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Quantum critical transition from charge-ordered to superconducting state in the negative-Uextended Hubbard model on a triangular lattice

S. Mazumdar、R. Torsten Clay2008-05-23Physical Review B

We demonstrate a robust frustration-driven charge order to superconductivity transition in the half-filled negative-$U$ extended Hubbard model. Superconductivity extends over a broad region of the parameter space. We argue that the model provides the correct insight to understanding unconventional superconductivity in…

Physics of Superconductivity and MagnetismPerovskite Materials and ApplicationsOrganic and Molecular Conductors Research

Thermal and dielectric properties of bismaleimide‐triazine resins containing octa(maleimidophenyl)silsesquioxane

Hongwei Cao、Riwei Xu、Dingsheng Yu2008-05-23Journal of Applied Polymer Science

Abstract Octa(maleimidophenyl)silsesquioxane (OMPS) was synthesized, characterized, and employed to modify the BT resin which composed of 4,4′‐bismaleimidodiphenylmethane (BMI) and 2,2′‐bis(4‐cyanatophenyl)propane (BCE). The curing reaction between OMPS and BT resin was first investigated. It was found that OMPS accel…

Synthesis and characterization of novel inorganic/organometallic compoundsSynthesis and properties of polymersSilicone and Siloxane Chemistry

Microstructure and electrical properties of (Li, Ag, Ta, Sb)-modified (K0.50Na0.50)NbO3 lead-free ceramics with good temperature stability

Jiagang Wu、Dingquan Xiao、Yuanyu Wang 等 8 位作者2008-05-23Journal of Physics D Applied Physics

0.98[(K0.4725Na0.4725Li0.055)NbO3]–0.02Ag(Ta1−xSbx)O3 lead-free piezoelectric ceramics were prepared by the conventional mixed-oxide method. The effects of the Sb content on the microstructure and the electrical properties of the ceramics were systematically investigated. The experimental results show that Sb strongly…

Ferroelectric and Piezoelectric MaterialsAcoustic Wave Resonator TechnologiesMicrowave Dielectric Ceramics Synthesis

An efficient algorithm for solving nonlinear equations with a minimal number of trial vectors: Applications to atomic-orbital based coupled-cluster theory

Marcin Ziółkowski、Ville Weijo、Poul Jørgensen 等 4 位作者2008-05-23The Journal of Chemical Physics

The conjugate residual with optimal trial vectors (CROP) algorithm is developed. In this algorithm, the optimal trial vectors of the iterations are used as basis vectors in the iterative subspace. For linear equations and nonlinear equations with a small-to-medium nonlinearity, the iterative subspace may be truncated…

Nonlinear Optical Materials ResearchSpectroscopy and Quantum Chemical StudiesMolecular spectroscopy and chirality

Preferential Oxidation of Carbon Monoxide in Hydrogen Stream over Au/MgOx−TiO2 Catalysts

Li-Hsin Chang、Yu‐Wen Chen、Natarajan Sasirekha2008-05-23Industrial & Engineering Chemistry Research

A series of Au/MgO x −TiO 2 with various Mg/Ti molar ratios was prepared to study its catalytic activity for preferential oxidation of carbon monoxide in hydrogen-rich stream (PROX). An incipient wetness impregnation method was used to prepare the MgO x −TiO 2 support, using aqueous solutions of Mg(NO 3 ) 2 on TiO 2 c…

Catalytic Processes in Materials ScienceCatalysis and Hydrodesulfurization StudiesCatalysis and Oxidation Reactions

Ordered Mesoporous Ni Nanowires with Enhanced Hydrogenation Activity Prepared by Electroless Plating on Functionalized SBA-15

Hui Li、Hong Lin、Hong Lin 等 9 位作者2008-05-23Chemistry of Materials

Highly ordered mesoporous Ni nanowires were synthesized by Ni electroless plating on the amine-functionalized SBA-15 (NH 2 −SBA-15) support, followed by removing the silica template with NaOH. The incorporation of amine groups into the pore channels and the subsequent activation of NH 2 −SBA-15 with PdCl 2 acetone sol…

Electrocatalysts for Energy ConversionMesoporous Materials and CatalysisNanomaterials for catalytic reactions

Ru-Doped Cobalt−Zirconia Nanocomposites by Flame Synthesis: Physicochemical and Catalytic Properties

Wey Yang Teoh、Ridwan Setiawan、Jan‐Dierk Grunwaldt 等 5 位作者2008-05-23Chemistry of Materials

