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Photo-orientation of mesoporous silica materials via transfer from an azobenzene-containing polymer monolayerElectronic supplementary information (ESI) available: details on the experimental procedures and IR spectra around the siloxane stretching band. See http://www.rsc.org/suppdata/jm/b3/b310296c/

Yasuhiro Kawashima、Masaru Nakagawa、Kunihiro Ichimura 等 4 位作者2004-01-01Journal of Materials Chemistry

Successful photo-orientation of mesostructured surfactant/silica hybrids is performed via hierarchically relayed multiple transfers among hetero-interfaces. A Langmuir–Blodgett monolayer of the azobenzene-containing polymer was first optically oriented via irradiation with linearly polarized light, and the photoinduce…

Photonic Crystals and ApplicationsMesoporous Materials and CatalysisElectrowetting and Microfluidic Technologies

Dianionic and trianionic macrocycles in cobalt N-confused porphyrin complexesElectronic supplementary information (ESI) available: Absorption spectra for 1, 2 and 4. See http://www.rsc.org/suppdata/cc/b4/b404261a/

John D. Harvey、Christopher J. Ziegler2004-01-01Chemical Communications

We report the syntheses of cobalt N-confused porphyrins; this work completes the series of the late first-row transition metals that have been incorporated into the core of N-confused porphyrin, and in these compounds the macrocycles can act as either a -2 or -3 anion.

Magnetism in coordination complexesPorphyrin and Phthalocyanine ChemistryMetal-Catalyzed Oxygenation Mechanisms

Monitoring photoswitching of azobenzene-based self-assembled monolayers on ultrathin platinum films by UV/Vis spectroscopy in the transmission modeElectronic supplementary information (ESI) available: synthesis and characterization of 1 and its photoisomerization in solution. See http://www.rsc.org/suppdata/jm/b3/b314710j/

Salvatore Sortino、Salvatore Petralia、Sabrina Conoci 等 4 位作者2004-01-01Journal of Materials Chemistry

The reversible trans ↔ cis photoisomerization of azobenzene-based self-assembled monolayers on ultrathin platinum films has been monitored for the first time by UV-Vis transmission spectroscopy with a conventional spectrophotometer.

Molecular Junctions and NanostructuresPhotochromic and Fluorescence ChemistryPhotoreceptor and optogenetics research

Formation of Mn 3 O 4 nanoparticles from the cluster [Mn 12 O 12 (C 2 H 5 COO) 16 (H 2 O) 3 ] anchored to hybrid mesoporous silica

Benjamin Folch、Joulia Larionova≠、Yannick Guari≠ 等 6 位作者2004-01-01Journal of Materials Chemistry

A new approach to the synthesis and the organization of Mn3O4 (hausmannite) nanoparticles has been developed using the thermolysis of the magnetic cluster [Mn12O12(C2H5COO)16(H2O)3] linked to a SBA-15 mesoporous silica functionalized with –COOH groups. The obtained composites were studied by X-Ray diffraction (XRD), i…

Magnetism in coordination complexesMesoporous Materials and CatalysisPolyoxometalates: Synthesis and Applications

Swelled plastics in supercritical CO2 as media for stabilization of metal nanoparticles and for catalytic hydrogenation

Hiroyuki Ohde、Mariko Ohde、Chien M. Wai2004-01-01Chemical Communications

Swelled plastics in supercritical carbon dioxide provide unique environments for stabilizing palladium and rhodium nanoparticles and for catalytic hydrogenation. Complete hydrogenation of benzene to cyclohexane can be achieved in 10 minutes using the plastic stabilized Rh nanoparticles at 50 degrees C in supercritical…

Catalytic Processes in Materials SciencePhase Equilibria and ThermodynamicsCarbon dioxide utilization in catalysis

Synthesis of unsymmetrical dibenzoquinoxaline discotic mesogensElectronic supplementary information (ESI) available: full synthetic and analytical details, POM images. See http://www.rsc.org/suppdata/cc/b4/b400998c/

E. Johan Foster、Jarret Babuin、Natalie Nguyen 等 4 位作者2004-01-01Chemical Communications

Unsymmetrical dibenzophenazine discotic mesogens were prepared via the corresponding tetraalkoxybenzil derivatives. These dibenzophenazines exhibit Colho phases over extremely broad temperature ranges.

