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Noise spectroscopy of a quantum-classical environment with a diamond qubit

Santiago Hernández-Gómez、Francesco Poggiali、Paola Cappellaro 等 4 位作者2018-08-24DSpace@MIT (Massachusetts Institute of Technology)

Knowing a quantum system's environment is critical for its practical use as a quantum device. Qubit sensors can reconstruct the noise spectral density of a classical bath, provided long enough coherence time. Here we present a protocol that can unravel the characteristics of a more complex environment, comprising both…

Diamond and Carbon-based Materials ResearchForce Microscopy Techniques and ApplicationsAtomic and Subatomic Physics Research

Strain-induced variant selection in heterogeneous nucleation ofα-Ti at screw dislocations inβ-Ti

Max Poschmann、Joseph Lin、Henry Geerlings 等 5 位作者2018-08-24Physical Review Materials

Heterogeneous nucleation of the $\ensuremath{\alpha}$ to $\ensuremath{\beta}$ phase transition at ${\ensuremath{\langle}1\phantom{\rule{4pt}{0ex}}1\phantom{\rule{4pt}{0ex}}1\ensuremath{\rangle}}_{\ensuremath{\beta}}$-type screw dislocations in pure titanium is examined through a combination of elasticity theory and mo…

Microstructure and mechanical propertiesMetal and Thin Film MechanicsTitanium Alloys Microstructure and Properties

Fabrication and Thermal Insulation Properties of Bamboo‐Shaped Polymer Fibers by Selective Solvent Vapor Annealing

Yu‐Jing Chiu、H. C. Chiu、Hsiao‐Fan Tseng 等 7 位作者2018-08-24Macromolecular Rapid Communications

Fibrillar materials have gained much attention recently because of their unique properties and potential applications. Although many methods have been developed to fabricate materials, it remains challenging to prepare fibrillar materials containing multicomponent materials or even with complex structures. Here, a fac…

Advanced Sensor and Energy Harvesting MaterialsElectrospun Nanofibers in Biomedical ApplicationsPolymer composites and self-healing

Local distortion and octahedral tilting in BaCe x Ti1−x O3 perovskite

Giorgia Confalonieri、Vincenzo Buscaglia、Giancarlo Capitani 等 8 位作者2018-08-24Journal of Applied Crystallography

Ceramics with perovskite structure and composition BaCe x Ti 1− x O 3 ( x = 0.02–0.30) show a progressive evolution with increasing x , from the long-range polar order of ferroelectric BaTiO 3 to the short-range polar order typical of relaxors. The ionic size mismatch between Ti 4+ and Ce 4+ determines strong local st…

Ferroelectric and Piezoelectric MaterialsMultiferroics and related materialsMicrowave Dielectric Ceramics Synthesis

Exploring the Self-Assembly Capabilities of ABA-Type SBS, SIS, and Their Analogous Hydrogenated Copolymers onto Different Nanostructures Using Atomic Force Microscopy

Νικόλαος Πολιτάκος、Galder Kortaberría2018-08-24Materials

In this work, the self-assembled morphologies obtained for poly(styrene-b-butadiene-b-styrene) (SBS) and poly(styrene-b-isoprene-b-styrene) (SIS) ABA-type copolymers were investigated before and after hydrogenation of the polydiene block, which led to poly(styrene-b-ethylene)/poly(ethylene-b-styrene) (SEES) and poly(s…

Polymer Surface Interaction StudiesForce Microscopy Techniques and ApplicationsBlock Copolymer Self-Assembly

Polyoxometalates entrapped in sol-gel matrices as electron exchange columns and catalysts for the reductive de-halogenation of halo-organic acids in water

Neelam Neelam、Dan Meyerstein、Ariela Burg 等 5 位作者2018-08-24Journal of Coordination Chemistry

Halo-organic acids in aqueous solutions are widespread pollutants. An enormous number of technologies have been proposed for their elimination. In this context, reducing electron exchange columns seem to be an optimal solution for their degradation, as they do not introduce any new chemical into the solution to be pur…

Advanced oxidation water treatmentPolyoxometalates: Synthesis and ApplicationsEnvironmental remediation with nanomaterials

Effect of γ‐irradiation on optical properties of Eu2O3‐doped polystyrene polymer films

Shilpa Bhavsar、Gnansagar B. Patel、N. L. Singh2018-08-24Luminescence

Abstract In the present study, europium (III) oxide (Eu 2 O 3 )‐doped polystyrene (PS) polymer films were synthesized using a solution‐casting technique for different filler levels. These films were irradiated with 5, 25 and 50 kGy γ doses and characterized using various techniques, viz. X‐ray diffraction (XRD), and U…

