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Disordered antireflective nanostructures on GaN-based light-emitting diodes using Ag nanoparticles for improved light extraction efficiency

Young Min Song、Eun Sil Choi、Gyeong Cheol Park 等 6 位作者2010-08-30Applied Physics Letters

In this study, we demonstrate GaN light-emitting diodes (LEDs) with antireflective subwavelength structures (SWS) for enhanced light extraction efficiency. To eliminate the internal Fresnel reflection, SWS were fabricated on an indium-tin-oxide (ITO) surface using an overall dry etch process of Ag nanoparticles. The a…

ZnO doping and propertiesGaN-based semiconductor devices and materialsOptical Coatings and Gratings

In Situ X-ray Scattering Studies of Protein Solution Droplets Drying on Micro- and Nanopatterned Superhydrophobic PMMA Surfaces

Angelo Accardo、Francesco Gentile、Federico Mecarini 等 7 位作者2010-08-30Langmuir

Superhydrophobic poly(methyl methacrylate) surfaces with contact angles of ∼170° and high optical and X-ray transparencies have been fabricated through the use of optical lithography and plasma etching. The surfaces contain either a microscale pattern of micropillars or a random nanofibrillar pattern. Nanoscale asperi…

Surface Modification and SuperhydrophobicityNanomaterials and Printing TechnologiesFluid Dynamics and Thin Films

Influence of molecular weight on rheological, thermal, and mechanical properties of PEEK

Mingjun Yuan、Jeffrey A. Galloway、Richard J. Hoffman 等 4 位作者2010-08-30Polymer Engineering and Science

Abstract This study focuses on the influence of molecular weight on the rheological, thermal, and mechanical behavior of poly(ether‐ether‐ketone) (PEEK), a semicrystalline high‐performance polymer. The results show that the molecular weight of PEEK has significant influence on its rheological, thermal, and mechanical…

Polymer crystallization and propertiesPolymer Nanocomposites and Propertiesbiodegradable polymer synthesis and properties

Plasmon-mediated superradiance near metal nanostructures

Vitaliy N. Pustovit、Tigran V. Shahbazyan2010-08-30Physical Review B

We develop a theory of cooperative emission of light by an ensemble of emitters, such as fluorescing molecules or semiconductor quantum dots, located near a metal nanostructure supporting surface plasmon. The primary mechanism of cooperative emission in such systems is resonant energy transfer between emitters and pla…

Gold and Silver Nanoparticles Synthesis and ApplicationsPlasmonic and Surface Plasmon ResearchThermal Radiation and Cooling Technologies

Influence of Disorder on Conductance in Bilayer Graphene under Perpendicular Electric Field

Hisao Miyazaki、Kazuhito Tsukagoshi、Akinobu Kanda 等 5 位作者2010-08-30Nano Letters

Electron transport in bilayer graphene placed under a perpendicular electric field is revealed experimentally. Steep increase of the resistance is observed under high electric field; however, the resistance does not diverge even at low temperatures. The observed temperature dependence of the conductance consists of tw…

Carbon Nanotubes in CompositesGraphene research and applicationsThermal properties of materials

(Non)formation of Methanol by Direct Hydrogenation of Formate on Copper Catalysts

Yong Yang、Charles A. Mims、R. S. Disselkamp 等 6 位作者2010-08-30The Journal of Physical Chemistry C

We have attempted to hydrogenate adsorbed formate species on copper catalysts to probe the importance of this postulated mechanistic step in methanol synthesis. Surface formate coverages up to 0.25 were produced at temperatures between 413 and 453 K on supported (Cu/SiO 2 ) copper and unsupported copper catalysts. The…

Catalytic Processes in Materials ScienceCatalysts for Methane ReformingCarbon dioxide utilization in catalysis

Growth of monolayer graphene on 8° off-axis 4H–SiC (000–1) substrates with application to quantum transport devices

