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Synthesis and Structural Characterization of Bi- and Trimetallic Octacyanometalate(IV) Complexes: [Δ,Λ-MII(en)3][cis-MII(en)2(OH2)][MIV(CN)8]·2H2O and [cis-MII(en)2(OH2)]2[(μ-NC)2MIV(CN)6]·4H2O (MII = Mn, Co, Ni; MIV = Mo, W)

J.R. Withers、C. Ruschmann、Pasano Bojang 等 5 位作者2004-12-16Inorganic Chemistry

Treatment of [M(II)(en)(3)][OTs](2) or methanolic ethylenediamine solutions containing transition metal p-toluenesulfonates (M(II) = Mn, Co) with aqueous K(4)M(IV)(CN)(8).2H(2)O or Cs(3)M(V)(CN)(8) (M(IV) = Mo, W; M(V) = Mo) affords crystalline clusters of [M(II)(en)(3)][cis-M(II)(en)(2)(OH(2))(mu-NC)M(IV)(CN)(7)].2H(…

Metal-Organic Frameworks: Synthesis and ApplicationsMagnetism in coordination complexesLanthanide and Transition Metal Complexes

Molecular Dynamics Computer Simulations of the Interface Structure of Calcium–Alumino–Silicate Intergranular Films between Combined Basal and Prism Planes of α‐Al 2 O 3

Shenghong Zhang、Stephen H. Garofalini2004-12-16Journal of the American Ceramic Society

The interface structures of calcium–alumino–silicate (CAS) glassy intergranular films (IGFs) formed between the combined basal and prism orientations of α‐Al 2 O 3 crystals were studied using molecular dynamics simulations. Preferential adsorption of specific ions from the IGFs to the contacting surfaces of the alumin…

Material Dynamics and PropertiesGlass properties and applicationsMetallic Glasses and Amorphous Alloys

Competing magnetic phases in mixed-valent manganese oxide perovskites

G.-L. Liu、J.-S. Zhou、John B. Goodenough2004-12-16Physical Review B

Measurement of specific heat ${C}_{p}(T)$ below $300\phantom{\rule{0.3em}{0ex}}\mathrm{K}$ of melt-grown samples of ${\mathrm{La}}_{1\ensuremath{-}x}{\mathrm{Ca}}_{x}\mathrm{Mn}{\mathrm{O}}_{3}$ $(0\ensuremath{\leqslant}x\ensuremath{\leqslant}0.3)$ and ${R}_{0.7}{A}_{0.3}\mathrm{Mn}{\mathrm{O}}_{3}$ $(R=\text{rare}\te…

Magnetic and transport properties of perovskites and related materialsAdvanced Condensed Matter PhysicsThermal Expansion and Ionic Conductivity

Synthesis of Germanium Nanocubes by a Low-Temperature Inverse Micelle Solvothermal Technique

Wang、Jianyu Huang、Ren2004-12-16Langmuir

We present a low-temperature inverse micelle solvothermal approach for the synthesis of germanium nanocubes using the surfactant heptaethylene glycol monododecyl ether as a capping agent. X-ray diffraction results indicate that the as-prepared nanocubes are diamond-type pure germanium. Transmission electron microscopy…

Quantum Dots Synthesis And PropertiesMolecular Junctions and NanostructuresNanowire Synthesis and Applications

[Cr iii (L)(CN) 4 ] − : a new building block in designing cyanide-bridged 4,2-ribbon-like chains {[Cr iii (L)(CN) 4 ] 2 Mn(H 2 O) 2 }·nH 2 O [L = 2-aminomethylpyridine (n = 6) and 1,10-phenanthroline (n = 4)]

Luminita Marilena Toma、Rodrigue Lescouëzec、Jacqueline Vaissermann 等 7 位作者2004-12-16New Journal of Chemistry

The preparation, X-ray crystallography and magnetic study of compounds PPh4[Cr(ampy)(CN)4]·H2O (1), PPh4[Cr(phen)(CN)4]·H2O·CH3OH (2), {[Cr(ampy)(CN)4]2Mn(H2O)2}·6H2O (3) and {[Cr(phen)(CN)4]2Mn(H2O)2}·4H2O (4), with PPh4+ = tetraphenylphosphonium cation, ampy = 2-aminomethylpyridine and phen = 1,10-phenanthroline, ar…

Magnetism in coordination complexesLanthanide and Transition Metal ComplexesOrganic and Molecular Conductors Research

Mathematical Modeling of Free-Radical Ethylene Copolymerization in High-Pressure Tubular Reactors

Costas Kiparissides、Apostolos Baltsas、Stratos Papadopoulos 等 7 位作者2004-12-16Industrial & Engineering Chemistry Research