Liquid Crystal Research AdvancementsOrganic Light-Emitting Diodes ResearchNonlinear Optical Materials Research

Plasma polymer chemical gradients for evaluation of surface reactivity: epoxide reaction with carboxylic acid surface groups

Morgan R. Alexander、Jason D. Whittle、David Barton 等 4 位作者2004-01-01Journal of Materials Chemistry

Organic surfaces of specific chemistry can be fabricated using plasma polymerisation. A recently developed deposition approach allows gradients in surface carboxyl group concentration to be fabricated over a distance of 13 mm from a mixed acrylic acid/octadiene plasma. The utility of these surfaces in the investigatio…

Surface Modification and SuperhydrophobicityDiamond and Carbon-based Materials ResearchAnalytical Chemistry and Sensors

High Resolution X-ray Structure of dTDP-Glucose 4,6-Dehydratase from Streptomyces venezuelae

S.T.M. Allard、W. W. Cleland、Hazel M. Holden2004-01-01Journal of Biological Chemistry

Desosamine is a 3-(dimethylamino)-3,4,6-trideoxyhexose found in some macrolide antibiotics. In Streptomyces venezuelae, there are seven genes required for the biosynthesis of this unusual sugar. One of the genes, desIV, codes for a dTDP-glucose 4,6-dehydratase, which is referred to as DesIV. The reaction mechanisms fo…

Protein Structure and DynamicsEnzyme Structure and FunctionBiochemical and Molecular Research

Semiconductive Properties of Passive Films Formed on Fe-18Cr in Borate Buffer Solution

Hiroaki Tsuchiya、Shinji Fujimoto、Toshio Shibata2004-01-01Journal of The Electrochemical Society

Passive films formed on Fe-18Cr alloy in a borate buffer solution were studied using impedance spectroscopy and photoelectrochemical response. The passive film was composed of an inner oxide and covering hydroxide layer. Both layers exhibited n-type semiconductor properties with an optical bandgap energy, E g , of 3.4…

Corrosion Behavior and InhibitionHigh-Temperature Coating BehaviorsHydrogen embrittlement and corrosion behaviors in metals

Water soluble star block poly(oxazoline) with porphyrin label: a unique emulsion and its shape direction

Ren‐Hua Jin2004-01-01Journal of Materials Chemistry

Water soluble star polymers consisting of a porphyrin center and four poly(oxazolines) arms such as Por-[poly(methyloxazoline)]4 (1), Por-[poly(ethyloxazoline)]4 (2), Por-[poly(methyloxazoline-co-ethyloxazoline)]4 (3) and Por-[poly(methyloxazoline)-b-poly(ethyloxazoline)]4 (4) were synthesized and used for the investi…

Supramolecular Chemistry and ComplexesPorphyrin and Phthalocyanine ChemistryCovalent Organic Framework Applications

Density, Surface Tension, and Viscosity of PbO‐B 2 O 3 ‐SiO 2 Glass Melts

Shigeru Fujino、Chawon Hwang、Kenji Morinaga2004-01-01Journal of the American Ceramic Society

The density, surface tension, and viscosity of the melts from the PbO‐B 2 O 3 ‐SiO 2 system have been measured at temperatures in the range 1073–1473 K. The effect of composition on these properties was also investigated. The density of the melt was found to increase linearly with increasing PbO content. Molar volume…

Glass properties and applicationsMetallurgical Processes and ThermodynamicsMaterials Engineering and Processing

The effect of alloying elements on the crystallization behaviour and on the properties of galvanized coatings

G. Vourlias、N. Pistofidis、G. Stergioudis 等 4 位作者2004-01-01Crystal Research and Technology

Abstract The influence of the alloying elements on the interface reactions of zinc coatings during the galvanization process was examined. These reactions affect the crystallization and the structure and properties of the outer layer of the coatings. Depending on the type and concentration of the alloying additions in…

Corrosion Behavior and InhibitionHydrogen embrittlement and corrosion behaviors in metalsConcrete Corrosion and Durability

Self-Standing Porous Silicon Films by One-Step Anodizing

Chetan Singh Solanki、R. Bilyalov、J. Poortmans 等 6 位作者2004-01-01Journal of The Electrochemical Society

