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Effects of inhomogeneous oxygen content in (La,Gd)0.7Ca0.3MnO3+δ perovskites

Jirong Sun、G.H. Rao、Y. Z. Zhang1998-06-15Applied Physics Letters

Magnetoresistance properties of compounds with the same formula La0.7−xGdxCa0.3MnO3+δ (x=0, 0.04) but synthesized by the solid-state reaction method from different starting materials are studied. Nearly stoichiometric compounds are obtained when La(OH)3 is used for sample preparation. However, under the same condition…

Magnetic and transport properties of perovskites and related materialsMultiferroics and related materialsAdvanced Condensed Matter Physics

Polymer surface chemistry and a novel attachment mechanism in corneal epithelial cells

Margaret D. M. Evans、John G. Steele1998-06-15Journal of Biomedical Materials Research

The initial attachment reaction of most cultured cell types to polymers is based on a linkage of integrin receptors to serum-derived fibronectin and vitronectin that adsorb onto the polymer surface. Recently isolated corneal epithelial cells have an additional attachment mechanism, known to operate on tissue culture p…

Polymer Surface Interaction StudiesOcular Surface and Contact LensCorneal Surgery and Treatments

Evidence for a Phase Transition in Glasses at Very Low Temperature: A Macroscopic Quantum State of Tunneling Systems?

Peter Strehlow、C. Enss、Siegfried Hunklinger1998-06-15Physical Review Letters

Dielectric measurements at very low temperature indicate that in the multicomponent glass $\mathrm{BaO}\ensuremath{-}{\mathrm{Al}}_{2}{\mathrm{O}}_{3}\ensuremath{-}{\mathrm{SiO}}_{2}$ a phase transition occurs at 5.84 mK. Below that temperature small magnetic fields of the order of $10\ensuremath{\mu}\mathrm{T}$ cause…

Material Dynamics and PropertiesGlass properties and applicationsTheoretical and Computational Physics

Ultraviolet photoabsorption measurements in alkali iodide and caesium bromide evaporated films

T. Boutboul、A. Breskin、R. Chechik 等 5 位作者1998-06-15Journal of Applied Physics

Ultraviolet–photon absorption constants were measured for thin CsI, KI, RbI, NaI and CsBr evaporated films, in the 140–200 nm spectral range. The constant measured for CsI is consistent with literature data; the absorption data for the other materials are given here for the first time. The absorption lengths for all m…

Luminescence Properties of Advanced MaterialsAdvanced Semiconductor Detectors and MaterialsElectronic and Structural Properties of Oxides

Ring formation and the structural and electronic properties of tetrahedral amorphous carbon surfaces

Jianjun Dong、D. A. Drabold1998-06-15Physical review. B, Condensed matter

In this paper, we report first-principles structural models of surfaces of tetrahedral amorphous carbon $(ta\ensuremath{-}\mathrm{C})$. The topology and defect structure of the amorphous surfaces are analyzed at the atomistic level. We examine the transition of the local bonding environment from the bulk to the surfac…

Graphene research and applicationsSemiconductor materials and devicesDiamond and Carbon-based Materials Research

Dielectric properties of oriented thin films of PbZrO3 on Si produced by pulsed laser ablation

Soma Chattopadhyay、Pushan Ayyub、V. R. Palkar 等 7 位作者1998-06-15Journal of Applied Physics

PbZrO 3 is an antiferroelectric perovskite with TC≈230 °C. We have deposited single phase, perfectly c-axis oriented thin films of PbZrO3 on Si(100) substrates by pulsed laser ablation at 700 °C. The growth conditions (substrate temperature, ambient oxygen pressure, and laser energy density) have been optimized and th…

Ferroelectric and Piezoelectric MaterialsAcoustic Wave Resonator TechnologiesElectronic and Structural Properties of Oxides

Random sequential adsorption on partially covered surfaces

Zbǐgniew Adamczyk、Paweł Weroński1998-06-15The Journal of Chemical Physics

The random sequential adsorption (RSA) approach was used to analyze adsorption of hard spheres at surfaces precovered with smaller sized particles. Numerical simulations were performed to determine the available surface function φl of larger particles for various particle size ratios λ=al/as and surface concentration…