Niels Olsen Saraiva Câmara、B. Jouault、Alessandra Caboni 等 10 位作者2010-08-30Applied Physics Letters

Using high temperature annealing conditions with a graphite cap covering the C-face of an 8° off-axis 4H–SiC sample, large and homogeneous single epitaxial graphene layers have been grown. Raman spectroscopy shows evidence of the almost free-standing character of these monolayer graphene sheets, which was confirmed by…

Advancements in Battery MaterialsGraphene research and applicationsDiamond and Carbon-based Materials Research

Large-scale surface reconstruction energetics of Pt(100) and Au(100) by all-electron DFT

Paula Havu、Volker Blum、Ville Havu 等 5 位作者2010-08-30arXiv

The low-index surfaces of Au and Pt all tend to reconstruct, a fact that is of key importance in many nanostructure, catalytic, and electrochemical applications. Remarkably, some significant questions regarding their structural energies remain even today, in particular for the large-scale quasihexagonal reconstructed…

Materials Sciencephysics.comp-ph

Polymer-Fullerene Bulk Heterojunction Solar Cells

Carsten Deibel、Vladimir Dyakonov2010-08-30arXiv

Organic solar cells have the potential to be low-cost and efficient solar energy converters, with a promising energy balance. They are made from carbon-based semiconductors, which exhibit favourable light absorption and charge generation properties, and can be manufactured by low temperature processes such as printing…

Materials Science

Possibilities of application of elastic mid-IR light scattering for inspection of internal gettering operations

O. V. Astafiev、A. N. Buzynin、V. P. Kalinushkin 等 5 位作者2010-08-30arXiv

A method of low-angle mid-IR light scattering is shown to be applicable for the contactless and non-destructive inspection of the internal gettering process in CZ Si crystals. A classifcation of scattering inhomogeneities in initial crystals and crystals subjected to the getting process is presented.

Mesoscale and Nanoscale PhysicsMaterials Sciencephysics.optics

On the nature of large-scale defect accumulations in Czochralski-grown silicon

V. P. Kalinushkin、A. N. Buzynin、V. A. Yuryev 等 5 位作者2010-08-30arXiv

Czochralski-grown boron-doped silicon crystals were studied by the techniques of the low-angle mid-IR-light scattering and electron-beam-induced current. The large-scale accumulations of electrically-active impurities detected in this material were found to be different in their nature and formation mechanisms from th…

Mesoscale and Nanoscale PhysicsMaterials Sciencecond-mat.otherphysics.optics

Direct Ethanol Fuel Cell Using Hydrotalcite Clay as a Hydroxide Ion Conductive Electrolyte

Kiyoharu Tadanaga、Yoshihiro Furukawa、Akitoshi Hayashi 等 4 位作者2010-08-30Advanced Materials

An alkaline-type direct ethanol fuel cell (DEFC) using a natural clay electrolyte with non-platinum catalysts is proposed. So-called hydrotalcite clay, Mg–Al layered double hydroxide intercalated with CO₃²⁻, is shown to be a hydroxide ion conductor. An alkaline-type DEFC using this natural clay as the electrolyte and…

Supercapacitor Materials and FabricationAdvanced Battery Materials and TechnologiesLayered Double Hydroxides Synthesis and Applications

Ultrasensitive and Selective Detection of a Prognostic Indicator in Early‐Stage Cancer Using Graphene Oxide and Carbon Nanotubes

Xiaohui Wang、Chunyan Wang、Konggang Qu 等 8 位作者2010-08-30Advanced Functional Materials

Abstract Cyclin A 2 is a prognostic indicator in early‐stage cancer. However, since most of peptide‐protein bindings do not produce an easily measurable output signal, this severely hinders homogeneous detection of protein using peptide as detection probe. Cyclin A 2 can be detected as low as 0.6 μ M using a well‐know…

Advanced biosensing and bioanalysis techniquesCarbon and Quantum Dots ApplicationsGraphene and Nanomaterials Applications

