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Theory of the observed ultralow friction between sliding polyelectrolyte brushes

J. B. Sokoloff2008-07-07The Journal of Chemical Physics

It is shown using a method based on a modified version of the mean field theory of Miklavic and Marcelja [J. Phys. Chem. 92, 6718 (1988)] that it should be possible for osmotic pressure due to the counterions associated with the two polyelectrolyte polymer brush coated surfaces to support a reasonable load (i.e., abou…

Electrostatics and Colloid InteractionsPolymer Surface Interaction StudiesForce Microscopy Techniques and Applications

Synthesis, Contact Printing, and Device Characterization of Ni-Catalyzed, Crystalline InAs Nanowires

Alexandra C. Ford、Johnny C. Ho、Zhiyong Fan 等 8 位作者2008-07-07arXiv

InAs nanowires have been actively explored as the channel material for high performance transistors owing to their high electron mobility and ease of ohmic metal contact formation. The catalytic growth of non-epitaxial InAs nanowires, however, has often relied on the use of Au colloids which is non-CMOS compatible. He…

Materials Science

Elastic properties of ternary arsenide SrFe2As2 and quaternary oxyarsenide LaOFeAs as basic phases for new 38-55K superconductors from first principles

I. R. Shein、A. L. Ivanovskii2008-07-07arXiv

Here we report the first-principle FLAPW-GGA calculations of the elastic properties of two related phases, namely, the ternary arsenide SrFe2As2 and the quaternary oxyarsenide LaOFeAs as the basic phases for the newly discovered "1111" and "122" 38-52K superconductors. The independent elastic constants (Cij), bulk mod…

SuperconductivityMaterials Science

Overhauser frequency shifts in semiconductor nanostructures

I. Tifrea、M. Poggio、D. D. Awschalom 等 4 位作者2008-07-07arXiv

We calculate the Overhauser frequency shifts in semiconductor nanostructures resulting from the hyperfine interaction between nonequilibrium electronic spins and nuclear spins. The frequency shifts depend on the electronic local density of states and spin polarization as well as the electronic and nuclear spin relaxat…

Materials ScienceMesoscale and Nanoscale Physics

Size Dependence and Convergence of the Retrieval Parameters of Metamaterials

Jiangfeng Zhou、Thomas Koschny、Maria Kafesaki 等 4 位作者2008-07-07arXiv

We study the dependence of the retrieval parameters, such as the electric permittivity, the magnetic permeability and the index of refraction, $n$, on the size of the unit cell of a periodic metamaterial. The convergence of the retrieved parameters on the number of the unit cells is also examined. We have concentrated…

Materials Sciencecond-mat.other

Nano‐ and Micropatterning of Optically Transparent, Mechanically Robust, Biocompatible Silk Fibroin Films

Hannah Perry、Ashwin Gopinath、David L. Kaplan 等 5 位作者2008-07-07Advanced Materials

Regular nanometer-scale patterning down to a few tens of nanometers and the manufacturing of diffractive optical elements in silk by using the ideas of soft lithography is reported. The unique processing of silk films makes them an ideal substrate to incorporate biological matter (such as small organics, enzymes, prot…

Biochemical and Structural CharacterizationNanofabrication and Lithography TechniquesSilk-based biomaterials and applications

Electrochemical Modification of Graphene

Ravi S. Sundaram、Cristina Gómez‐Navarro、Kannan Balasubramanian 等 5 位作者2008-07-07OpenAlex

Nanoparticles on an atomic carpet: Individual graphene sheets have been decorated with metal nanoparticles through electrochemistry. The attachment of Pd particles onto graphene renders it sensitive to hydrogen. The controlled functionalization of graphene paves the way for various electronic applications.

Graphene and Nanomaterials ApplicationsGraphene research and applicationsAdvancements in Battery Materials

Dense Self‐Assembly on Sparse Chemical Patterns: Rectifying and Multiplying Lithographic Patterns Using Block Copolymers

Joy Cheng、Charles Rettner、Daniel P. Sanders 等 5 位作者2008-07-07OpenAlex

A lithography-friendly self-assembly process which multiplies and rectifies an existing resist patterns is demonstrated here. A polymer film (right figure) has assembled at a 14 nm half-pitch on a thin resist pattern at twice the period (left figure). This directed self-assembly process dramatically heals defects and…

Block Copolymer Self-AssemblyAdvanced Polymer Synthesis and CharacterizationNanofabrication and Lithography Techniques

Epitaxial-Graphene/Graphene-Oxide Junction: An Essential Step towards Epitaxial Graphene Electronics

Xiaosong Wu、Mike Sprinkle、Xuebin Li 等 6 位作者2008-07-07arXiv

Graphene-oxide (GO) flakes have been deposited to bridge the gap between two epitaxial-graphene electrodes to produce all-graphene devices. Electrical measurements indicate the presence of Schottky barriers at the graphene/graphene-oxide junctions, as a consequence of the band gap in GO. The barrier height is found to…

Carbon Nanotubes in CompositesMolecular Junctions and NanostructuresGraphene research and applications

Electromagnetic wave absorption properties of porous carbon/Co nanocomposites

Qinglei Liu、Di Zhang、Tongxiang Fan2008-07-07OpenAlex

Porous carbon/Co nanocomposites were fabricated by a sol-gel method. The electromagnetic parameters were measured in the 2–18GHz range. Compared with porous carbon composite, porous carbon/Co nanocomposite has larger dielectric loss due to the enhanced interfacial polarization relaxation loss and Ohmic loss. The maxim…

Electromagnetic wave absorption materialsAdvanced Antenna and Metasurface TechnologiesDielectric materials and actuators