Material Dynamics and PropertiesTheoretical and Computational PhysicsPolymer Surface Interaction Studies

Ab initiostudy of iron and iron hydride: II. Structural and magnetic properties of close-packed Fe and FeH

Christian Elsässer、Jing Zhu、Steven G. Louie 等 6 位作者1998-06-15Journal of Physics Condensed Matter

The energetical ordering and magnetic states of hexagonal and double-hexagonal close-packed (hcp, dhcp) as well as face-centred cubic (fcc) Fe and FeH crystals are studied via spin-polarized ab initio total-energy calculations in the local spin-density approximation and with generalized gradient corrections by means o…

Fusion materials and technologiesHydrogen Storage and MaterialsBoron and Carbon Nanomaterials Research

Rheological Response from Phase-Separated Domains as Studied by Shear Microscopy

Katsuo Matsuzaka、Tsuyoshi Koga、Takeji Hashimoto1998-06-15Physical Review Letters

The relation between rheological properties and phase-separated structures of polymer blend solutions is investigated by using the shear microscopy method to obtain insight into the mechanism of steady state formation under shear flow. The time dependence of viscosity and morphology is observed after a stepwise increa…

Polymer crystallization and propertiesPolymer Nanocomposites and PropertiesRheology and Fluid Dynamics Studies

Mesoscopic-scale dielectric relaxation at the glass transition

L. E. Walther、N. E. Israeloff、E. Vidal Russell 等 4 位作者1998-06-15Physical review. B, Condensed matter

Using scanning-probe-microscopy techniques, we have measured dielectric relaxation on ultrasmall, mesoscopic, length scales in a glassy polymer (polyvinyl acetate) film near its glass transition. The effective length scale sampled by these techniques is \ensuremath{\sim}50 nm. This is large enough to probe subsurface…

Material Dynamics and PropertiesGlass properties and applicationsForce Microscopy Techniques and Applications

A neutron scattering study of the quasi-one-dimensional conductor

J. E. Lorenzo、R. Currat、P. Monceau 等 6 位作者1998-06-15Journal of Physics Condensed Matter

The Peierls phase transition in the quasi-one-dimensional conductor is investigated by means of elastic and inelastic neutron scattering. The effective critical exponent , extracted from the temperature dependence of the integrated intensity from the CDW satellite reflections, is anomalously low, suggesting that the p…

Physics of Superconductivity and MagnetismOrganic and Molecular Conductors ResearchThermal Expansion and Ionic Conductivity

Colossal magnetoresistance in Gd1/2Sr1/2MnO3

B. Garcı́a-Landa、J. M. De Teresa、M. R. Ibarra 等 6 位作者1998-06-15Journal of Applied Physics

Colossal magnetoresistance has been observed in polycrystalline Gd0.5Sr0.5MnO3 perovskite. Irreversibility and sharp anomalies in the magnetostriction, magnetization, and magnetoresistance isotherms take place at low temperatures (<90 K), which have been attributed to the establishment of a charge-ordered state…

Magnetic and transport properties of perovskites and related materialsShape Memory Alloy TransformationsMultiferroics and related materials

Blackbody emission under laser excitation of silicon nanopowder produced by plasma-enhanced chemical-vapor deposition

J. Costa、P. Roura、J.R. Morante 等 4 位作者1998-06-15Journal of Applied Physics

Previous results concerning radiative emission under laser irradiation of silicon nanopowder are reinterpreted in terms of thermal emission. A model is developed that considers the particles in the powder as independent, so under vacuum the only dissipation mechanism is thermal radiation. The supralinear dependence ob…

Silicon Nanostructures and PhotoluminescenceNanowire Synthesis and ApplicationsLaser-Ablation Synthesis of Nanoparticles