Nanocomposites of Ru-doped cobalt−zirconia (20 wt % Co) were made by rapid and scalable flame spray pyrolysis (FSP). They were characterized by nitrogen adsorption, X-ray diffraction, electron microscopy, and X-ray photoelectron spectroscopy revealing that cobalt clusters were highly dispersed within the zirconia matr…

Catalytic Processes in Materials ScienceCatalysts for Methane ReformingCatalysis and Oxidation Reactions

Kinetics of gypsum dehydration at reduced pressure: an energy dispersive X-ray diffraction study

Marilena Carbone、Paolo Ballirano、Ruggero Caminiti2008-05-23European Journal of Mineralogy

Gypsum (CaSO(4)center dot 2H(2)O) dehydration kinetics were investigated through energy dispersive X-ray diffraction (EDXD), under reduced pressure (100 Pa), in the temperature range 313-353 K. The process follows the JMAK (Johnson-Mehl-Avrami Kinetic) model. The fitting procedure of the Arrhenius expression provides…

Calcium Carbonate Crystallization and InhibitionCrystallization and Solubility StudiesThermal and Kinetic Analysis

Inhibition of steel corrosion in HCl media by phosphite compound

L. Herrag、B. Hammouti、S. Elkadiri 等 6 位作者2008-05-23Pigment & Resin Technology

Purpose The purpose of this paper is to investigate the inhibitive effect of the phosphite NaCo(H 2 PO 3 ) 3 •H 2 O (PhCo) for the corrosion of mild steel in HCl solutions. The study is another trial to find a mineral inhibitor for mild steel corrosion. Design/methodology/approach The inhibitory effect has been evalua…

Corrosion Behavior and InhibitionHydrogen embrittlement and corrosion behaviors in metalsConcrete Corrosion and Durability

Exergy Analysis of a Gas Turbine Cycle With Steam Generation for Methane Conversion Within Solid Oxide Fuel Cells

Mikhail Granovskii、İbrahim Dinçer、Marc A. Rosen2008-05-23Journal of Electrochemical Energy Conversion and Storage

The combination of fuel cells with conventional mechanical power generation technologies (heat engines) promotes effective transformation of the chemical energy of fuels into electrical work. The implementation of solid oxide fuel cells (SOFCs) within gas turbine systems powered by natural gas (methane) requires an in…

Advancements in Solid Oxide Fuel CellsChemical Looping and Thermochemical ProcessesCatalysis and Oxidation Reactions

Ni–Fe Alloy-Supported Intermediate Temperature SOFCs Using LaGaO3 Electrolyte Film for Quick Startup

Tatsumi Ishihara、Jingwang Yan、Makiko Enoki 等 5 位作者2008-05-23Journal of Electrochemical Energy Conversion and Storage

Intermediate temperature solid oxide fuel cells (SOFCs), which are highly tolerant against a thermal cycle, are studied by using the Ni–Fe porous alloy substrate prepared by an in situ reduction. It was found that Ni–Fe alloy exhibits high activity against anodic reaction and suitable compatibility with LaGaO3 electro…

Advancements in Solid Oxide Fuel CellsCatalysis and Oxidation ReactionsElectronic and Structural Properties of Oxides

Ferromagnetic semiconductors and the role of disorder

Bruce W. Wessels2008-05-23New Journal of Physics

In this paper, we report on the role of short-range disorder in stabilizing ferromagnetism in transition metal-doped compound semiconductors. While both theory and experiment have centered on dilute magnetic semiconductors where the magnetic ions substitute randomly for cation sites, there is increasing evidence that…

ZnO doping and propertiesMagnetic and transport properties of perovskites and related materialsElectronic and Structural Properties of Oxides

Synthesis of random polyampholyte brushes by atom transfer radical polymerization

Sarah Sanjuan、Yvette Tran2008-05-23Journal of Polymer Science Part A Polymer Chemistry

Abstract We report the synthesis of random polyampholyte brushes containing 2‐(dimethylamino)ethyl methacrylate (DMAEMA) and methacrylic acid (MAA). The preparation of polyampholyte brushes is performed by the “grafting from” strategy using surface‐initiated atom transfer radical polymerization (ATRP). The first step…

Advanced Polymer Synthesis and CharacterizationPolymer Surface Interaction StudiesPickering emulsions and particle stabilization

Effect of die geometry on foaming behaviors of high‐melt‐strength polypropylene with CO2

Patrick Lee、Wanrudee Kaewmesri、Jing Wang 等 7 位作者2008-05-23Journal of Applied Polymer Science

