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Computer generation of dense polydisperse sphere packings

Anuraag R. Kansal、Salvatore Torquato、Frank H. Stillinger2002-10-24The Journal of Chemical Physics

We present an extension of the Lubachevsky and Stillinger [J. Stat. Phys. 60, 561 (1990)] packing algorithm to generate packings of polydisperse spheres. The original Lubachevsky–Stillinger algorithm is a nonequilibrium protocol that allows a set of monodisperse spheres to grow slowly over time eventually reaching an…

Pickering emulsions and particle stabilizationMaterial Dynamics and PropertiesTheoretical and Computational Physics

Violation of Ioffe-Regel condition but saturation of resistivity of the high Tc cuprates

M. Calandra、O. Gunnarsson2002-10-24arXiv

We demonstrate that the resistivity data of a number of high Tc cuprates, in particular La(2-x)SrxCuO4, are consistent with resistivity saturation, although the Ioffe-Regel condition is strongly violated. By using the f-sum rule together with calculations of the kinetic energy in the t-J model, we show that the satura…

Materials ScienceStrongly Correlated Electrons

A low-dimensional spin S = 1/2 system at the quantum critical limit: Na2V2O7

J. L. Gavilano、D. Rau、S. Mushkolaj 等 6 位作者2002-10-24arXiv

We report the results of measurements of the dc-susceptibility and the 23Na-NMR response of Na2V2O7, a recently synthesized, non metallic low dimensional spin system. Our results indicate that upon reducing the temperature to below 100 K, the V^{4+} moments are gradually quenched, leaving only one moment out of 9 acti…

Strongly Correlated ElectronsMaterials Science

Diversity of order and densities in jammed hard-particle packings

Anuraag R. Kansal、Salvatore Torquato、Frank H. Stillinger2002-10-24Physical review. E, Statistical physics, plasmas, fluids, and related interdisciplinary topics

Recently the conventional notion of random close packing has been supplanted by the more appropriate concept of the maximally random jammed (MRJ) state. This inevitably leads to the necessity of distinguishing the MRJ state among the entire collection of jammed packings. While the ideal method of addressing this quest…

Granular flow and fluidized bedsComposite Material MechanicsMaterial Dynamics and Properties

Wireless LAN techniques for mobile instrument control

Joern Beckmann、Joerg Pulz2002-10-24arXiv

A choice of wireless technologies is available today. Not all of them are suitable to be used in a instrument control network at a neutron scattering facility. This paper will start with an overview of the wireless communication protocols IrDA, IEEE 802.11 WLAN, Bluetooth and protocols used by cellular phones. Afterwa…

Materials Science

c-Axis Intra-Layer Couplings in the CuO_2 Planes of High-T_c Cuprates

J. Röhler2002-10-24arXiv

We discuss the static deformations of the doped CuO_2 lattices in YBa_2Cu_3O_x. Intrinsic lattice effects driven by the strong correlations of the electron system are separated from extrinsic chemical and bandstructure effects. c-axis displacements of the planar copper atoms seem to be a generic property of the metall…

Materials ScienceSuperconductivityStrongly Correlated Electrons

User office proposal handling and analysis software

Joern Beckmann、Juergen Neuhaus2002-10-24arXiv

At FRM-II the installation of a user office software is under consideration, supporting tasks like proposal handling, beam time allocation, data handling and report creation. Although there are several software systems in use at major facilities, most of them are not portable to other institutes. In this paper the req…

Materials Science

Preparation and characterization of surface plasmon resonance tunable gold and silver films

Rajeev Gupta、Mark J. Dyer、Wayne A. Weimer2002-10-24Journal of Applied Physics

Precise control of thermal evaporation deposition parameters allows the reproducible production of silver and gold island films on glass substrates with tunable surface plasmon resonance wavelengths. Specific combinations of substrate temperature, deposition rate, and film thickness produce films exhibiting surface pl…

Optical Coatings and GratingsPlasmonic and Surface Plasmon ResearchGold and Silver Nanoparticles Synthesis and Applications

Electric-field-aligned growth of single-walled carbon nanotubes on surfaces

Ant Ural、Yiming Li、Hongjie Dai2002-10-24Applied Physics Letters

Aligned single-walled carbon nanotubes are grown onto the surfaces of SiO2/Si substrates in electric fields established across patterned metal electrodes. Calculations of the electric field distribution under the designed electrode structures, the directing ability of electric fields, and the prevention of surface van…

Carbon Nanotubes in CompositesGraphene research and applicationsMolecular Junctions and Nanostructures