Annealing behaviors of photoluminescence from SiOx:H

Zhixun Ma、Xianbo Liao、Jie He 等 7 位作者1998-06-15Journal of Applied Physics

The strong photoluminescence (PL) of SiOx:H prepared by plasma enhanced chemical vapor deposition has been systematically studied in conjunction with infrared and micro-Raman spectra. We have found that each PL spectrum is comprised of two Gaussian components, a main band and a shoulder. The main band might originate…

Thin-Film Transistor TechnologiesSilicon Nanostructures and PhotoluminescenceNanowire Synthesis and Applications

Green photoluminescence from Er-containing amorphous SiN thin films

A. R. Zanatta、L.A.O. Nunes1998-06-15Applied Physics Letters

Green light emission at room temperature was achieved from nonhydrogenated amorphous silicon–nitrogen (a-SiN) thin films. The films were deposited by cosputtering a silicon target covered with metallic erbium platelets in an Ar+N2 atmosphere. According to the deposition conditions, the nitrogen concentration [N] reach…

Semiconductor materials and devicesThin-Film Transistor TechnologiesSilicon Nanostructures and Photoluminescence

Atomic and electronic structures of large and small carbon tori

Vincent Meunier、Ph. Lambin、A. A. Lucas1998-06-15Physical review. B, Condensed matter

The stability of large carbon tori is examined within the elasticity theory. Tori of diameter larger than 200 nm obtained by bending a single-wall nanotube and connecting the two ends together are proved to be stable. Molecular mechanics is used for optimizing the structure of a small polygonal torus $({\mathrm{C}}_{1…

Carbon Nanotubes in CompositesGraphene research and applicationsDiamond and Carbon-based Materials Research

Prevention of calcification of glutaraldehyde-crosslinked porcine aortic cusps by ethanol preincubation: Mechanistic studies of protein structure and water-biomaterial relationships

Narendra Vyavahare、Danielle Hirsch、Eyal Lerner 等 7 位作者1998-06-15Journal of Biomedical Materials Research

Clinical usage of bioprosthetic heart valves (BPHVs) fabricated from glutaraldehyde-pretreated porcine aortic valves is restricted due to calcification-related failure. We previously reported a highly efficacious ethanol pretreatment of BPHVs for the prevention of cuspal calcification. The aim of the present study is…

Corrosion Behavior and InhibitionCultural Heritage Materials AnalysisCollagen: Extraction and Characterization

Mie scattering effects from monodispersed ZnS nanospheres

Stefan Scholz、R. Vacassy、Joydeep Dutta 等 5 位作者1998-06-15Journal of Applied Physics

Transmission spectra of monodispersed particles exhibit pronounced resonance features from which particle properties can be deduced. ZnS powders were used as model materials since they can be synthesized by homogeneous precipitation with a narrow size distribution. The optical extinction spectra can be simulated using…

Gold and Silver Nanoparticles Synthesis and ApplicationsQuantum Dots Synthesis And PropertiesSurfactants and Colloidal Systems

On-site Coulomb repulsion in the small polaron system La 1 − x Ca x MnO 3

D. C. Worledge、L. Miéville、T. H. Geballe1998-06-15Physical review. B, Condensed matter

Conductivity measurements from 300 to 1200 K of ${\mathrm{La}}_{1\ensuremath{-}x}{\mathrm{Ca}}_{x}{\mathrm{MnO}}_{3}$ thin films, with doping from $x=0$ to $x=1,$ show that the entire doping range fits the adiabatic small polaron model $\ensuremath{\sigma}=(A/T)\mathrm{exp}(\ensuremath{-}{E}_{a}/kT).$ Furthermore the…

Magnetic and transport properties of perovskites and related materialsAdvanced Condensed Matter PhysicsElectronic and Structural Properties of Oxides

Localized Mechanical Instabilities and Structural Transformations in Silica Glass under High Pressure

Daniel J. Lacks1998-06-15Physical Review Letters

Molecular simulations show that the structural transformations which occur in silica glass under high pressure do not require thermal activation, and arise from localized mechanical instabilities associated with disappearances of local minima on the potential energy surface. This result leads to the prediction that th…

High-pressure geophysics and materialsMaterial Dynamics and PropertiesGlass properties and applications