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Ligand Design for Heterobimetallic Single‐Chain Magnets: Synthesis, Crystal Structures, and Magnetic Properties of MIICuII (M=Mn, Co) Chains with Sterically Hindered Methyl‐Substituted Phenyloxamate Bridging Ligands

Emilio Pardo、Rafael Ruiz‐García、Francesc Lloret 等 9 位作者2006-12-05Chemistry - A European Journal

Two new series of neutral oxamato-bridged heterobimetallic chains of general formula [MCu(L(x))(2)] m DMSO (m=0-4) (L(1)=N-2-methylphenyloxamate, M=Mn (1 a) and Co (1 b); L(2)=N-2,6-dimethylphenyloxamate, M=Mn (2 a) and Co (2 b); L(3)=N-2,4,6-trimethylphenyloxamate, M=Mn (3 a) and Co (3 b)) have been prepared by react…

Magnetism in coordination complexesPorphyrin and Phthalocyanine ChemistryLanthanide and Transition Metal Complexes

Ordered Mesoporous Copper Oxide with Crystalline Walls

Xiaoyong Lai、Xiaotian Li、Wangchang Geng 等 6 位作者2006-12-05Angewandte Chemie International Edition

Order, order: Mesoporous copper oxide was synthesized for the first time by double replication from ordered mesoporous silica SBA-15 via the ordered mesoporous carbon intermediate CMK-3 (see picture). The new material has potentially exciting applications in catalysis or lithium-ion batteries.

Catalytic Processes in Materials ScienceMesoporous Materials and CatalysisCopper-based nanomaterials and applications

Hexagon-preserving carbon foams: Properties of hypothetical carbon allotropes

Agnieszka Kuc、Gotthard Seifert2006-12-05Physical Review B

Carbon foams are hypothetical carbon allotropes that contain graphitelike ($s{p}^{2}$ carbon) segments, connected by $s{p}^{3}$ carbon atoms, resulting in porous structures. In this work the density-functional-based tight-binding method with periodic boundary conditions was employed to study the energetics, the stabil…

Carbon Nanotubes in CompositesGraphene research and applicationsBoron and Carbon Nanomaterials Research

Effect of Nanotube Functionalization on the Coefficient of Thermal Expansion of Nanocomposites

Shiren Wang、Zhiyong Liang、Philippe Gonnet 等 6 位作者2006-12-05Advanced Functional Materials

Abstract Single‐walled carbon nanotubes (SWNTs) are functionalized through both covalent and noncovalent bonding approaches to enhance dispersion and interfacial bonding. The coefficient of thermal expansion (CTE) of the functionalized‐SWNT‐reinforced epoxy composites are measured with a thermal mechanical analyzer (T…

Carbon Nanotubes in CompositesPolymer Nanocomposites and PropertiesThermal properties of materials

Dynamics of Spontaneous Magnetization Reversal in Exchange Biased Heterostructures

Zhi-Pan Li、Casey W. Miller、Igor V. Roshchin 等 4 位作者2006-12-05arXiv

The dependence of thermally induced spontaneous magnetization reversal on time-dependent cooling protocols was studied. Slower cooling and longer waiting close to the Nèel temperature of the antiferromagnet ($T_N$) enhances the magnetization reversal. Cycling the temperature around $T_N$ leads to a thermal training ef…

Materials Science

Controlled-Synthesis, Self-Assembly Behavior, and Surface-Dependent Optical Properties of High-Quality Rare-Earth Oxide Nanocrystals

Rui Si、Ya‐Wen Zhang、Huanping Zhou 等 5 位作者2006-12-05Chemistry of Materials

Single-crystalline and monodisperse cubic rare-earth (RE = La to Lu, Y) oxide nanocrystals (ultrathin nanoplates and nanodisks) have been synthesized via a nonhydrolytic approach in oleic acid (OA)/oleylamine (OM)/1-octadecene (ODE) using various rare-earth complexes, including acetylacetonate, benzoylacetonate, and a…

Luminescence Properties of Advanced MaterialsPerovskite Materials and ApplicationsQuantum Dots Synthesis And Properties