A comprehensive mathematical model is developed for the free-radical copolymerization of ethylene with various comonomers (e.g., vinyl acetate, methyl or ethyl acrylate, and acrylic or methacrylic acid) in high-pressure tubular reactors. Polar copolymers usually exhibit lower crystallinity and yield strength than low-…

Phase Equilibria and ThermodynamicsProcess Optimization and IntegrationThermal and Kinetic Analysis

Metastable States in Alumina‐Rich La 2 O 3 :Al 2 O 3 and Nd 2 O 3 :Al 2 O 3

Thomas S. Key、Buckley Crist2004-12-16Journal of the American Ceramic Society

Alumina‐rich mixtures of La 2 O 3 and Al 2 O 3 have equilibrium phases that are perovskite (LaAlO 3 ) and β‐alumina (LaAl 11 O 18 ). Annealing initially glassy samples with compositions 3La 2 O 3 –5Al 2 O 3 or 11La 2 O 3 –14Al 2 O 3 between 860° and 1075°C creates a metastable state that is clearly detected by X‐ray d…

Ferroelectric and Piezoelectric MaterialsGlass properties and applicationsMicrowave Dielectric Ceramics Synthesis

Characterization of an archaeal malic enzyme from the hyperthermophilic archaeon Thermococcus kodakaraensis KOD1

Wakao Fukuda、Yulia Sari Ismail、Toshiaki Fukui 等 5 位作者2004-12-16Archaea

Although the interconversion between C4 and C3 compounds has an important role in overall metabolism, limited information is available on the properties and regulation of enzymes acting on these metabolites in hyperthermophilic archaea. Malic enzyme is one of the enzymes involved in this interconversion, catalyzing th…

Bacterial Genetics and BiotechnologyEnzyme Structure and FunctionAmino Acid Enzymes and Metabolism

Self‐Cleaning Fabrics for Decontamination of Organophosphorous Pesticides and Related Chemical Agents

A. Singh、Y. Lee、Walter J. Dressick2004-12-16Advanced Materials

Cotton threads bearing adsorbed branched polyethylenimine–organophosphorous hydrolase (BPEI/OPH) multilayers are woven into cotton cloth (CC) that actively hydrolyzes methyl parathion (MPT) in solution to p-nitrophenol (PNP) over several weeks. These results form the basis for smart fabrics capable of remediation of e…

Microplastics and Plastic PollutionPolymer Surface Interaction StudiesPesticide and Herbicide Environmental Studies

Synthesis of Nanocrystalline Boron Carbide via a Solvothermal Reduction of CCl 4 in the Presence of Amorphous Boron Powder

Yunle Gu、Luyang Chen、Yitai Qian 等 5 位作者2004-12-16Journal of the American Ceramic Society

Nanocrystalline boron carbide (B 4 C) was synthesized via a solvothermal reduction of carbon tetrachloride using metallic lithium as reductant in the presence of amorphous boron powder at 600°C in an autoclave. The X‐ray diffraction pattern of the product powder was indexed to the hexagonal B 4 C phase, with lattice c…

Advanced ceramic materials synthesisDiamond and Carbon-based Materials ResearchBoron and Carbon Nanomaterials Research

Vulcanization characteristics and mechanical properties of natural rubber–scrap rubber compositions filled with leather particles

K. Ravichandran、N. Natchimuthu2004-12-16Polymer International

Abstract Scrap rubber recycling combined with waste leather particles in natural rubber compounds has been studied. The effect of leather and scrap rubber loading on vulcanization characteristics of natural rubber compounds has been evaluated. The presence of leather was found to reduce the scorch time and increase th…

Polymer crystallization and propertiesPolymer Nanocomposites and PropertiesNatural Fiber Reinforced Composites

Effect of Sucrose on Fabrication of Ceramic Foams from Aqueous Slurries

Mamata Pradhan、Parag Bhargava2004-12-16Journal of the American Ceramic Society

Ceramic foams with porosity exceeding 90% were prepared by direct foaming and casting of aqueous suspensions containing cetyl trimethyl ammonium bromide (CTAB) as a foaming agent. Foaming of the suspensions, particularly with lower viscosity, was initially non‐homogeneous but the foam appeared to homogenize with milli…

Catalysis and Hydrodesulfurization StudiesPickering emulsions and particle stabilization

Ballistic Impact of Braided Composites with a Soft Projectile

Gary D. Roberts、J. Michael Pereira、Duane M. Revilock 等 6 位作者2004-12-16Journal of Aerospace Engineering

Impact tests using a soft gelatin projectile were performed to identify failure modes that occur at high strain energy density during impact loading. Failure modes were identified for aluminum plates and for composites plates and half-rings made from triaxial carbon fiber braid having a 0∕±60° architecture. For alumin…

Energetic Materials and CombustionHigh-Velocity Impact and Material BehaviorStructural Response to Dynamic Loads