Luminescence Properties of Advanced MaterialsLanthanide and Transition Metal ComplexesPolymer Nanocomposite Synthesis and Irradiation

Electrospun Three-Dimensional Nanofibrous Structure via Probe Arrays Inducing

Yifang Liu、Ruimin Liu、Xiang Wang 等 8 位作者2018-08-24Micromachines

The fast and precise direct-printing of micro three-dimensional (3D) structures is the important development trend for micro/nano fabrication technique. A novel method with probe arrays was built up to realize the controllable deposition of 3D electrospun nanofibrous structures. Firstly, several 3D nanofibrous structu…

Advanced Sensor and Energy Harvesting MaterialsElectrospun Nanofibers in Biomedical ApplicationsAdditive Manufacturing and 3D Printing Technologies

Biosynthesis, Characteristics and Antibacterial Activity of Silver Nanoparticles Using <i>Lemon Citrus Latifolia</i> Extract

Duong Huynh Thanh Linh、Nguyen Phung Anh、Truong Thi Ai Mi 等 9 位作者2018-08-24MATERIALS TRANSACTIONS

Silver nanoparticles (AgNPs) were synthesized from aqueous AgNO3 precursor via an effective and ecofriendly method using Lemon Citrus Latifolia (LCL) extract as the reducing and stabilizing agent under sunlight condition. The AgNPs formation was confirmed by ultraviolet-visible absorption spectroscopy at the wavelengt…

Nanoparticles: synthesis and applicationsGold and Silver Nanoparticles Synthesis and ApplicationsLaser-Ablation Synthesis of Nanoparticles

Multistep Development of the Hyperfine Fields in λ-(BEDT-STF)2FeCl4 Studied by Mössbauer Spectroscopy

Shuhei Fukuoka、Masashi Sawada、Takaaki Minamidate 等 10 位作者2018-08-24Journal of the Physical Society of Japan

We have investigated the magnetic properties of λ-(BEDT-STF)2FeCl4 by Mössbauer measurement to reveal the origin of the paramagnetic-like behavior of the 3d spin system observed in λ-(BETS)2FeCl4 using the donor substitution effect. We found that the temperature dependence of the hyperfine fields shows multistep devel…

Magnetism in coordination complexesOrganic and Molecular Conductors ResearchSolid-state spectroscopy and crystallography

Synthesis, Photophysical, Electrochemical Properties, DFT Studies and DSSC Performance of BODIPY Cored Triazole Bridged 3,6‐Ditertiary Butyl Carbazole Decorated Dendrimers

Janakiraman Babu、Ganesan Shanmugam、Masiyappan Karuppusamy 等 4 位作者2018-08-24ChemistrySelect

Abstract A series of BODIPY cored dendrimers up to second generation decorated with 3,6‐ditertiary butyl carbazole at the surface and triazole as the bridging unit has been achieved by convergent approach. The synthesised dendrimers show excellent photophysical and electrochemical properties. All the dendrimers exhibi…

Advanced biosensing and bioanalysis techniquesConducting polymers and applicationsLuminescence and Fluorescent Materials

ExcelAutomat 1.3: Fragment analysis based on the distortion/interaction‐activation strain model

Jalal Z. A. Laloo、Nandini Savoo、Nassirah Laloo 等 5 位作者2018-08-24Journal of Computational Chemistry

The distortion/interaction-activation strain model (D/I-ASM), a fragment analysis method, is applied to study the structure-reactivity relationship in reactions. The application of D/I-ASM involves the generation of input files for points along a reaction profile, submission of input files to a quantum software packag…

Computational Drug Discovery MethodsMolecular Junctions and NanostructuresMachine Learning in Materials Science

Protein Corona Formation on Magnetic Nanoparticles Conjugated with Luminescent Europium Complexes

Latif Ullah Khan、Romana Petry、Amauri J. Paula 等 5 位作者2018-08-24ChemNanoMat

Abstract The evaluation of the nanoparticles interactions with blood plasma enables a first and important insight on the organization of the adsorbed protein layer. In this context, we studied the formation of protein corona on magneto‐luminescent Fe 3 O 4 @calix‐Eu(TTA) nanoparticles in human plasma. The difference i…

Nanoparticle-Based Drug DeliveryLanthanide and Transition Metal ComplexesProtein Interaction Studies and Fluorescence Analysis

