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Bifunctional Molecular Sieve Catalysts for the Benign Ammoximation of Cyclohexanone: One-Step, Solvent-Free Production of Oxime and ε-Caprolactam with a Mixture of Air and Ammonia

Robert Raja、Gopinathan Sankar、John Meurig Thomas2001-07-31Journal of the American Chemical Society

ADVERTISEMENT RETURN TO ISSUEPREVCommunicationNEXTBifunctional Molecular Sieve Catalysts for the Benign Ammoximation of Cyclohexanone: One-Step, Solvent-Free Production of Oxime and ε-Caprolactam with a Mixture of Air and AmmoniaRobert Raja, Gopinathan Sankar, and John Meurig ThomasView Author Information Davy Faraday…

Covalent Organic Framework ApplicationsIonic liquids properties and applicationsNanomaterials for catalytic reactions

High-temperature structural evolution ofRNiO3(R=Ho,Y, Er, Lu)perovskites: Charge disproportionation and electronic localization

J. A. Alonso、M. J. Martínez‐Lope、M. T. Casáis 等 6 位作者2001-07-31Physical review. B, Condensed matter

The structural changes of polycrystalline $R{\mathrm{NiO}}_{3}$ perovskites $(R=\mathrm{Ho},$ Y, Er, and Lu, prepared under high-oxygen pressure) across the metal-insulator (MI) transition ${(T}_{\mathrm{MI}}$ ranging between 573 and 600 K) have been studied by high-resolution neutron- and synchrotron diffraction tech…

Magnetic and transport properties of perovskites and related materialsAdvanced Condensed Matter PhysicsThermal Expansion and Ionic Conductivity

Fluorescent Probes as Reporters on the Local Structure and Dynamics in Sol−Gel-Derived Nanocomposite Materials

Tracey Keeling-Tucker、John D. Brennan2001-07-31Chemistry of Materials

The use of steady-state and time-resolved fluorescence spectroscopy to probe the internal microenvironment of sol−gel-derived organic−inorganic nanocomposites formed from alkoxysilane precursors is reviewed. The review focuses on the use of small organic probes and fluorescent biomolecules that provide information on…

Porphyrin and Phthalocyanine ChemistryLuminescence and Fluorescent MaterialsMesoporous Materials and Catalysis

Reaction-Bonded Silicon Carbide by Reactive Infiltration

Prasert Sangsuwan、Joaquín Orejas、Jorge E. Gatica 等 5 位作者2001-07-31Industrial & Engineering Chemistry Research

Exothermic reactions between a porous matrix and an infiltrating melt provide a more economic alternative for synthesizing many ceramics, intermetallics, and composites. It has recently been demonstrated that infiltration of cast microporous carbon preforms by silicon melt can be used to fabricate high-density, nearly…

Advanced ceramic materials synthesisHeat and Mass Transfer in Porous MediaAluminum Alloys Composites Properties

Metal-to-Ligand Electron Transfer in Diiminopyridine Complexes of Mn−Zn. A Theoretical Study

Peter H. M. Budzelaar、Bas de Bruin、A.W. Gal 等 5 位作者2001-07-31Inorganic Chemistry

A series of complexes ML2(x+) (M = Mn-Zn, L = 2,6-bis(iminomethyl)pyridine) was investigated by theoretical methods. Electron transfer from the metal "t(2g)" orbitals to the ligand pi orbitals is reflected in the elongation of ligand C-N bonds and shortening of the C(py)-C(imine) bonds. Using zinc complexes as referen…

Metal complexes synthesis and propertiesMetal-Catalyzed Oxygenation MechanismsMagnetism in coordination complexes

Collision Drag Effect on Propagation of Sound in Liquid ${}^3$He in Aerogel

Takayuki Ichikawa、Mikio Ymamoto、Seiji Higashitani 等 4 位作者2001-07-31arXiv

Sound propagation in a Fermi liquid with impurities is studied using the Landau-Boltzmann equation and the result is compared with a recent experiment in liquid ${}^3$He in aerogel by Northwestern University group. The sound absorption calculated using the fixed impurity model is a few orders of magnitude larger than…

