Materials Literature
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Linear and third-order nonlinear dielectric susceptibilities and the dielectric polarization were measured in $6.5∕65∕35$ lanthanum lead zirconate titanate (PLZT) hot-pressed ceramics. On cooling linear dielectric data show a transition from an ergodic to a nonergodic relaxor phase, while, on heating, a ferroelectric…
Anaerobic reaction of ferrous thiocyanate with the deprotonated form of the pentadentate dinucleating Schiff base 1,3-bis[(2-pyridylmethyl)imino]propan-2-ol (LH) yields the novel trinuclear [Fe3L2(NCS)4(H2O)] species 1. LH results from the bis-condensation of 2-acetyl-pyridine with 1,3-diaminopropan-2-ol and includes…
Changes in structure and phase transition behavior are investigated for two types of La-doped sodium bismuth titanate ceramics. When A-site vacancies are formed by La incorporation, the phase transition near 200 °C becomes pronounced. Hysteresis loop and ε(T) demonstrate that the structure above 200 °C is the incommen…
This work reports Raman spectroscopy measurements from single wall carbon nanotubes (SWNTs) addressing the nature of the $G$-band resonance Raman spectra. Experimental results on different samples are presented, i.e., aligned and misaligned SWNT samples, as well as isolated and bundled SWNTs. It is shown that the Rama…
A photochromic diarylethene with phenolic Schiff base 1a can be easily transformed to photochromic diarylethene with benzoxazole 3a in the conditions of base and phototrigger. Both of their photochromic properties are investigated. They show that the conversions of ring-open form to ring-closed form at photostationary…
A theory of the Stark effect in semiconductor quantum dots has been developed for the case of dominating polarization interaction of an electron and a hole with the nanocrystal surface. A shift of electron and hole quantum well levels in a nanocrystal in the interband absorption range in a uniform external electric fi…
Abstract Four monoamide derivatives of Gd−DTPA with alkyl chains consisting of 12, 14, 16, or 18 carbon atoms were synthesized. The gadolinium( III ) complexes with chain lengths of 14, 16 or 18 carbon atoms were efficiently incorporated into mixed micelles whereas the complex with a chain length of 12 carbon atoms wa…
The effect of hydrostatic pressure on the emission spectra and fluorescence lifetimes of ${\mathrm{Eu}}^{3+}$:lithium borate glass has been measured up to $32.6\phantom{\rule{0.3em}{0ex}}\text{GPa}$ at room temperature (RT) and up to $25.2\phantom{\rule{0.3em}{0ex}}\text{GPa}$ at $15\phantom{\rule{0.3em}{0ex}}\mathrm{…
Phonon-dispersion curves for a series of single-wall carbon nanotubes (SWCNT's) have been obtained by ab initio supercell approach. Force constants are calculated using norm-conserving pseudopotential plane-wave method in the framework of the density-functional theory and local-density approximation. Cumulant force-co…
Both $\mathrm{Cu}$ and $\mathrm{Fe}$ metals, with face-centered cubic (fcc) crystal structures, are nonmagnetic. However, the substitution of $\mathrm{Cu}$ atoms by Fe in the fcc-$\mathrm{Cu}$ lattice leads to the formation of a random solid solution and the appearance of ferromagnetic order, with a value of the magne…
Thio amino acids can be integrated into the backbone of peptides without significantly perturbing their structure. In this contribution we use ultrafast infrared and visible spectroscopy as well as state-of-the-art ab initio computations to investigate the photoisomerization of the trans form of N-methylthioacetamide…
Multistep reactions catalyzed by a covalently immobilized enzyme-cofactor-enzyme system were achieved. Lactate dehydrogenase (LDH), glucose dehydrogenase (GDH), and cofactor NADH were incorporated into two porous silica glass supports. One of the glass supports had pores of 30 nm in diameter, while the other was of 10…
Summary Morphological, geochemical and mineralogical studies were carried out in a representative soil catena of the low‐elevation plateaux of the upper Amazon Basin to interpret the steps and mechanisms involved in the podzolization of low‐activity clay soils. The soils are derived from Palaeozoic sandstones. They co…
Two new homologous series of bent-core compounds have been synthesized. Their mesophase behaviour has been investigated by polarizing microscopy, differential scanning calorimetry, X-ray diffraction, NMR spectroscopy, and by dielectric and electro-optical measurements. It was found that, with one exception, all the ch…
Monte Carlo simulations were performed to study the adsorption and orientation of antibodies on charged surfaces based on both colloidal and all-atom models. The colloidal model antibody consists of 12 connected beads representing the 12 domains of an antibody molecule. The structure of the all-atom antibody model was…
We have applied nanoporous anodic alumina films as planar optical waveguides and studied changes in the effective dielectric constants of these thin films due to various processes occurring in the pores. We demonstrate the potential of the porous anodic alumina waveguide for high sensitivity (bio-) chemical sensing wi…
Spinel-type ferrites are widely used in practical applications. A fascinating property of Zn-Ni ferrites which reveals a direction for application is reported. A large negative magnetoresistance effect has been observed in ZnFe2O4 and Ni substituted Zn1−xNixFe2O4 ferrites of spinel structure. These materials are eithe…
Gravitomagnetic charge that can also be referred to as the dual mass or magnetic mass is the topological charge in gravity theory. A gravitomagnetic monopole at rest can produce a stationary gravitomagnetic field. Due to the topological nature of gravitomagnetic charge, the metric of spacetime where the gravitomagneti…
We calculate the photoemission spectral function of the one-dimensional Hubbard model away from half filling using the dynamical density-matrix renormalization group method. An approach for calculating momentum-dependent quantities in finite open chains is presented. Comparison with exact Bethe ansatz results demonstr…
Recently introduced constitutive equations for the rheology of dense, disordered materials are investigated in the context of stick-slip experiments in boundary lubrication. The model is based on a generalization of the shear transformation zone (STZ) theory, in which plastic deformation is represented by a population…