Recent progress in carbon nanotube-based gas sensors

Ting Zhang、Syed Mubeen、Nosang V. Myung 等 4 位作者2008-07-07OpenAlex

The development of carbon nanotube-(CNTs-)based gas sensors and sensor arrays has attracted intensive research interest in the last several years because of their potential for the selective and rapid detection of various gaseous species by novel nanostructures integrated in miniature and low-power consuming electroni…

Gas Sensing Nanomaterials and SensorsCarbon Nanotubes in CompositesAnalytical Chemistry and Sensors

Pore Architecture of a Bovine Acellular Vocal Fold Scaffold

Chet C. Xu、Roger W. Chan2008-07-06Tissue Engineering Part A

An acellular xenogeneic scaffold derived from the bovine vocal fold lamina propria has shown some promise for in vitro vocal fold tissue engineering. To further explore the potential of the scaffold for cellular attachment, migration, and infiltration, as well as the transport of oxygen, proteins, and nutrients in viv…

Cellular and Composite StructuresTissue Engineering and Regenerative MedicineElectrospun Nanofibers in Biomedical Applications

Low voltage control of ferromagnetism in a semiconductor p-n junction

M. H. S. Owen、J. Wunderlich、V. Novak 等 11 位作者2008-07-06arXiv

The concept of low-voltage depletion and accumulation of electron charge in semiconductors, utilized in field-effect transistors (FETs), is one of the cornerstones of current information processing technologies. Spintronics which is based on manipulating the collective state of electron spins in a ferromagnet provides…

Materials Science

Enhanced Ferromagnetic Stability in Cu Doped Passivated GaN Nanowires

H. J. Xiang、Su-Huai Wei2008-07-06arXiv

Density functional calculations are performed to investigate the room temperature ferromagnetism in GaN:Cu nanowires (NWs). Our results indicate that two Cu dopants are most stable when they are near each other. Compared to bulk GaN:Cu, we find that magnetization and ferromagnetism in Cu doped NWs is strongly enhanced…

Materials Science

Comment on: Quantum interference of tunnel trajectories between states of different spin length in a dimeric molecular nanomagnet

W. Wernsdorfer2008-07-06arXiv

Ramsey et al. [Nature Phys. 4, 277-281 (2008)] report the observation of quantum interference associated with tunnelling trajectories between states of different total spin length in a dimeric molecular nanomagnet. They argue that the interference is a consequence of the unique characteristics of a molecular Mn12 whee…

Materials ScienceMesoscale and Nanoscale Physics

Intense Near‐IR Emission from Nanoscale Lanthanoid Fluoride Clusters

M.D. Romanelli、G.A. Kumar、Thomas J. Emge 等 5 位作者2008-07-05Angewandte Chemie

Fluoridcluster von Lanthanoiden werden durch Metathese von Ln(SePh)3 mit NH4F in organischen Lösungsmitteln erhalten. Die ersten Produkte dieser Reaktionen, [(py)24Ln28F68(SePh)16] (Ln=Pr, Nd; py=Pyridin; siehe Struktur), sind die größten diskreten Lanthanoidcluster, die bislang isoliert wurden. In Emissionsexperiment…

Inorganic Fluorides and Related CompoundsLuminescence Properties of Advanced MaterialsLanthanide and Transition Metal Complexes

Metal‐Enhanced 1270 nm Singlet Oxygen Phosphorescence

Rasmus Toftegaard、Jacob Arnbjerg、Kim Daasbjerg 等 7 位作者2008-07-05Angewandte Chemie

Ein Booster für die Singulettsauerstoffemission: Mithilfe speziell entwickelter Gold-Nanoscheiben kann einer der unwahrscheinlichsten natürlichen Übergänge – die Relaxation von Singulettsauerstoff unter Lichtemission – deutlich verstärkt werden. Der Grund hierfür sind Wechselwirkungen mit lokalisierten Oberflächenplas…

Nanoplatforms for cancer theranosticsAdvanced biosensing and bioanalysis techniquesGold and Silver Nanoparticles Synthesis and Applications

Promoting Effect of Coexisting H2O on the Activity of Ir/WO3/SiO2 Catalyst for the Selective Reduction of NO with CO

Masaaki Haneda、Hideaki Hamada2008-07-05Chemistry Letters

Abstract The catalytic activity of Ir/WO3/SiO2 for the selective reduction of NO with CO (CO-SCR) in the presence of excess O2 was significantly increased by the presence of coexisting H2O, whereas NO reduction hardly occurred in the absence of H2O. Coexisting H2O plays an important role preventing catalyst deactivati…

Gas Sensing Nanomaterials and SensorsGa2O3 and related materialsCatalytic Processes in Materials Science

Single‐Phase MnFe 2 O 4 Powders Obtained by the Polymerized Complex Method

Mónica Popa、P. Bruna、Daniel Crespo 等 4 位作者2008-07-05Journal of the American Ceramic Society

The present investigation reports on a simple technique for the preparation of single‐phase MnFe 2 O 4 nanocrystalline powders using the polymerized complex method, starting from manganese carbonate and iron nitrate. A mixed aqueous solution with citric acid, ethylene glycol, Fe, and Mn ions was polymerized. The phase…

Iron oxide chemistry and applicationsMagnetic Properties and Synthesis of FerritesMultiferroics and related materials

Applicability of Optical Scattering Model to β‐Quartz Solid Solution Glass–Ceramics with Nanoscale Crystalline Phase

Akihiko Sakamoto、Yusuke Himei、Tadashi Seto2008-07-05Journal of the American Ceramic Society

The applicability of Rayleigh‐Gans and quasi‐continuum scattering models to β‐quartz solid solution (s.s.) glass–ceramics was studied. We evaluated the validity of these models using two specimens with different microstructures. The refractive indices of the crystalline and glass phases of the specimens were calculate…

Glass properties and applications