Abstract This article reports on a systematic study that was conducted to investigate the effects of die geometry (i.e., pressure and pressure drop rate) on the cell nucleation and growth behaviors of noncrosslinked high‐melt‐strength (HMS) polypropylene (PP) foams blown with supercritical CO 2 . The experimental resu…

Polymer crystallization and propertiesPhase Equilibria and ThermodynamicsPolymer Foaming and Composites

Crystallization of polycaprolactone–clay nanocomposites

Leandro N. Ludueña、Analı́a Vázquez、Vera A. Álvarez2008-05-23Journal of Applied Polymer Science

Abstract The isothermal crystallization process of polycaprolactone/clay nanocomposites was studied at several temperatures. The effects of the clay type (modified and unmodified) and clay content were analyzed. Bulk crystallization was studied with differential scanning calorimetry and modeled with Avrami's equation.…

Polymer crystallization and propertiesPolymer Nanocomposites and Propertiesbiodegradable polymer synthesis and properties

Newly Synthesized Water Soluble Cholinium-Purpurin Photosensitizers and Their Stabilized Gold Nanoparticles as Promising Anticancer Agents

Dorjnamjin Demberelnyamba、Mama Ariunaa、Young Key Shim2008-05-23International Journal of Molecular Sciences

For possible future use in Photodynamic Therapy (PDT) and/or Photothermal Therapy (PTT) of cancer and screening of cancer cells a new type of ionic liquid photosensitizer -Cholinium-Purpurin-18 (Chol-Pu-18) - was synthesized and small gold (Au) nanoparticles, stabilized by this photosensitizer were prepared without ad…

Gold and Silver Nanoparticles Synthesis and ApplicationsAdvanced biosensing and bioanalysis techniquesInnovative Microfluidic and Catalytic Techniques Innovation

Antireflection Polymer Hole Array Structures by Imprinting Using Metal Molds from Anodic Porous Alumina

Takashi Yanagishita、Kazuyuki Nishio、Hideki Masuda2008-05-23Applied Physics Express

Antireflection (AR) structures of polymer composed of an ordered array of holes with a tapered shape were formed by imprinting using a metal mold prepared from an anodic porous alumina. The metal molds (Ni) were prepared using an anodic porous alumina as a template and were used for the photoimprinting of polymers. Th…

Surface Modification and SuperhydrophobicityOptical Coatings and GratingsAnodic Oxide Films and Nanostructures

Determining gap nodal structures in Fe-based superconductors: Theory of the angle dependence of the low-temperature specific heat in an applied magnetic field

S. Gräser、G. R. Boyd、Chao Cao 等 6 位作者2008-05-23Physical Review B

Since the discovery of high-${T}_{c}$ ${\mathrm{LaO}}_{1\ensuremath{-}x}{\mathrm{F}}_{x}\mathrm{FeAs}$ and other such systems based on $\mathrm{FeAs}$ layers, several proposals have been made for the superconducting order parameter ${\ensuremath{\Delta}}_{\mathbf{k}}$, on both phenomenological and microscopic grounds.…

Magnetic and transport properties of perovskites and related materialsRare-earth and actinide compoundsIron-based superconductors research

The Very‐Low Shear Modulus of Multi‐Walled Carbon Nanotubes Determined Simultaneously with the Axial Young's Modulus via in situ Experiments

Xianlong Wei、Yang Liu、Qing Chen 等 5 位作者2008-05-23Advanced Functional Materials

Abstract The natural frequencies ( f ) as a function of the length ( L ) of single, multi‐walled carbon nanotubes (CNTs) are measured using the electric‐field‐induced resonance method together with the “nanoknife” technique for cutting nanotubes to the desired length. The experimental f ‐ L data for short CNTs are fou…

Carbon Nanotubes in CompositesForce Microscopy Techniques and ApplicationsMechanical and Optical Resonators

Investigation of pure and Co2+-doped ZnO quantum dot electronic structures using the density functional theory: choosing the right functional

Ekaterina Badaeva、Yong Feng、Daniel R. Gamelin 等 4 位作者2008-05-23New Journal of Physics

The electronic structures of pure and Co 2+ -doped ZnO quantum dots (QDs) with sizes up to 300 atoms were investigated using three different density functional theory approximations: local spin density approximation (LSDA), gradient-corrected Perdew–Burke–Ernzerhof (PBE) and the hybrid PBE1 functionals with LANL2DZ ps…

ZnO doping and propertiesMagnetic and transport properties of perovskites and related materialsAdvanced Condensed Matter Physics