Mechanistic Models for Nanobeams with Surface Stress Effects

Yasothorn Sapsathiarn、R. K. N. D. Rajapakse2018-08-24Journal of Engineering Mechanics

In this paper, a mechanistic model for nanobeams with surface energy effects is developed by using a variational formulation. This work is motivated by the unusual response of nanocantilevers predicted by models based on the Young-Laplace equation for surface stress. The governing equation and boundary conditions deri…

Carbon Nanotubes in CompositesMechanical and Optical ResonatorsNonlocal and gradient elasticity in micro/nano structures

Quantum dot induced acute changes in lung mechanics are mouse strain dependent

David Scoville、Collin C. White、Dianne Botta 等 9 位作者2018-08-24Inhalation Toxicology

INTRODUCTION: Concerns have been raised regarding occupational exposure to engineered nanomaterials (ENMs). Potential impacts on lung function from inhalation exposures are of concern as the lung is a sensitive ENM target in animals. Epidemiological data suggest that occupational exposure to ENMs may impact respirator…

Nanoparticles: synthesis and applicationsAir Quality and Health ImpactsOccupational exposure and asthma

An innovative procedure for testing RTV and composite insulators sampled from service in search of diagnostic quantities

M. Marzinotto、Giovanni Mazzanti、E.A. Cherney 等 4 位作者2018-08-24IEEE Electrical Insulation Magazine

The proven reliability of ceramic cap-and-pin insulators for high voltage (HV) and extra-high voltage (EHV) overhead lines suffers in the presence of harsh industrial or strong salt pollution [1]. In these cases, apart from the countermeasures such as increasing creepage distance, washing, and applying greases, insula…

High voltage insulation and dielectric phenomenaLightning and Electromagnetic PhenomenaElectromagnetic Compatibility and Measurements

Influence of silica architecture on the catalytic activity of immobilized glucose oxidase

Gousia Begum、Cathleen Oschatz、Martin Oschatz 等 6 位作者2018-08-24Bioinspired Biomimetic and Nanobiomaterials

Immobilizing enzymes on solid support materials is of great interest for many applications as it improves enzyme lifetime and enables its recycling. Synthetic mesoporous silica materials are widely used as supports for enzyme immobilization due to their high enzyme-loading capacity and their excellent mass transport p…

Electrochemical sensors and biosensorsEnzyme Catalysis and ImmobilizationMesoporous Materials and Catalysis

Highly Sensitive Colorimetric Detection of Early Stage Aluminum Corrosion in Water Using Plasmonic Gold Nanoparticle Films

Alexander B. Tesler、Takumi Sannomiya、Alexander Vaskevich 等 5 位作者2018-08-24Advanced Optical Materials

Abstract Corrosion remains the major reason for the failure of metallic parts. Therefore, spotting and evaluating the severity of corrosion at its early stages is of great importance. Herein, a novel optical corrosion probe based on plasmonic gold nanoparticles immobilized on aluminum surface is demonstrated. The meas…

Gold and Silver Nanoparticles Synthesis and ApplicationsAdvanced biosensing and bioanalysis techniquesNanoplatforms for cancer theranostics

Pressure–Temperature Phase Diagrams and Transition Mechanisms of Hybrid Organic–Inorganic NH···N Bonded Ferroelectrics

Anna Olejniczak、Marek Szafrański、Andrzej Katrusiak2018-08-24Crystal Growth & Design

The ferroelectric–paraelectric transitions of 1,4-diazabicyclo[2.2.2]octane (dabco) tetrafluoroborate (dabcoHBF 4 ) and perchlorate (dabcoHClO 4 ), between their phases II (orthorhombic space group Pm 2 1 n ) and I (tetragonal space group P 4/ nmm ) proceed at T C = 377 and 378 K, respectively. On approaching phase I…

Crystallography and molecular interactionsSolid-state spectroscopy and crystallographyInorganic Fluorides and Related Compounds

Statistical adhesion strength of an amorphous polymer–its miscible blend interface self-healed at a temperature below the bulk glass transition temperature

Yuri M. Boiko2018-08-24The Journal of Adhesion

The distribution of the lap-shear strength developed at an amorphous asymmetric compatible interface between the contacting thick (bulk) films of entangled polystyrene (PS) with its miscible blend with poly(2,6-dimethyl-1,4-phenylene oxide) (PPO) (75 wt.% PS and 25 wt.% PPO) at a constant healing temperature (T) of 90…

Polymer crystallization and propertiesPolymer Nanocomposites and PropertiesPolymer composites and self-healing