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Interaction between tetrathiafulvalene carboxylic acid and ytterbium DO3A: solution state self-assembly of a ternary complex which is luminescent in the near IRElectronic supplementary information (ESI) available: cyclic voltammograms of TTF-YbDO3A and YbDO3A. See http://www.rsc.org/suppdata/cc/b2/b204218e/

Stephen Faulkner、Benjamin P. Burton‐Pye、T. Khan 等 6 位作者2002-07-04Chemical Communications

Tetrathiafulvalene carboxylate associates with the charge neutral complex, Yb.DO3A, in methanolic solution to give rise to a novel ternary species; the tetrathiafulvalene unit transfers energy to the lanthanide, causing luminescence from the Yb metal, indicating for the first time that an electron donor chromophore ca…

Magnetism in coordination complexesLanthanide and Transition Metal ComplexesOrganic and Molecular Conductors Research

Polarization-dependent soft-x-ray absorption of highly oriented ZnO microrod arrays

J-H Guo、Lionel Vayssières、Clas Persson 等 5 位作者2002-07-04Journal of Physics Condensed Matter

Polarization-dependent x-ray absorption measurements were performed on crystalline ZnO three-dimensional arrays consisting of highly oriented microrods as well as on particulate thin films consisting of monodisperse spherical nanoparticles. Strong anisotropic effects have been observed for the highly oriented ZnO rods…

ZnO doping and propertiesMultiferroics and related materialsGa2O3 and related materials

Synthesis of an ordered macroporous carbon with 62 nm spherical pores that exhibit unique gas adsorption properties

Soonki Kang、Jong‐Sung Yu、Michał Kruk 等 4 位作者2002-07-04Chemical Communications

An ordered macroporous carbon with 62 nm spherical pores was synthesized using colloidal-crystal templating and found to exhibit unique gas adsorption properties that have been so far attributed to adsorption in mesopores (size below 50 nm).

Zeolite Catalysis and SynthesisMesoporous Materials and CatalysisCovalent Organic Framework Applications

Defects in ultrathin copper nanowires

Jeong Won Kang、Jae Jeong Seo、Ki Ryang Byun 等 4 位作者2002-07-04arXiv

We have performed atomistic simulations for cylindrical multi-shell (CMS)-type Cu nanowires containing defects. Our investigation has revealed some physical properties that have not been detected in previous studies that have considered defect-free nanowires. Since the vacancy formation energy is lowest in the core of…

Materials Science

Superconductivity, critical current density, and flux pinning in MgB_{2-x}(SiC)_{x/2} superconductor after SiC nanoparticle doping

S. X. Dou、A. V. Pan、S. Zhou 等 8 位作者2002-07-04arXiv

We investigated the effect of SiC nano-particle doping on the crystal lattice structure, critical temperature T_c, critical current density J_c, and flux pinning in MgB_2 superconductor. A series of MgB_{2-x}(SiC)_{x/2} samples with x = 0 to 1.0 were fabricated using in-situ reaction process. The contraction of the la…

Materials ScienceSuperconductivity

Synthesis and Gelation of DOPA-Modified Poly(ethylene glycol) Hydrogels

Bruce P. Lee、Jeffrey L. Dalsin、Phillip B. Messersmith2002-07-04OpenAlex

3,4-Dihydroxyphenylalanine (DOPA) residues are known for their ability to impart adhesive and curing properties to mussel adhesive proteins. In this paper, we report the preparation of linear and branched DOPA-modified poly(ethylene glycol)s (PEG-DOPAs) containing one to four DOPA endgroups. Gel permeation chromatogra…

biodegradable polymer synthesis and propertiesPolymer Surface Interaction StudiesCollagen: Extraction and Characterization

Metal Oxide Nanoparticles as Bactericidal Agents

Peter K. Stoimenov、Rosalyn L. Klinger、George L. Marchin 等 4 位作者2002-07-04OpenAlex

Reactive magnesium oxide nanoparticles and halogen (Cl 2, Br 2 ) adducts of these MgO particles were allowed to contact certain bacteria and spore cells. Bacteriological test data, atomic force microscopy (AFM) images, and electron microscopy (TEM) images are provided, which yield insight into the biocidal action of t…

Electronic and Structural Properties of OxidesMagnesium Oxide Properties and ApplicationsNanotechnology research and applications

Interlocking Inorganic Screw Helices: Synthesis, Structure, and Magnetism of the Novel Framework Uranium Orthothiophoshates A11U7(PS4)13 (A=K, Rb)

