ConversionCatalytic Processes in Materials ScienceNanomaterials for catalytic reactions

Electronic Switching Effect and Phase-Change Transition in Chalcogenide Materials

Andrea Redaelli、A. Pirovano、F. Pellizzer 等 6 位作者2004-09-28IEEE Electron Device Letters

The threshold switching mechanism in amorphous chalcogenides is investigated, showing experimental data that once and for all demonstrate its electronic nature. The physical mechanisms responsible for the switching to the highly conductive state are discussed and the impact of cumulative read-out pulses is also invest…

Chalcogenide Semiconductor Thin FilmsPhase-change materials and chalcogenidesOptical and Acousto-Optic Technologies