Materials Literature
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By employing 3D current collectors, hybrid coplanar microsupercapacitors are fabricated. These devices show excellent energy density of 200 μW h cm−2 compared to the state-of-the-art microsupercapacitors (1–40 μW h cm−2), and superior power density (4.4 mW cm−2) compared to thin film batteries and microbatteries at co…
We report on a new chemical sensor based on black phosphorus/molybdenum diselenide van der Waals hetero-junctions. Due to the atomically thin nature of two-dimensional (2D) materials, surface adsorption of gas molecules can effectively modulate the band alignment at the junction interface, making the device a highly s…
The spins of point defects in silicon carbide are promising candidates for qubits and sensors under $a\phantom{\rule{0}{0ex}}m\phantom{\rule{0}{0ex}}b\phantom{\rule{0}{0ex}}i\phantom{\rule{0}{0ex}}e\phantom{\rule{0}{0ex}}n\phantom{\rule{0}{0ex}}t$ conditions. Unlike defect-bearing diamond, SiC is regarded as an indust…
SO2 poisoning of methane oxidation over alumina-supported, [email protected]xZr1−xO2 nanoparticle catalysts was systematically studied by means of advanced PhotoElectron Spectroscopy (PES) methods. The [email protected]xZr1−xO2 units were synthesized and deposited on two modified-alumina supports, i.e. high surface ar…
Recently, there have been efforts to use clean and renewable energy because of finite fossil fuels and environmental problems. Owing to the site-specific and weather-dependent characteristics of the renewable energy supply, solid oxide electrolysis cells (SOECs) have received considerable attention to store energy as…
Abstract This work proposes a complete and consistent set of cross sections for electron collisions with carbon dioxide (CO 2 ) molecules to be published in the IST-Lisbon database with LXCat. The set is validated from the comparison between swarm parameters calculated using a two-term Boltzmann solver and the availab…
We have performed an x-ray holotomography study of a three-dimensional (3D) photonic band gap crystal. The crystals was made from silicon by CMOS-compatible methods. We manage to obtain the 3D material density throughout the fabricated crystal. We observe that the structural design is for most aspects well-realized by…
We performed X-ray diffraction and electrical resistivity measurement up to pressures of 5 GPa and the first-principles calculations utilizing experimental structural parameters to investigate the pressure-induced topological phase transition in BiTeBr having a noncentrosymmetric layered structure (space group P3m1).…
In van der Waals heterostructures, the periodic potential from the Moiré superlattice can be used as a control knob to modulate the electronic structure of the constituent materials. Here we present a nanoscale angle-resolved photoemission spectroscopy (nano-ARPES) study of transferred graphene/h-BN heterostructures w…
Nanometre-scale pores and capillaries have long been studied because of their importance in many natural phenomena and their use in numerous applications. A more recent development is the ability to fabricate artificial capillaries with nanometre dimensions, which has enabled new research on molecular transport and le…
Alkali-doped fullerides A$_n$C$_{60}$ show a remarkably wide range of electronic phases in function of A= Li, Na, K, Rb, Cs and the degree of doping, $n=1-5$. While the presence of strong electron correlations is well established, recent investigations give also evidence for dynamical Jahn-Teller instability in the in…
Ferroelectrics that allow a coupling between the polarization and another order parameter are of great interest because they could make the electric field control of nonpolar order parameters possible. In recent years, ``hybrid improper''' ferroelectrics - materials where the polarization couples to two different stru…
The modern semilocal exchange potential is an accurate and efficient approximation to the exact exchange potential of density functional theory. We tried to combine it with the dynamical mean-field theory to derive a new first-principles many-body approach for studying correlated electronic materials. As a paradigm, t…
Topological insulators are attracting considerable interest due to their potential for technological applications and as platforms for exploring wide-ranging fundamental science questions. In order to exploit, fine-tune, control and manipulate the topological surface states, spectroscopic tools which can effectively p…
The Coulomb interaction among massless Dirac fermions in graphene is unscreened around the isotropic Dirac points, causing a logarithmic velocity renormalization and a cone reshaping. In less symmetric Dirac materials possessing anisotropic cones with tilted axes, the Coulomb interaction can provide still more exotic…
The early strength evolution of self-consolidating concrete (SCC) is studied by a set of non-standard mechanical tests for compressive, tensile, shear and bending failure. The results are applicable in an industrial environment for process control, e.g. of slip casting with adaptive molds in robotic fabrication. A pro…
Superconductivity originates from pairing of electrons near the Fermi energy. The Fermi surface topology and pairing symmetry are thus two pivotal characteristics of a superconductor. Superconductivity in one monolayer (1 ML) FeSe thin film has attracted great interest recently due to its intriguing interfacial proper…
A dandelion‐like supramolecular polymer (DSP) with a “sphere‐star‐parachute” topological structure consisting of a spherical hyperbranched core and many parachute‐like arms is constructed by the non‐covalent host–guest coupling between a cyclodextrin‐endcapped hyperbranched multi‐arm copolymer (host) and many function…
The ambient environmental instability and degradation mechanism of single- and few-layer WTe2 are investigated. Oxidation of W and Te atoms appears to be a main reason for degradation. Single-layer samples' Raman signals disappear within 20 min in air. Few-layer WTe2 exhibits saturating degradation behavior: only the…
This paper reports a simple and economical method for the fabrication of nanopatterned optical fiber nanotips. The proposed patterning approach relies on the use of the nanosphere lithography of the optical fiber end facet. Polystyrene (PS) nanospheres are initially self-assembled in a hexagonal array on the surface o…