A novel technique for the formation and lift-off of thin porous silicon films from starting substrates in a single step by electrochemical etching in hydrofluoric acid-based solutions is described. Lift-off or separation of porous silicon (PS) film occurs under specific sets of current density and HF concentration, wh…

Semiconductor materials and devicesSilicon Nanostructures and PhotoluminescenceNanowire Synthesis and Applications

Hierachically porous nanocrystalline cobalt oxide monoliths through nanocasting

Jan‐Henrik Smått、Bernd Spliethoff、Jarl B. Rosenholm 等 4 位作者2004-01-01Chemical Communications

Nanocrystalline cobalt oxide, Co(3)O(4), monoliths exhibiting hierarchical bimoidal porosity have been prepared by nanocasting of porous silica monoliths.

Catalytic Processes in Materials ScienceMesoporous Materials and CatalysisNanoporous metals and alloys

Mechanical properties of plasma-treated sisal fibre-reinforced polypropylene composites

Xiaowen Yuan、Krishnan Jayaraman、Debes Bhattacharyya2004-01-01Journal of Adhesion Science and Technology

In recent years, sisal fibres have become a promising reinforcement for composites because of their low cost, low density, high specific strength, high specific modulus, easy availability and renewability. However, the poor adhesion between the hydrophilic sisal fibre and the hydrophobic thermoplastic matrices has adv…

Natural Fiber Reinforced CompositesTribology and Wear AnalysisMechanical Engineering and Vibrations Research

Remarkable thermodynamic stability toward hydrolysis of tripodal titanium alkoxidesElectronic supplementary information (ESI) available: syntheses and spectroscopic characterization of new compounds. See http://www.rsc.org/suppdata/cc/b3/b315092e/

V. Ugrinova、Gregory A. Ellis、Seth N. Brown2004-01-01Chemical Communications

The monomeric titanium(IV) hydroxide complex, LTi(OH)(LH(3)= tris(2-hydroxy-3,5-di-tert-butylbenzyl)amine), which is sterically inhibited from condensation to a mu-oxo dimer, cannot be prepared by hydrolysis of the alkoxide, with K(eq)= 0.012 for hydrolysis of the titanium methoxide in THF.

Radioactive element chemistry and processingPolyoxometalates: Synthesis and ApplicationsChemical Synthesis and Reactions

Effect of Sintering Temperature on Dielectric Properties of Pb(Fe1/2Nb1/2)O3Perovskite Material

K. Singh、S. A. Band、W. K. KINGE2004-01-01Ferroelectrics

Lead iron niobate [Pb(Fel/2Nb1/2)]O3 (PFN) are synthesized by using precursor method. Three different sintering temperatures (1000, 1040 and 1100°C) are selected to optimize the PFN processing technique. X-ray powder diffraction studies confirm the formation of single-phase perovskite PFN. The scanning electron micros…

Ferroelectric and Piezoelectric MaterialsMicrowave Dielectric Ceramics SynthesisDielectric properties of ceramics

High-frequency electron paramagnetic resonance investigation of the Fe3+ impurity center in polycrystalline PbTiO3 in its ferroelectric phase

Hrvoje Meštrić、Rüdiger‐A. Eichel、Dinse, Klaus-Peter 等 6 位作者2004-01-01TUbilio (Technical University of Darmstadt)

The intrinsic iron(III) impurity center in polycrystalline lead titanate was investigated by means of high-frequency electron paramagnetic resonance (EPR) spectroscopy in order to determine the local-environment sensitive fine structure parameter D. At a spectrometer frequency of 190 GHz, spectral analysis of a powder…

Ferroelectric and Piezoelectric MaterialsSolid-state spectroscopy and crystallographyMicrowave Dielectric Ceramics Synthesis

Nanoassemblies formed from hydrophilic block copolymers and multivalent ions

Nicolas Sanson、Frédéric Bouyer、Corine Gérardin 等 4 位作者2004-01-01Physical Chemistry Chemical Physics

We recently reported on the controlled formation of highly stable metal hydroxide nanoparticles. Growth control and stabilization of particles were achieved by performing hydrolysis and polycondensation reactions of polymer-complexed metal cations, the polymers being double hydrophilic block copolymers (DHBCs). The pr…

Advanced Polymer Synthesis and CharacterizationPolymer Surface Interaction StudiesElectrostatics and Colloid Interactions