Electrochemical Study of High Electrochemical Double Layer Capacitance of Ordered Porous Carbons with Both Meso/Macropores and Micropores

Hirotoshi Yamada、Haruka Nakamura、Fumihiro Nakahara 等 5 位作者2006-12-05The Journal of Physical Chemistry C

Porous carbons with large meso/macropore surface areas were prepared by the colloidal-crystal-templating technique. The porous carbons exibited extremely high specific electrochemical double layer (EDL) capacitance of 200−350 F g -1 in an aqueous electrolyte (1 M H 2 SO 4 ). The pore structure dependence of the capaci…

Electrocatalysts for Energy ConversionSupercapacitor Materials and FabricationConducting polymers and applications

Microstructure of strained La2CuO4+delta thin films on varied sub-strates

Jiaqing He、Robert F. Klie、Gennady Logvenov 等 5 位作者2006-12-05arXiv

Layered perovskite La2CuO4+delta(LCO) thin films were epitaxially grown on SrTiO3 (STO) and LaSrAlO4 (LSAO) substrates by atomic-layer-by-layer molecular beam epitaxy. The lattice de-fects and residual strain in these films were investigated by means of transmission electron mi-croscopy and electron energy loss spectr…

Materials Science

Tunable Wettability by Clicking Counterions Into Polyelectrolyte Brushes

Omar Azzaroni、A. A. Brown、Wilhelm T. S. Huck2006-12-05Advanced Materials

Abstract Polymer brushes have recently emerged as an extremely versatile way to modify surface properties in a robust and controlled way. The introduction of responsive polymers and block copolymers in polymer‐brush systems has also opened up new routes to ‘smart' surfaces with switchable surface properties. Here, the…

Advanced Polymer Synthesis and CharacterizationPolymer Surface Interaction StudiesAdhesion, Friction, and Surface Interactions

Layer-by-layer assembly: from conventional to unconventional methods

Xi Zhang、Huan Chen、Hongyu Zhang2006-12-05OpenAlex

Layer-by-layer (LbL) assembly is a powerful means for fabricating multilayer thin films with controlled architecture and composition. This feature article discusses different types of methods for LbL assembly. On the one hand, some of the conventional LbL methods are introduced, which are driven by electrostatic inter…

Polymer Surface Interaction StudiesMolecular Junctions and NanostructuresNanofabrication and Lithography Techniques

Twenty Years of Polymer‐Clay Nanocomposites

Akane Okada、Arimitsu Usuki2006-12-05OpenAlex

Abstract Summary: More than twenty years have passed since we invented PCN, in which only a few wt.‐% of silicate is randomly and homogeneously dispersed in the polymer matrix. When molded, these nanocomposites show superior properties compared to those of pristine polymers. The number of papers on PCN has increased r…

Polymer Nanocomposites and PropertiesFlame retardant materials and propertiesSynthesis and properties of polymers

Kinetics of Two-Phase Electrocrystallization Processes

M. Y. Abyaneh2006-12-04Journal of The Electrochemical Society

In this paper, current-time transient (CTT) forms associated with the two remaining models of two-phase growth are identified. The first model represents a scenario in which growth centers associated with the phase with the higher outward growth rate are conically shaped, while the shape of the remaining growth center…

Electrodeposition and Electroless CoatingsCrystallization and Solubility Studiesnanoparticles nucleation surface interactions

Synthesis and Characterization of Glasses as an Electrolyte for Low-Temperature H[sub 2]∕O[sub 2] Fuel Cells

T. Uma、Masayuki Nogami2006-12-04Journal of The Electrochemical Society

This study is an attempt to prepare proton-conducting glasses based on heteropolyacids for the fuel cell application. The phosphomolybdic acid (PMA)-containing glass membranes were characterized by thermogravimetry/differential thermal analysis, -adsorption-desorption analysis, and impedance measurements. Thermogravim…

Advanced Battery Materials and TechnologiesConducting polymers and applicationsPolyoxometalates: Synthesis and Applications

Synthesis and properties of novel poly(arylene ether)s and poly(arylene thioether)s based on a pyridazine biphenol or a phthalazine biphenol