Supramolecular Multiscale Fibers through One‐Dimensional Assembly of Dendritic Molecules

Maryna Ornatska、Sergiy Peleshanko、B Rybak 等 5 位作者2004-12-16Advanced Materials

One-dimensional supramolecular structures self-assemble from irregular, highly branched, flexible amphiphiles containing a polyester core and an alkyl- or anthracene-functionalized shell. A combination of intermolecular interactions and steric limitations cause the structures to form nearly perfectly organized microfi…

Luminescence and Fluorescent MaterialsSupramolecular Self-Assembly in MaterialsDendrimers and Hyperbranched Polymers

Amphiphilic meso-Disubstituted Porphyrins: Synthesis and the Effect of the Hydrophilic Group on Absorption Spectra at the Air−Water Interface

Masaru Yao、Yuko Iwamura、Hidenari Inoue 等 4 位作者2004-12-16Langmuir

Five amphiphilic meso-disubstituted porphyrins bearing one polar group were synthesized, and their monolayer films were prepared. Their limiting molecular areas obtained from pi-A isotherms were 0.5-0.6 nm2, which were smaller than those of the corresponding meso-tetrasubstituted porphyrins. At the air-water interface…

Porphyrin and Phthalocyanine ChemistryPhotochemistry and Electron Transfer StudiesLuminescence and Fluorescent Materials

Matrix Cracking in 3D Orthogonal Melt‐Infiltrated SiC/SiC Composites with Various Z ‐Fiber Types

Gregory N. Morscher、Hee Mann Yun、James A. DiCarlo2004-12-16Journal of the American Ceramic Society

The occurrence of matrix cracks in melt‐infiltrated SiC/SiC composites with a three‐dimensional (3D) orthogonal architecture was determined at room temperature for specimens tested in tension parallel to the Y ‐direction (perpendicular to Z ‐bundle weave direction). The fiber types were Sylramic and Sylramic‐iBN in th…

Advanced ceramic materials synthesisMechanical Behavior of CompositesAluminum Alloys Composites Properties

Numerical Simulation of Anisotropic Shrinkage in a 2D Compact of Elongated Particles

Veena Tikare、Michael Braginsky、Eugene A. Olevsky 等 4 位作者2004-12-16Journal of the American Ceramic Society

Microstructural evolution during simple solid‐state sintering of two‐dimensional compacts of elongated particles packed in different arrangements was simulated using a kinetic, Monte Carlo model. The model used simulates curvature‐driven grain growth, pore migration by surface diffusion, vacancy formation, diffusion a…

Advanced ceramic materials synthesisAluminum Alloys Composites PropertiesInjection Molding Process and Properties

Enhanced Emission of Nile Red Fluorescent Nanoparticles Embedded in Hybrid Sol−Gel Glasses

M. Luisa Ferrer、Francisco del Monte2004-12-16The Journal of Physical Chemistry B

Highly fluorescent Nile Red (NR) nanoparticles embedded in a hybrid sol-gel glass are reported. The crystallite growth within the confined system created by the porous hybrid matrix results in NR nanoparticles of averaged dimensions below 36 nm. The preparation process allows for the control of both the conformation a…

Quantum Dots Synthesis And PropertiesPorphyrin and Phthalocyanine ChemistryLuminescence and Fluorescent Materials

Correlation between Sm2(Fe,Ga)17 and its precursor Sm(Fe,Ga)9

Lotfi Bessais、E. Dorolti、C. Djéga‐Mariadassou2004-12-16Journal of Applied Physics

We have shown that the out-of-equilibrium hexagonal P6∕mmm phase adopts the stoichiometry Sm(Fe,Ga)9 in the Sm–Fe–Ga system. X-ray diffraction analysis has been combined with Mössbauer spectrometry. A specific program for the Wigner–Seitz cell (WSC) volume calculation of the equilibrium and of the metastable structure…

Magnetic properties of thin filmsMagnetic Properties and ApplicationsMagnetic Properties of Alloys

Synthesis, Crystal Structure, and High-Precision High-Frequency and -Field Electron Paramagnetic Resonance Investigation of a Manganese(III) Complex: [Mn(dbm)2(py)2](ClO4)

Guillem Aromı́、Joshua Telser、Andrew Ozarowski 等 6 位作者2004-12-16Inorganic Chemistry

The complex [Mn(dbm)(2)(py)(2)](ClO(4)) (dbm = anion of 1,3-diphenyl-1,3-propanedione (dibenzoylmethane), py = pyridine) was synthesized and characterized by X-ray crystallography. It has tetragonally distorted geometry with the axial positions occupied by the py ligands and the equatorial positions by the dbm ligands…

Metal complexes synthesis and propertiesMagnetism in coordination complexesLanthanide and Transition Metal Complexes