Materials Literature
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The synthesis and characterization of a family of Mn(2)(III)Mn(2)(II)Ln(III)(2) complexes (Ln = Gd (1), Tb (2), Dy (3), and Ho (4)) of formula [Mn(4)Ln(2)O(2)(O(2)CBu(t))(6)(edteH(2))(2)(NO(3))(2)] are reported, where edteH(4) is N,N,N',N'-tetrakis(2-hydroxyethyl)ethylenediamine. The analogous Mn(4)Y(2) (5) complex ha…
We present a compact physics-based model of the current-voltage characteristics of graphene field-effect transistors, of especial interest for analog and RF applications where band-gap engineering of graphene could be not needed. The physical framework is a field-effect model and drift-diffusion carrier transport. Exp…
The cyclization reaction of the photochromic diarylethene derivative 1,2-bis(2,4-dimethyl-5-phenyl-3-thienyl)perfluorocyclopentene was studied in its single crystal phase with femtosecond transient absorption spectroscopy. The transient absorption measurements were performed with a robust acquisition scheme that expli…
Magnetism is very important in various areas of science and technology, ranging from magnetic recording through energy generation to trapping cold atoms. Physicists have managed to master magnetism—to create and manipulate magnetic fields—almost at will. Surprisingly, there is at least one property that has been elusi…
We report a Fe K$\ensuremath{\beta}$ x-ray emission spectroscopy study of local magnetic moments in various iron-based superconductors in their paramagnetic phases. Local magnetic moments are found in all samples studied: PrFeAsO, $\mathrm{Ba}{(\mathrm{Fe},\mathrm{Co})}_{2}{\mathrm{As}}_{2}$, LiFeAs, Fe${}_{1+x}$(Te,S…
The magnetic properties and transition from an antiferromagnetic (AFM) to a ferromagnetic (FM) state in semi-Heusler alloys Cu${}_{1\ensuremath{-}x}$Ni${}_{x}$MnSb, with x 0.3 have been investigated in detail by dc magnetization, neutron diffraction, and neutron depolarization. We observe that for x 0.05, the system C…
The classical modeling of dislocation climb based on a continuous description of vacancy diffusion is compared to recent atomistic simulations of dislocation climb in body-centered cubic iron under vacancy supersaturation [Phys. Rev. Lett. 105, 095501 (2010)]. A quantitative agreement is obtained, showing the ability…
The atomic interaction and magnetic properties of ultrathin Fe films grown on cleaved and polished MgO(100) surfaces were studied by conversion electron Mössbauer spectroscopy (CEMS) in broad temperature range. Fe with different layer thickness was deposited on MgO substrates. The layers were formed on polished and cl…
The deposition of thin SiO$_x$C$_y$H$_z$ or SiO$_x$H$_y$ films by means of atmospheric pressure microplasma jets with admixture of Hexamethyldisiloxane (HMDSO) and oxygen and the role of surface reactions in film growth are investigated. Two types of microplasma jets, one with a planar electrodes and operated in heliu…
Reflected neutron beam originating from a crystal monochromator contains higher order wavelength contribution. Creating multilayer mirror structures with custom reflectivity curves including a monochromatic polarized neutron beam is a challenge in modern neutron optics. In this work we present the study of three types…
The association of ions in electrolyte solutions at very low concentration and low temperature is studied using computer simulations and quasi-chemical ion-pairing theory. The specific case of the restricted primitive model (charged hard spheres) is considered. Specialised simulation techniques are employed that lead…
Fe and 2Si were co-deposited on Si (111) surface at 853 K. The formation of silicides was investigated by Mossbauer spectroscopy and electron microscopy. Depending on the thickness of the deposited films different phases were formed. At low thickness, stable $ε$-FeSi (B20) and metastable [CsCl]-Fe$_{1-x}$Si (B2) phase…
L10 (CuAu(I)-type) ordered FePd as well as FePt and CoPt, due to their high magnetic anisotropy, are candidate materials for future ultra-high density magnetic recording. Atomic diffusion governs the structural relaxation and associated changes in the physical and magnetic properties in these alloys. Such processes in…
The continuous need towards improving the capacity of magnetic storage devices requires materials with strong perpendicular magnetic anisotropy. FePd, CoPd and their Co(Fe)Pt counterparts very attractive candidate for such purposes. The magnetic properties of these films are largely dependent on the orientation and lo…
Adsorption, diffusion, and dissociation of CO(2) on the anatase (101) surface were investigated using dispersion-corrected density functional theory. On the oxidized surface several different local minima were identified of which the most stable corresponds to a CO(2) molecule adsorbed at a five-fold coordinated Ti si…
Measurements of London penetration depth are a sensitive tool to study multi-band superconductivity and it has provided several important insights to the behavior of Fe-based superconductors. We first briefly review the "experimentalist - friendly" self-consistent Eilenberger model that relates the measurable superflu…
The possibility of utilizing the Si and Ge nanostructures to promote surface-enhanced Raman scattering (SERS) is discussed. The vibronic coupling of the conduction band and valence band states of Si or Ge with the excited and ground states of the target molecule during the charge transfer (CT) process could enhance th…
For the first time, 3-dimensional luminescence spectra (luminescence intensity as a function of the excitation and emission wavelengths) have been obtained for bismuth-doped optical fibers of various compositions in a wide spectral range (450-1700 nm). The bismuth-doped fibers investigated have the following core comp…
The parent phases of the Fe-arsenide superconductors harbor an antiferromagnetic ground state. Significantly, the Néel transition is either preceded or accompanied by a structural transition that breaks the four-fold symmetry of the high-temperature lattice. Borrowing language from the field of soft condensed matter p…
Abstract A novel OA/ionic liquid two‐phase system combining the merits of thermal decomposition method, the IL‐based strategy, and the two‐phase approach is introduced to synthesize high‐quality lanthanide‐doped NaGdF 4 upconversion nanocrystals with different crystal‐phases in OA‐phase and IL‐phase through a one‐step…