Christine Gieck、Wolfgang Tremel2002-07-03Chemistry - A European Journal

The novel quaternary uranium thiophosphate K11U7(PS4)13 has been synthesized by reacting uranium metal, K2S, S, and P2S5 at 700 degrees C in an evacuated silica tube. The crystal structure was determined by single crystal X-ray diffraction techniques. K11U7(PS4)13 crystallizes in the tetragonal space group I42d (a = 3…

Crystal Structures and PropertiesRadioactive element chemistry and processingLanthanide and Transition Metal Complexes

Tris(o-phenylendioxy)cyclotriphosphazen mit eingeschlossenen Iodmolekülen: ein supramolekularer elektrischer Leiter

T. Hertzsch、Felix Budde、Edwin Weber 等 4 位作者2002-07-03Angewandte Chemie

Effizienter Gastaustausch: In einer Iodatmosphäre zeigt das organische Zeolithanalogon TPP⋅x(THF) (x=0.35–0.6) eine sofortige I2-Sorption. Der zuvor farblose Kristall (a) färbt sich an den Kristallenden (b) und ist nach 1–2 Tagen vollständig mit I2 durchdrungen (c). Die elektrische Leitfähigkeit der TPP⋅y(I2)-Kristall…

Metal-Organic Frameworks: Synthesis and ApplicationsMagnetism in coordination complexesAdvanced NMR Techniques and Applications

[ɛ-PMo12O36(OH)4{La(H2O)4}4]5+: The Firstɛ-PMo12O40 Keggin Ion and Its Association with the Two-Electron-Reducedα-PMo12O40 Isomer

Pierre Mialane、Anne Dolbecq、Laurent Lisnard 等 6 位作者2002-07-03Angewandte Chemie

Sechs Mo-Dimere, die um ein zentrales PO4-Tetraeder gruppiert sind, bilden den Kern des neuartigen, von vier {La(H2O)4}3+-Einheiten umgebenen ε-Keggin-Polyoxokations [ε-PMo12O36(OH)4{La(H2O)4}4]5+ (siehe Struktur). 31P-NMR-spektroskopische Untersuchungen ergaben, dass ε-Keggin-Ionen in wässriger Lösung nicht stabil si…

Metal-Organic Frameworks: Synthesis and ApplicationsPolyoxometalates: Synthesis and ApplicationsVanadium and Halogenation Chemistry

Simplified model of stress‐induced crystallization kinetics of polymers

Jianxin Guo、K. A. Narh2002-07-03Advances in Polymer Technology

Abstract A stress‐induced crystallization model for semicrystalline plastics is proposed based on the theory that stress‐induced orientation of molecules and chains increase the melting temperature of thermoplastics, and hence, the supercooling which is the driving force for crystallization. By assuming that the effec…

Polymer crystallization and propertiesPolymer Nanocomposites and PropertiesAdditive Manufacturing and 3D Printing Technologies

Structural disorder in liquid and solid CuI at high temperature probed by x-ray absorption spectroscopy

A. Trapananti、Andrea Di Cicco、Marco Minicucci2002-07-03Physical review. B, Condensed matter

A detailed investigation of local structure and phase transitions in copper iodide (CuI), at high temperatures, has been carried out performing x-ray absorption spectroscopy (XAS), x-ray absorption temperature scans, and energy scanning x-ray diffraction measurements. Low-noise XAS spectra have been recorded in a wide…

Theoretical and Computational PhysicsX-ray Spectroscopy and Fluorescence AnalysisX-ray Diffraction in Crystallography

Facile Azidothermal Metathesis Route to Gallium Nitride Nanoparticles

Jianjun Wang、L. Grocholl、Edward G. Gillan2002-07-03Nano Letters

This report describes a straightforward, metathesis (exchange) reaction between gallium chloride and sodium azide that produces gallium nitride nanoparticles below 210 °C. Slowly heating these two reagents together circumvents rapid, exothermic reactions, which can decompose the nitride product. The resulting GaN powd…

GaN-based semiconductor devices and materialsQuantum Dots Synthesis And PropertiesSemiconductor materials and devices

Kinetics of MTO-Catalyzed Olefin Epoxidation in Ambient Temperature Ionic Liquids: UV/Vis and 2H NMR Study MTO= methyltrioxorhenium.