Jing Xu、Yuezhong Meng、Shuanjin Wang 等 4 位作者2006-12-04Journal of Polymer Science Part A Polymer Chemistry

Abstract Novel sulfur‐containing biphenol monomers were prepared in high yields by the reaction of 4‐mercaptophenol with chloropyridazine or chlorophthalazine compounds. High‐molecular‐weight poly(arylene ether)s were synthesized by a nucleophilic substitution reaction between these sulfur‐containing monomers and acti…

Synthesis and characterization of novel inorganic/organometallic compoundsSynthesis and properties of polymersSilicone and Siloxane Chemistry

Low threshold amplified spontaneous emission based on coumarin 151 encapsulated in mesoporous SBA-15

Dingke Zhang、Sumei Zhang、Dongge Ma 等 5 位作者2006-12-04Applied Physics Letters

Amplified spontaneous emission (ASE) characteristics of a blue dye coumarin 151 encapsulated in a highly ordered mesoporous SBA-15 were studied. The spectra narrowing was observed and found that the threshold and loss were greatly reduced, and the gain is significantly increased compared with spin-coated coumarin 151…

Photochemistry and Electron Transfer StudiesLuminescence and Fluorescent MaterialsLanthanide and Transition Metal Complexes

Catalytic Reduction of 4,4[sup ʹ]-(2,2,2-Trichloroethane-1,1-diyl)bis(chlorobenzene) with Cobalt(I) Salen Electrogenerated at Vitreous Carbon Cathodes in Dimethylformamide

Philip C. Gach、Mohammad S. Mubarak、Jonathan A. Karty 等 4 位作者2006-12-04Journal of The Electrochemical Society

Catalytic Reduction of 4 , 4 ′ -(2,2,2-Trichloroethane-1,1-diyl)bis(chlorobenzene) with Cobalt(I) Salen Electrogenerated at Vitreous Carbon Cathodes in Dimethylformamide, Gach, Philip C., Mubarak, Mohammad S., Karty, Jonathan A., Peters, Dennis G.

Porphyrin and Phthalocyanine ChemistryElectrochemical Analysis and ApplicationsOxidative Organic Chemistry Reactions

Investigation of Porogen Behavior during the Curing Process of Ultralow-k Spin-On Materials

A. Zenasni、F. Ciaramella、V. Jousseaume 等 5 位作者2006-12-04Journal of The Electrochemical Society

Ultralow- integration issues for node and below is a major challenge. Pore creation was studied vs the matrix film cross-linking. After curing at low temperature some bumps were found dispersed at the top of the film surface. The porosity could be changed by varying the porogen loadings and curing program ramp. At hig…

Mesoporous Materials and CatalysisBlock Copolymer Self-AssemblyCopper Interconnects and Reliability

Microstructure and enhanced in-plane ferroelectricity of Ba0.7Sr0.3TiO3 thin films grown on MgAl2O4 (001) single-crystal substrate

Xuechang Zhou、T. Heindl、G. K. H. Pang 等 8 位作者2006-12-04Applied Physics Letters

The microstructure and in-plane dielectric and ferroelectric properties of highly oriented Ba0.7Sr0.3TiO3 (BST) thin film grown on MgAl2O4 (001) single-crystal substrate through pulsed laser deposition were investigated. X-ray diffraction measurements indicated that BST had a distorted lattice with a tetragonality a∕c…

Ferroelectric and Piezoelectric MaterialsMultiferroics and related materialsMicrowave Dielectric Ceramics Synthesis

Hole transport in p-type ZnO films grown by plasma-assisted molecular beam epitaxy

Jianwu Sun、Ying‐Bing Lu、Yichun Liu 等 10 位作者2006-12-04Applied Physics Letters

The hole transport properties of nitrogen doped p-type ZnO grown on c-plane sapphire (c-Al2O3) were investigated by temperature-dependent Hall-effect measurements. The experimental Hall mobility was found to be considerably lower than the calculated mobility including ionized impurity scattering, acoustic-mode deforma…

ZnO doping and propertiesGas Sensing Nanomaterials and SensorsGa2O3 and related materials