Materials Literature
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Microporous, pillared graphene-based frameworks are generated in a simple functionalization/coupling procedure starting from reduced graphene oxide. They are used for the fabrication of high-performance supercapacitor devices.
Molecular ferroelectrics with high-temperature reversible phase-transition behaviors are very rare and have currently become one of the hotspots in the field of ferroelectric materials. Herein we display two new crown ether clathrates possessing unusual high-temperature ferroelectric phase-transition behaviors, cycloh…
A bulk dielectric polymer film with an intrinsic ultralow k value of 1.52 at 10 kHz has been successfully synthesized based on a novel polyimide FPTTPI. More importantly, such outstanding dielectric properties remain stable up to 280 °C. The excellent ultralow dielectric properties are mainly because of the larger fre…
High-quality large-sized hexagoal WSe2 crystals can be grown on dielectric substrates using atmospheric chemical vapor deposition in the presence of hydrogen gas. These hexagonal crystals (lateral width >160 um) have a carrier mobility of 100 cm(2) V(-1) s(-1) and a photoresponsivity of ≈1100 mA W(-1), which is compar…
The application potential of cellulose nanofibril (CNF) aerogels has been hindered by the slow and costly freeze‐ or supercritical drying methods. Here, CNF aerogel membranes with attractive mechanical, optical, and gas transport properties are prepared in ambient conditions with a facile and scalable process. Aqueous…
One-way propagation of light, analogous to the directional flow of electrons in the presence of electric potential difference, has been an important goal in the wave-matter interaction. Breaking time-reversal symmetry in photonic flows is faced with challenges different from those for electron flows. In recent years s…
Recently, there has been a great deal of interest in using the photoisomerization of azobenzene compounds to control specific biological targets in vivo. These azo compounds can be used as research tools or, in principle, could act as optically controlled drugs. Such "photopharmaceuticals" offer the prospect of target…
<p>Semicontinuous gold films 4 nm to 12 nm thick were characterized using patterned coplanar waveguides over a frequency range of 100 MHz to 20 GHz. Such films can form two dimensional fractal aggregates mixed with dielectric voids with unusually large electromagnetic absorption. Surface conductance and microwav…
We investigate the catalytic activity of the subnanometer-sized bimetallic Au19Pt cluster for oxidation of CO via first-principles density functional theory calculations. For this purpose we consider two structurally similar and energetically close homotops of the Au19Pt cluster with the Pt atom occupying an edge (Td-…
ABSTRACT The delivery of sub‐micron droplets of dilute polymer solutions to a heated substrate by electrospray atomization enabled precisely controlled and continuous deposition, or growth, of block copolymer thin films. It also provided, in principle, the ability to fabricate heterolattice materials using sequential…
The geometry and internal packing of twisted ropes composed of carbon nanotubes (CNTs) are considered, and a numerical solution in the context of the mesoscopic distinct element method (MDEM) is proposed. Compared to the state of the art, MDEM accounts in a computationally tractable manner for both the deformation of…
In this work, we have devised a new approach to measure the critical pressure that a liquid marble can withstand. A liquid marble is gradually squeezed under a mechanical compression applied by two parallel plates. It ruptures at a sufficiently large applied pressure. Combining the force measurement and the high-speed…
In the present paper, we studied the sintering of a submicronic α-alumina powder and modeled its behavior using Olevsky's model. We further introduced a method for the identification of the creep parameters based on SPS experiments that greatly simplify parameter determination. Subsequently, we used the set of paramet…
Abstract The protocol for analysis of rock-forming mineral compositions by X-ray electron probe microanalysis used at the Institute of Geology and Mineralogy, Novosibirsk, Russia, is described. The analysis is conducted with a JXA-8100 electron probe microanalyzer capable to support a highly stable beam at relatively…
In this study we explore the fundamental aspects of Pickering emulsions stabilized by oppositely charged particles. Using oppositely charged latex particles as a model system, Pickering emulsions with good long-term stability can be obtained without the need for any electrolyte. The effects of parameters like oil to w…
The Japanese art of turning flat sheets into 3D intricate structures, origami, has inspired design of mechanical metamaterials. Mechanical metamaterials are artificially engineered materials with uncommon properties. Miura-ori is a remarkable origami folding pattern with metamaterial properties and a wide range of app…
The exploration of emerging materials physics and prospective applications of two-dimensional materials greatly relies on the growth control of their thickness, phases, morphologies and film-substrate interactions. Though substantial progresses have been made for the development of two-dimensional films from conventio…
Exchange bias is often observed when anti-ferromagnetic and ferromagnetic phases coexist. The coexistence of two competing magnetic phases can persist to the lowest temperatures if the disorder-broadened 1st order transition separating them is interrupted, as is proposed in the kinetic arrest phenomenon. The fractions…
Organic-inorganic halide perovskites, especially methylammonium lead halide, have recently led to a remarkable breakthrough in photovoltaic devices. However, due to the environmental and stability concerns of the heavy metal, lead, in these perovskite based solar cells, research in the non-lead perovskite structures h…
The ability to fabricate dense small features over a large area is important for graphene plasmonics. We present the first self-assembled graphene plasmonic resonators operating in the mid-IR. The resonators are 35 nm in diameter with 20 nm spacing and cover a centimeter sized area. The resonators exhibit a very broad…