Materials Literature
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The observation of a high-mobility two-dimensional electron gas between two insulating complex oxides, especially LaAlO3/SrTiO3, has enhanced the potential of oxides for electronics. The occurrence of this conductivity is believed to be driven by polarization discontinuity, leading to an electronic reconstruction. In…
In this paper we use a Terahertz (THz) time-domain system to image and analize the structure of an artwork attributed to Spanish artist Goya painted in 1771. The Thz images show features that cannot be seen in the optical or X-ray images that providence evidence of its authenticity, which is validated by other indepen…
In this study, an analytical solution is presented for thermo-electro-elastic analysis of piezoelectric semi-infinite bodies. For this purpose, governing equations are derived for a transversely isotropic piezoelectric material under axisymmetric thermo-electro-mechanical loading condition. A general closed form analy…
In this paper, strain gradient elasticity formulation for analysis of FG (Functionally Graded) micro-cylinders is presented. The material properties are assumed to obey a power law in radial direction. The governing differential equation is derived as a fourth order ODE. A power series solution for stresses and displa…
The development of automated high-intensity macromolecular crystallography (MX) beamlines at synchrotron facilities has resulted in a remarkable increase in sample throughput. Developments in X-ray detector technology now mean that complete X-ray diffraction datasets can be collected in less than one minute. Such high…
Spiropyran (SP) mechanophore was synthesized into the soft or hard phase of segmented polyurethanes (SPU) and used as a molecular probe of force and orientation. Upon either tensile stretching or irradiation with UV light the SP-linked segmented polyurethane (SP-SPU) adopt a deep purple coloration and are fluorescent,…
We report on the introduction of a systematic method for the quantitative and reliable characterization of covalently functionalized graphene based on Scanning-Raman-Microscopy (SRM). This allows for recording and analyzing several thousands of Raman spectra per sample and straightforward display of various Raman prop…
Two-dimensional atomic sheets of graphene represent a new class of nanoscale materials with potential applications in electronics. However, exploiting the intrinsic characteristics of graphene devices has been problematic due to impurities and disorder in the surrounding dielectric and graphene/dielectric interfaces.…
The aberration-corrected scanning transmission electron microscope has great sensitivity to environmental or instrumental disturbances such as acoustic, mechanical, or electromagnetic interference. This interference can introduce distortions to the images recorded and degrade both signal noise and resolution performan…
The study of the chemical and biological properties of CeO2 nanoparticles (CNPs) has expanded recently due to its therapeutic potential, and the methods used to synthesize these materials are diverse. Moreover, conflicting reports exist regarding the toxicity of CNPs. To help resolve these discrepancies, we must first…
We present an atomistic study of the behavior and interactions of hydrogen and vacancies in body centered cubic (bcc) iron, using both ab initio and classical molecular dynamics methods. Hydrogen causes damage to materials through embrittlement, hardening, and swelling; we investigate the role of vacancies in these pr…
Radioactive counterions were used to track the ratio of positive to negative polymer repeat units within a polyelectrolyte multilayer made from poly(diallyldimethylammonium chloride), PDADMAC, and poly(styrene sulfonate), PSS. For this widely employed pair of "linearly" assembled polyelectrolytes it was found that the…
We report a controllable wet method for effective decoration of 2-dimensional (2D) molybdenum disulfide (MoS2) layers with Au nanoparticles (NPs). Au NPs can be selectively formed on the edge sites or defective sites of MoS2 layers. The Au-MoS2 nano-composites are formed by non-covalent bond. The size distribution, mo…
By applying the optical nanocircuit concepts to metasurfaces, we propose an effective route to locally control light transmission over a deeply subwavelength scale. This concept realizes the optical equivalent of a transmit-array, whose use is demonstrated for light bending and focusing with unprecedented efficiency o…
In recent years the outbreak of re-emerging and emerging infectious diseases has been a significant burden on global economies and public health. The growth of population and urbanization along with poor water supply and environmental hygiene are the main reasons for the increase in outbreak of infectious pathogens. T…
Two new steroidal glycosides, 1α,3α-dihydroxy-5β-pregn-16-en-20-one 3-O-α-L-rhamnopyranoside (1) and 1β,3β,27-trihydroxycholest-16-en-22-one 1,3-di-O-α-L-rhamnoside (2), along with seven known steroidal glycosides (3-9), were isolated from Reineckia carnea herba. Their structures were determined by detailed analysis o…
The atomic step edges on a transition-metal (TM) surface play an important role in surface catalysis due to their distinct reactivities from that of the terrace. The nonuniform growth of graphene on Ni(111) is just such a case. Using first-principles calculations, we show that the step edges of Ni(111) can be passivat…
We report strongly modified optical emission of InAs/InP quantum dots (QDs) coupled to the surface plasmon resonance (SPR) of In nanoparticles grown by metal-organic vapor phase epitaxy. With increasing In deposition time, the In nanoparticle size increases and the SPR redshifts significantly. When overlapping with th…
We fabricate free-standing graphene structures from epitaxial graphene on silicon carbide using a photoelectrochemical (PEC) etching process. A combination of Raman spectroscopy and magnetotransport measurements was used to investigate multiterminal devices in various geometries. From the analysis of Raman data and Sh…
A rigorous definition of the concept of pseudo-symmetry, which is as important to chemistry as the concepts of symmetry implemented through group theory, should allow us to apply those group theoretical tools to molecules that are significantly distorted from those ideal symmetries best known and understood by the che…