Gregory S. Owens、Armando Durazo、Mahdi M. Abu‐Omar2002-07-03Chemistry - A European Journal

The kinetics of oxygen-atom transfer from the peroxo complexes of methyltrioxorhenium (MTO) to alkenes in ionic liquids have been investigated. Noncatalytic conversions of alkenes to epoxide were monitored by UV/Vis at 360 nm, where the monoperoxorhenium (mpRe) and diperoxorhenium (dpRe) complexes absorb. Water- and p…

Polyoxometalates: Synthesis and ApplicationsCatalysis and Oxidation ReactionsOxidative Organic Chemistry Reactions

[{Fe(OMe)2[O2CC(OH)Ph2]}12]: Synthesis and Characterization of a New Member in the Family of Molecular Ferric Wheels with the Carboxylatobis(alkoxo) Bridging Unit

Catherine P. Raptopoulou、V. Tangoulis、E. Devlin2002-07-03Angewandte Chemie International Edition

New wheels: The 1:2 reaction of ferric nitrate with benzilic acid (Ph2C(OH)COOH) in methanol at pH≈4.0 results in the formation of a new member of the molecular ferric-wheels family with the carboxylatobis(alkoxo) bridging unit. The molecular structure of [{Fe(OMe)2[Ph2C(OH)COO]}12] (see picture) consists of a centros…

Metal complexes synthesis and propertiesMagnetism in coordination complexesMetal-Catalyzed Oxygenation Mechanisms

Abfangen und Einspeisen von Energie in Farbstoff-Zeolith-Nanoantennen

Huub Maas、Gion Calzaferri2002-07-03Angewandte Chemie

Zapfenförmige Fluorophore an den Ausgängen von Zeolith-L-Kanälen können elektronische Anregungsenergie von Pyronin+-Molekülen im Innern des Kristalls abfangen (siehe Schema, oben). Den umgekehrten Vorgang, d. h. das Einspeisen elektronischer Anregungsenergie durch solche „Zapfen“ (unten), erreicht man mit Oxonin+-Mole…

Conducting polymers and applicationsPorphyrin and Phthalocyanine ChemistryLuminescence and Fluorescent Materials

Si−B−C−N Ceramic Precursors Derived from Dichlorodivinylsilane and Chlorotrivinylsilane. 2. Ceramization of Polymers and High-Temperature Behavior of Ceramic Materials

Anita Müller、Jiangqiang Peng、Hans Jürgen Seifert 等 5 位作者2002-07-03Chemistry of Materials

Starting from five different Si−B−C−N polymeric precursors with B/N atomic ratios ranging from 1:3 to 1:0.5, ceramic materials were synthesized by thermolysis at 1400 °C in about 70−75% yield. During this transformation, the Si/B/N ratio remained roughly constant, whereas H and C contents were reduced. The crystalliza…

Advanced ceramic materials synthesisMXene and MAX Phase MaterialsAdvanced materials and composites

Amyloid Architecture: Complementary Assembly of Heterogeneous Combinations of Three or Four Peptides into Amyloid Fibrils

Yuta Takahashi、Akihiko Ueno、Hisakazu Mihara2002-07-03ChemBioChem

The amyloid fibril is a misfolded and undesirable state for proteins that has been proposed to be a causative agent for a variety of fatal diseases known as amyloid diseases, such as Alzheimer's and prion diseases. However, the fibril has a highly ordered tertiary structure in which numerous beta-strand polypeptide ch…

Chemical Synthesis and AnalysisSupramolecular Self-Assembly in MaterialsClick Chemistry and Applications

5,10,15-Triaryl-21,23-dioxacorrole and Its Isomer with a Protruding Furan Ring

Miłosz Pawlicki、Lechosław Latos‐Grażyński、Ludmiła Szterenberg2002-07-03The Journal of Organic Chemistry

An oxa-analogue of 5,10,15-triarylcorrole, i.e., 5,10,15-triaryl-21,23-dioxacorrole (21,23-O(2)Cor)H, where two pyrrole rings are replaced by furan moieties, has been produced by condensation of 2,5-bis(arylhydroxymethyl)furan, 2-phenylhydroxymethylfuran, and pyrrole. 2-Phenylhydroxymethylfuran serves as the suitable…

Molecular Sensors and Ion DetectionPorphyrin and Phthalocyanine ChemistryLuminescence and Fluorescent Materials

An Umpolung Approach tocis-Hyponitrite Complexes

Navamoney Arulsamy、D. Scott Bohle、Jerome A. Imonigie 等 4 位作者2002-07-03Angewandte Chemie International Edition

Ligand formed by CN bond cleavage: Transition-metal-promoted heterolytic cleavage of the CN bond in 1 results in the formation of five new complexes of cis hyponitrite with Group 10 transition metals. The new complexes include [Ni(η2-O2N2)(dppf)] (dppf=1,1′-bis(diphenylphosphanyl)ferrocene) which is structurally cha…

Organometallic Complex Synthesis and CatalysisMetal complexes synthesis and propertiesMagnetism in coordination complexes