Materials Science

Modelling (001) surfaces of II-VI semiconductors

M. Ahr、M. Biehl、T. Volkmann2001-07-31arXiv

First, we present a two-dimensional lattice gas model with anisotropic interactions which explains the experimentally observed transition from a dominant c(2x2) ordering of the CdTe(001) surface to a local (2x1) arrangement of the Cd atoms as an equilibrium phase transition. Its analysis by means of transfer-matrix an…

Materials Sciencecond-mat.stat-mech

Epitaxy and Magneto-transport properties of the diluted magnetic semiconductor p- Be(1-x)MnxTe

L. Hansen、D. Ferrand、G. Richter 等 10 位作者2001-07-31arXiv

We report on the MBE-growth and magnetotransport properties of p-type BeMnTe, a new ferromagnetic diluted magnetic semiconductor. BeMnTe thin film structures can be grown almost lattice matched to GaAs for Mn concentrations up to 10% using solid source MBE. A high p-type doping with nitrogen can be achieved by using a…

Materials Science

Irreversible nucleation in multilayer growth

Paolo Politi、Claudio Castellano2001-07-31arXiv

The epitaxial growth process of a high symmetry surface occurs because adatoms meet and nucleate new islands, that eventually coalesce and complete atomic layers. During multilayer growth, nucleation usually takes place on top of terraces where the geometry of the diffusion process is well defined: We have studied in…

cond-mat.stat-mechMaterials Science

A Highly Efficient Catalyst for the “Living” and “Immortal” Polymerization of ε-Caprolactone and l-Lactide

Yi‐Chang Liu、Bao‐Tsan Ko、Chu‐Chieh Lin2001-07-31Macromolecules

A novel ligand, 2,2‘-methylenebis(4,6-di(1-methyl-1-phenylethyl)phenol) (MMPEP-H 2 ) ( 1 ), has been prepared by the reaction of 2,4-bis(α,α-dimethylbenzyl)phenol with formaldehyde in the presence of a catalytic amount of benzenesulfonic acid. Further reaction of compound 1 with Me 3 Al in diethyl ether produces a fou…

biodegradable polymer synthesis and propertiesSilicone and Siloxane ChemistryCarbon dioxide utilization in catalysis

Structure and Thermomechanical Properties of Polyurethane Block Copolymers with Shape Memory Effect

Bo Sun Lee、Byoung Chul Chun、Yong‐Chan Chung 等 5 位作者2001-07-31OpenAlex

Shape memory polyurethane (PU) block copolymers composed of 4,4‘-methylenebis(phenylisocyanate), poly(tetramethylene glycol), and 1,4-butanediol as a chain extender were synthesized by a two-step process. FT-IR spectra showed that carbonyl peak appearing at 1700 cm -1 increased with higher hard segment content, wherea…

Polymer composites and self-healingSynthetic Organic Chemistry MethodsMarine Sponges and Natural Products

Detonation synthesis ultradispersed diamonds: properties and applications

V. Yu. Dolmatov2001-07-31OpenAlex

Published data on the properties of a novel nanomaterial viz., detonation synthesis ultradispersed diamonds (UDD), are summarised and systematised for the first time. Certain properties of UDD synthesised under different conditions are compared. Particular attention is drawn to substantiation of the cluster model of U…

Carbon Nanotubes in CompositesDiamond and Carbon-based Materials ResearchLaser-Ablation Synthesis of Nanoparticles

A Survey of Structure−Property Relationships of Surfaces that Resist the Adsorption of Protein

Emanuele Ostuni、Robert Chapman、R. Erik Holmlin 等 5 位作者2001-07-31OpenAlex

This paper describes the use of surface plasmon resonance (SPR) spectroscopy and self-assembled monolayers (SAMs) to determine the characteristics of functional groups that give surfaces the ability to resist the nonspecific adsorption of proteins from solution. Mixed SAMs presenting different functional groups were p…

Advanced Biosensing Techniques and ApplicationsMolecular Junctions and NanostructuresPolymer Surface Interaction Studies

