Materials Literature
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Carbon dots (Cdots) are an important probe for imaging and sensing applications because of their fluorescence property, good biocompatibility, and low toxicity. However, complex procedures and strong acid treatment are often required and Cdots suffer from low photoluminescence (PL) emission. Herein, a facile and gener…
Carbon nanotubes: The end section of a carbon nanotube, cut by acid treatment, contains hydrophilic oxygen groups, around which water molecules can assemble to block the entry of the tube. Hydrogen of pressures up to 10 000 bar can be locked inside the tube by such an “aqueous valve” (see picture).
We propose and analyze a novel mechanism for long-range spin-spin interactions in diamond nanostructures. The interactions between electronic spins, associated with nitrogen-vacancy centers in diamond, are mediated by their coupling via strain to the vibrational mode of a diamond mechanical nanoresonator. This couplin…
We propose in this work, contact Schottky Nickel/porous silicon (PSi) system, coupled to nanocrystallites size variation of material for a possible technique to reduce dark current. The device consists of metal- semiconductor-metal photodiode (MSM-PD). Higher barrier ΦΒ enhances the performance of MSM-PD through reduc…
A series of novel, highly symmetrical phthalocyanines bearing eight peptide residues has been prepared by microwave-assisted Cu(I)-catalyzed 1,3-dipolar cycloaddition (‘click’ reaction). Water-soluble conjugates were obtained after straightforward deprotection of the amine and amide functionalities. The phthalocyanin…
Recent experiments suggest that the interfacial thermal conductance of transfer printed metal-dielectric interfaces is ∼45 MW/m2K at 300 K, approaching that of interfaces formed using physical vapor deposition. We investigate this anomalous result using a combination of theoretical deformation mechanics and nanoscale…
Abstract Two porphyrin‐based dyes were synthesized that incorporate two additional chromophores to absorb in a wider UV/Vis region. In the first dye, a porphyrin ring is linked through an amide bond to two [Ru(bpy) 3 ] 2+ units, forming a symmetric [Ru(bpy) 3 ]‐porphyrin‐[Ru(bpy) 3 ] {Por(COOH) 2 [Ru(bpy) 3 ] 2 } syst…
It is shown that the nanocryatalline silicon ballistic electron emitter operates in a SiCl4 solution without using any counter electrodes and that thin amorphous Si films are efficiently deposited on the emitting surface with no contaminations and by-products. Despite the large electrochemical window of the SiCl4 solu…
We study the spatiotemporal low-frequency microrheology of a gelatin gel during the sol-gel transition after a fast temperature quench by tracking the motion of embedded colloidal particles. From the particle dynamics two different mechanisms responsible for the gelation of the sol phase can be identified: a fast proc…
This work investigates properties of a smectic C^* liquid crystal film containing defects that cause distinctive spiral patterns in the filmʼs texture. The phenomena are described by a Ginzburg–Landau type model and the investigation provides a detailed analysis of minimal energy configurations for the filmʼs director…
Second harmonic (SH) generation from AlGaAs near-wavelength high-contrast gratings was studied in polarization-dependent reflection measurements. The grating design is critical in determining the strength and polarization of the second harmonic signal. The second harmonic response was enhanced by more than 3 orders of…
The role of framework oxygen atoms in N(2)O decomposition [N(2)O(g)→N(2)(g) and 1/2O(2)(g)] over Fe-ferrierite is investigated employing a combined experimental (N(2)(18)O decomposition in batch experiments followed by mass spectroscopy measurements) and theoretical (density functional theory calculations) approach. T…
The evolution of grain boundary microstructure during annealing in sputtered gold thin films was investigated on the basis of FEG-SEM/EBSD/OIM analyses of nanocrystalline microstructure, in order to find a clue to the precise control of grain boundary microstructure for development of high performance polycrystalline…
The application of new biomaterial technologies offers the potential to direct the stem cell fate, targeting the delivery of cells and reducing immune rejection, thereby supporting the development of regenerative medicine. Cells respond to their surrounding structure and with nanostructures exhibit unique proliferativ…
Effect of solvent quality on phase transition of lyotropic rigid-chain liquid crystal polymer is studied by dissipative particle dynamics simulation. A rod composed of fused DPD particles is used to represent the solvated rigid polymer. The effect of solvent quality is investigated by adjusting the repulsion parameter…
In the binary mixture phase diagram of MC881 and MC452, the borderline between anticlinic antiferroelectric SmC(A)(*) and synclinic ferroelectric SmC(*) becomes apparently parallel to the temperature ordinate axis at the critical concentration r(c). The free energy difference between SmC(A)(*) and SmC^{*} is extremely…
The relaxor behavior of tetragonal tungsten bronze uniaxial relaxor ferroelectric calcium strontium barium niobate (Ca0.22Sr0.12Ba0.66Nb2O6 or CSBN-22) single crystal was studied by measuring elastic constants and thermal expansion with the aid of resonant ultrasound spectroscopy and dilatometry, respectively, in the…
In this paper, Cu(x)O photocatalyst on plasmonic nanoporous Au film is proposed to enhancing the H(2) evolution rate of pure water splitting. The nanoporous Au film can simultaneously provide surface-enhanced absorption and built-in potential. The reflection spectrum shows that the surface plasmon (SP) assisted absorp…
The phenomenon of giant magnetoresistance (GMR) in spin-valves under applied magnetic field is well established. We present piezoelectric control of the GMR ratio at room temperature for standard multilayered spin-valve structure fabricated on (011)-Pb(Mg1/3Nb2/3)O3-PbTiO3 (PMN-PT) piezoelectric substrate. Four sample…
We have recently reported erbium (Er)-related visible and infrared (∼1540 nm) electroluminescence (EL) from the light-emitting device (LED) based on Er-doped TiO2 (TiO2:Er)/p+-Si heterostructure, triggered by the energy transferred from oxygen-vacancy-related self-trapped excitons (STEs) to Er3+ ions in anatase TiO2.…