Conductivity of a graphene strip: Width and gate-voltage dependencies

F. T. Vasko、I. V. Zozoulenko2010-08-30Applied Physics Letters

We study the conductivity of a graphene strip taking into account electrostatically induced charge accumulation on its edges. Using a local dependency of the conductivity on the carrier concentration we find that the electrostatic size effect in doped graphene strip of the width of 0.5–3 μm can result in a significant…

Graphene research and applicationsAdvanced Physical and Chemical Molecular InteractionsSurface and Thin Film Phenomena

Efficient Approach for Simulating Distorted Materials

Pekka Koskinen、Oleg O. Kit2010-08-30Physical Review Letters

The operation principles of nanoscale devices are based upon both electronic and mechanical properties of materials. Because these properties can be coupled, they need to be investigated simultaneously. At this moment, however, the electronic structure calculations with custom-made long-range mechanical distortions ar…

Carbon Nanotubes in CompositesGraphene research and applicationsTheoretical and Computational Physics

Fluctuations and Scaling in Creep Deformation

Jari Rosti、Juha Koivisto、Lasse Laurson 等 4 位作者2010-08-30Physical Review Letters

The spatial fluctuations of deformation are studied in the creep in Andrade's power law and the logarithmic phases, using paper samples. Measurements by the digital image correlation technique show that the relative strength of the strain rate fluctuations increases with time, in both creep regimes. In the Andrade cre…

Microstructure and mechanical propertiesGranular flow and fluidized bedsHigh-Velocity Impact and Material Behavior

Atomic Imaging Using Secondary Electrons in a Scanning Transmission Electron Microscope : Experimental Observations and Possible Mechanisms

H. Inada、D. Su、R. F. Egerton 等 8 位作者2010-08-30arXiv

We report our detailed investigation of high-resolution imaging using secondary electrons (SE) with a subnanometer probe in an aberration-corrected transmission electron microscope, Hitachi HD2700C. This instrument also allows us to acquire the corresponding annular-dark-field (ADF) images simultaneously and separatel…

Materials Science

Leveraging Nanoscale Plasmonic Modes to Achieve Reproducible Enhancement of Light

Ryan T. Hill、Jack J. Mock、Yaroslav Urzhumov 等 9 位作者2010-08-30Nano Letters

The strongly enhanced and localized optical fields that occur within the gaps between metallic nanostructures can be leveraged for a wide range of functionality in nanophotonic and optical metamaterial applications. Here, we introduce a means of precise control over these nanoscale gaps through the application of a mo…

Gold and Silver Nanoparticles Synthesis and ApplicationsPlasmonic and Surface Plasmon ResearchOrbital Angular Momentum in Optics

Micropore Analysis of Polymer Networks by Gas Sorption and 129Xe NMR Spectroscopy: Toward a Better Understanding of Intrinsic Microporosity

Jens Weber、Johannes Schmidt、Arne Thomas 等 4 位作者2010-08-30Langmuir

The microporosity of two microporous polymer networks is investigated in detail. Both networks are based on a central spirobifluorene motif but have different linker groups, namely, imide and thiophene units. The microporosity of the networks is based on the "polymers of intrinsic microporosity (PIM)" design strategy.…

Metal-Organic Frameworks: Synthesis and ApplicationsMembrane Separation and Gas TransportCovalent Organic Framework Applications

Space charge limited conduction with exponential trap distribution in reduced graphene oxide sheets

Daeha Joung、Anindarupa Chunder、Lei Zhai 等 4 位作者2010-08-30Applied Physics Letters

We elucidate on the low mobility and charge traps of the chemically reduced graphene oxide (RGO) sheets by measuring and analyzing temperature dependent current-voltage characteristics. The RGO sheets were assembled between source and drain electrodes via dielectrophoresis. At low bias voltage the conduction is Ohmic…

Graphene research and applicationsLow-power high-performance VLSI designAdvanced Memory and Neural Computing