Materials Literature
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In this study, gold nanoparticles (GNP) were stabilized for the first time as dimers by a conducting polymer (CP). The morphology of kissing particles was examined by high-resolution transmission electronic microscopy (HRTEM). The broad-band localized surface plasmon resonance (LSPR) tunable by solvent variation and m…
We have studied the elastocaloric effect in a Co-doped Ni-Mn-Ga magnetic Heusler shape memory alloy in the vicinity of its martensitic transition. Measurements of the length change as a function of temperature have been carried out across the transition under applied compression stresses and magnetic fields. The isoth…
A novel method was used to synthesize triangular gold nanoparticles (AuNPs) (i.e., trisodium citrate reduction of HAuCl 4 in the presence of nonionic fluorosurfactant). The as-prepared triangular AuNPs owned higher surface-to-volume ratio and more active surface sites compared to spherical AuNPs, which facilitated the…
The teratogenic potential of commercially available copper oxide (CuO), titanium dioxide (TiO2) and zinc oxide (ZnO) nanoparticles (NPs) was evaluated using the standardized FETAX test. After characterization of NP suspensions by TEM, DLS and AAS, histopathological screening and advanced confocal and energy-filtered e…
The influence of static correlations beyond the pair level on the dynamics of selected model glass formers is investigated. The pair structure, angular distribution functions, and statistics of Voronoi polyhedra of two well-known Lennard-Jones mixtures as well as of the corresponding Weeks-Chandler-Andersen variants,…
Based on transformation optics, we present a shrinking device, which can transform an arbitrary object virtually into a small-size object with different material parameters as one desires. Such an illusion device will confuse the detectors or the viewers, and hence the real size and material parameters of the enclosed…
The growth of polysaccharide multilayers consisting of positively charged chitosan (CH) and negatively charged heparin (HEP) was monitored in situ by employing a quartz crystal microbalance (QCM-D) and dual-polarization interferometry (DPI). The main focus was on how the physicochemical properties of the solution affe…
A theoretical study proposes the atomic configuration of electron-beam irradiated C$_{60}$ thin films. We examined the electronic structure and electron-transport properties of the C$_{60}$ clusters using density-functional calculations and found that a rhombohedral C$_{60}$ polymer with $sp^3$-bonded dumbbell-shaped…
In this paper, we report a novel electrochemical doping method for conducting polymer films based on bipolar electrochemistry. The electrochemical doping of conducting polymers such as poly(3-methylthiophene) (PMT), poly(3,4-ethylenedioxythiophene) (PEDOT), and poly(aniline) (PANI) on a bipolar electrode having a pote…
This work reviews and examines two particular issues related with the new technique of electrical detection of ferromagnetic resonance (FMR). This powerful technique has been broadly applied for studying magnetization and spin dynamics over the past few years. The first issue is the relation and distinction between di…
The commissioning and performance characterization of a position-sensitive detector designed for fast X-ray powder diffraction experiments on beamline I11 at Diamond Light Source are described. The detecting elements comprise 18 detector-readout modules of MYTHEN-II silicon strip technology tiled to provide 90° covera…
Diffusionless phase transitions are at the core of the multifunctionality of (magnetic) shape memory alloys, ferroelectrics and multiferroics. Giant strain effects under external fields are obtained in low symmetric modulated martensitic phases. We outline the origin of modulated phases, their connection with tetragon…
First-principles calculations based on density functional theory are performed on graphene/BN and BN bilayers to investigate the effect of the strain on their energy gaps. For the graphene/BN bilayer, the bands have characteristic graphenelike features with a small band gap at $K$. Application of strain modulates the…
We report a direct STM observation of Ge hut array nucleation on the Si(001) surface during ultrahigh vacuum molecular-beam epitaxy at 360C. Nuclei of pyramids and wedges have been observed on the wetting layer MxN patches starting from the coverage of about 5.1 Å (~3.6 ML). Further development of hut arrays consists…
Large-scale and gap error free calculations of the electronic structure of vacancies in 4H-SiC have been carried out using a hybrid density functional (HSE06) and an accurate charge correction scheme. Based on the results the carbon vacancy is proposed to be responsible for the Z1/2 and EH6/7 DLTS centers
We investigate the optical properties of edge-functionalized graphene nanosystems, focusing on the formation of junctions and charge-transfer excitons. We consider a class of graphene structures that combine the main electronic features of graphene with the wide tunability of large polycyclic aromatic hydrocarbons. By…
We report the discovery of ${\mathrm{K}}_{x}$Fe${}_{2\ensuremath{-}y}$S${}_{2}$ single crystals, isostructural to ${\mathrm{K}}_{x}$Fe${}_{2\ensuremath{-}y}$Se${}_{2}$ superconductors. The sulfide compound is a small gap semiconductor and shows spin-glass behavior below 32 K. Our results indicate that stoichiometry, d…
Using powder neutron diffraction we have discovered an unusual magnetic order-order transition in the Ising spin chain compound Ca3Co2O6. On lowering the temperature an antiferromagnetic phase with propagation vector k=(0.5,-0.5,1) emerges from a higher temperature spin density wave structure with k=(0, 0, 1.01). This…
The suitability of magnetic nanoparticles (MNPs) to act as heat nano-sources by application of an alternating magnetic field has recently been studied due to their promising applications in biomedicine. The understanding of the magnetic relaxation mechanism in biocompatible nanoparticle systems is crucial in order to…
Degradable and electrically conductive polysaccharide hydrogels (DECPHs) have been synthesized by functionalizing polysaccharide with conductive aniline oligomers. DECPHs based on chitosan (CS), aniline tetramer (AT), and glutaraldehyde were obtained by a facile one-pot reaction by using the amine group of CS and AT u…