Characterization of retanned chrome bovine leather by thermomechanical analysis

T. Bosch、A. M. Manich、Julieta Carilla 等 5 位作者2001-07-30Journal of Applied Polymer Science

Abstract The thermomechanical analysis is applied to characterize the shrinking process of bovine chrome leather. The interpretation of the curves obtained is performed and a value of glass transition temperature is estimated. The influence of the sampling zone on the thermomechanical parameters is discussed. The infl…

Collagen: Extraction and CharacterizationMaterials Engineering and ProcessingMaterial Properties and Processing

SEPARATION OF HYDROGEN ISOTOPES BY CHEMICAL ISOTOPE EXCHANGE IN SYSTEMS INVOLVING METAL AND INTERMETALLIC COMPOUND HYDRIDES

B.M. Andreev、Э. П. Магомедбеков2001-07-30Separation Science and Technology

This article reviews and analyzes the results obtained by studying isotope effects and kinetics of isotope exchange in systems involving heavy hydrogen isotopes and intermetallic compound hydrides for the last 20 years. Particular attention is paid to the analysis of possibilities to realize the separation process in…

Fusion materials and technologiesNuclear Materials and PropertiesChemical Synthesis and Characterization

Static analysis of off-axis crystal film growth onto a lattice-mismatched substrate

Ayaka Yamada、Paul Fons、Ralf Hunger 等 6 位作者2001-07-30Applied Physics Letters

The interface construction of tilt growth that is sometimes observed for epilayer growth on a lattice mismatched substrate is modeled on the basis that tilt relieves misfit strain in the epilayer. In this model off-axis misfit accommodation is assumed to be due to only tilt dislocations or tilt dislocations combined w…

Copper Interconnects and ReliabilitySemiconductor materials and devicesOptical Coatings and Gratings

Selective adsorption and patterning of Si nanoparticles fabricated by laser ablation on functionalized self-assembled monolayer

Kenji Hata、M. Fujita、Shoji Yoshida 等 9 位作者2001-07-30Applied Physics Letters

We demonstrate an in situ selective adsorption of Si nanoparticles fabricated by laser ablation on a functionalized self-assembled monolayer (SAM). Si nanoparticles adsorbed on –CH3 terminated a SAM while Si particles did not adsorb on –NH2, –F, –OH, and –COOH, terminated SAMs. The end group of a SAM solely determines…

Force Microscopy Techniques and ApplicationsMolecular Junctions and NanostructuresSilicon Nanostructures and Photoluminescence

Study on aging of clay–rubber masterbatch from modified clay

Mei Chen、Ning‐Jian Ao、Ying Chen 等 9 位作者2001-07-30Journal of Applied Polymer Science

Abstract Clay was modified by using a polymeric coating agent, a silicane coupling agent, and a titanate coupling agent together with the antioxidant for preparing the clay–rubber masterbatch. After the thermooxidative, photooxidative, and ozone aging, the properties of the masterbatch were also determined. The result…

Polymer Science and PVCPolymer Nanocomposites and PropertiesPolymer Nanocomposite Synthesis and Irradiation

<title>Innovative beam column connections using shape memory alloys</title>

Roberto T. Leon、Reginald DesRoches、Justin Ocel 等 4 位作者2001-07-30Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

The application of Nitinol shape memory alloys (SMA) in steel connections is evaluated using connections incorporating SMA tendons. Shape memory alloys are a class of alloys that exhibit thermo-mechanical characteristics that are ideally suited for seismic applications. They have the ability to dissipate significant e…

Shape Memory Alloy Transformations

Nonisothermal crystallization of isotactic polypropylene blended with poly(α‐pinene). I. Bulk crystallization

Maria Laura Di Lorenzo、Sossio Cimmino、Clara Silvestre2001-07-30Journal of Applied Polymer Science

Abstract The influence of a natural terpene resin, poly(α‐pinene) (PαP), on the nonisothermal crystallization process of isotactic polypropylene (iPP) was investigated. The solidification process strongly depends on cooling rate, composition, and miscibility of the system. For the blends containing PαP up to 30 wt %,…

Polymer Nanocomposites and PropertiesPolymer crystallization and propertiesbiodegradable polymer synthesis and properties