Materials Literature
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The formation of a (quasi) two-dimensional electron gas between the band insulators NaTaO3 and SrTiO3 is studied by means of the full-potential linearized augmented plane-wave method of density functional theory. Optimization of the atomic positions points to only small changes in the chemical bonding at the interface…
Acid-induced double lactonization in triarylamine-conjugated dimethyl diethynylfumarate E-1 opens up a new synthetic route to Pechmann dyes. This one-pot reaction affords three donor-acceptor-donor quadrupolar molecules (P(55)-1, P(66)-1, and P(56)-1); P(56)-1 comprises a missing structural isomer of Pechmann dyes. Th…
This paper presents the design, simulation, and measurement of an asymmetric triple-band metamaterial composed of single geometry electric field coupled resonators in the terahertz region. Theoretical and experimental results show that the structure has three distinct and strong absorption frequency peaks near 0.38, 0…
Switchable voltage modulation of the magnetic properties is reported in different multiferroic bilayers with magnetic films grown on pre-poled ferroelectric substrates, based on the magneto-optical Kerr effect observations. The dynamic voltage control of the magnetic coercive field (Hc) is dependent not only on the ma…
Hafnia-alumina nanolaminates show improved smoothness and reduced crystallinity relative to pure hafnia in films formed by atomic layer deposition (ALD). However, typical nanolaminates also show reduced cross-plane thermal conductivity due to the much larger interface density relative to continuous films. We find that…
Abstract We show measurements on a bilayer graphene quantum dot (QD) with an integrated charge detector. The focus lies on enabling charge detection with a 30 nm wide bilayer graphene nanoribbon located approximately 35 nm next to a bilayer graphene QD with an island diameter of about 100 nm. Local resonances in the n…
In the study, we introduced the local mean free path of phonons with boundary effects. The local thermal conductivity distribution from boundary to film bulk region was obtained, and the boundary scattering effect was examined by introducing a phonon Knudsen layer thickness. We calculated the ratio of effective therma…
Correlation between the elastic modulus (B) and the Raman shift (Δω) of TiO2 and their responses to the variation of crystal size, applied pressure, and measuring temperature have been established as a function depending on the order, length, and energy of a representative bond for the entire specimen. In addition to…
Light polarization-sensitive UV photodetectors (PSPDs) using non-polar a-plane ZnMgO/ZnO multiple quantum wells grown both on sapphire and ZnO substrates have been demonstrated. For the PSPDs grown on sapphire with anisotropic biaxial in-plain strain, the responsivity absorption edge shifts by ΔE ∼ 21 meV between ligh…
[100] oriented Sr0.75Ba0.25Nb2O6 relaxor crystals have been studied by means of acoustic emission (AE) over a wide 20–400 °C temperature range. Both the Burns temperature, Td = 350 °C, and the intermediate temperature, T* = 183°C, and the susceptibility maximum temperature, Tm (59 °C on heating and 47 °C on cooling),…
Nanohybrids of silver nanoparticles (AgNPs) supported on mica clay were synthesized by in situ reduction of silver nitrate in an aqueous solution. The required mica platelets of high aspect ratio were previously prepared by the exfoliation of mica clay stacks in a multilayered structure through an ionic exchange react…
Using density functional theory calcualtions, we reveal a novel control on the functionalizations of hexagonal boron nitride ( h -BN) structures by carrier doping. When the system is electron-doped, adatoms (e.g., H or F atoms) will exclusively bond with B atoms, resulting in possible magnetization of the system, wher…
Abstract Carbon‐encapsulated ferromagnetic Cobalt nanoparticles (Co@C) have been synthesized by catalytic chemical vapour deposition (CCVD). The nanoparticles, mainly ranging between 10 and 15 nm, are tightly encapsulated by 2–3 concentric graphitic carbon shells and protected from oxidation. Because of their magnetic…
Enhanced electron field emission (EFE) properties have been observed for nitrogen implanted ultra-nanocrystalline diamond (UNCD) films grown by microwave plasma enhanced CVD. X-ray photoelectron spectroscopy (XPS) measurements show that sp2 fraction and C-N bonding increase upon N-implantation and annealing. Significa…
Intense green upconversion emission in Ho:Yb:Gd2O3 spherical nanoparticles is reported through hetrolooping enhanced energy transfer process. Different techniques used for structural characterization divulge the formation of spherical Ho:Yb:Gd2O3 crystals of diameter ∼100 nm. Efficient energy transfer from Yb3+ → Ho3+…
Electrical characteristics of Cr/Au and Ti/Au metal contacts on epitaxial graphene on 4H-SiC showed significant variations in resistance parameters at 300 K. These parameters decreased substantially as the temperature increased to 673 K. The work function, binding energy, and diffusion energy of the deposited metals w…
The porosity dependence of the elastic properties of porous silicon in different crystallographic directions is studied. The velocity of longitudinal acoustic waves in porous silicon layers electrochemically etched in (100), (110), and (111) oriented wafers has been measured by acoustic spectroscopy in the gigahertz f…
Low-k dielectrics have predominantly replaced silicon dioxide as the interlayer dielectric for interconnects in state of the art integrated circuits. In order to further reduce interconnect RC delays, additional reductions in k for these low-k materials are being pursued via the introduction of controlled levels of po…
Using the first-principle phonon calculations under the quasiharmonic approximation, thermal expansions in III-nitrides with wurtzite AlN, GaN, and InN are reported. The results showed that it is different for each thermal expansion of three III-nitrides at low temperatures, which is consistent with their Grüneisen pa…
It is shown that the short-circuit photocurrent measured under illumination in Pb(Zr,Ti)O3 epitaxial films is strongly dependent on the metal used as the top electrode. The magnitude of the photocurrent varies by more than 2 orders of magnitude from Pt (largest signal) to Al (smallest signal). The differences are for…