Direct Observation of Percolation in a Manganite Thin Film

Liuwan Zhang、Casey Israel、Amlan Biswas 等 5 位作者2002-10-24OpenAlex

Upon cooling, the isolated ferromagnetic domains in thin films of La0.33Pr0.34Ca0.33MnO3 start to grow and merge at the metal-insulator transition temperature TP1, leading to a steep drop in resistivity, and continue to grow far below TP1. In contrast, upon warming, the ferromagnetic domain size remains unchanged unti…

Rare-earth and actinide compoundsAdvanced Condensed Matter PhysicsMagnetic and transport properties of perovskites and related materials

Flexoelectric polarization of barium strontium titanate in the paraelectric state

Wenhui Ma、L. E. Cross2002-10-24OpenAlex

The strain-gradient-induced polarization (flexoelectric effect) was investigated in Ba0.67Sr0.33TiO3 (BST) ceramic at temperatures above the 21 °C Curie point. At 23 °C the flexoelectric coefficient μ12 was more than one order of magnitude greater than the highest value measured in lead magnesium niobate ceramic. Over…

Nonlocal and gradient elasticity in micro/nano structuresFerroelectric and Piezoelectric MaterialsAcoustic Wave Resonator Technologies

Ideal Pure Shear Strength of Aluminum and Copper

Shigenobu Ogata、Ju Li、Sidney Yip2002-10-24OpenAlex

Although aluminum has a smaller modulus in [111]<112> shear than that of copper, we find by first-principles calculation that its ideal shear strength is larger because of a more extended deformation range before softening. This fundamental behavior, along with an abnormally high intrinsic stacking fault energy and a…

X-ray Diffraction in CrystallographyBoron and Carbon Nanomaterials ResearchMicrostructure and mechanical properties

CuO Nanowires Can Be Synthesized by Heating Copper Substrates in Air

Xuchuan Jiang、Thurston Herricks、Younan Xia2002-10-24OpenAlex

This paper describes a vapor-phase approach to the facial synthesis of cupric oxide (CuO) nanowires supported on the surfaces of various copper substrates that include grids, foils, and wires. A typical procedure simply involved the thermal oxidation of these substrates in air and within the temperature range from 400…

Electronic and Structural Properties of OxidesZnO doping and propertiesCopper-based nanomaterials and applications

Fluorescence Quenching of Dye Molecules near Gold Nanoparticles: Radiative and Nonradiative Effects

E. Dulkeith、Arne C. Morteani、T. Niedereichholz 等 10 位作者2002-10-24OpenAlex

The radiative and nonradiative decay rates of lissamine dye molecules, chemically attached to differently sized gold nanoparticles, are investigated by means of time-resolved fluorescence experiments. A pronounced fluorescence quenching is observed already for the smallest nanoparticles of 1 nm radius. The quenching i…

Gold and Silver Nanoparticles Synthesis and ApplicationsProtein Interaction Studies and Fluorescence AnalysisPhotochemistry and Electron Transfer Studies

Small-angle x-ray scattering measurements of hydrogen evolution from an epitaxial Nb film

Brent J. Heuser、Monica M. C. Allain、Wangchun Chen2002-10-23Physical review. B, Condensed matter

Small-angle x-ray scattering (SAXS) measurements have been performed to investigate particle morphology during in situ hydrogen evolution from a 1000-\AA{} epitaxial Nb film on $(112\ifmmode\bar\else\textasciimacron\fi{}0)$ sapphire initially loaded to saturation with hydrogen. The SAXS intensity follows the plate or…

Copper Interconnects and ReliabilityMetal and Thin Film MechanicsPhysics of Superconductivity and Magnetism

Polyaniline emeraldine base in N‐methyl‐2‐pyrrolidinone containing secondary amine additives: A rheological investigation of solutions

Dali Yang、Benjamin R. Mattes2002-10-23Journal of Polymer Science Part B Polymer Physics

Abstract From a rheological study of emeraldine base (EB)/ N ‐methyl‐2‐pyrrolidinone (NMP)/2‐methyl‐aziridine (2MA) solutions, a correlation between the solution concentration and solution viscosity was found. We investigated the rheokinetic mechanism of the EB dissolution process and determined the reaction rate, act…

Conducting polymers and applicationsAnalytical Chemistry and SensorsSynthesis and properties of polymers

Structure and Properties of γ-Brass-Type Pt2Zn11—δ (0.2 < δ < 0.3)

Bernd Harbrecht、Srinivasa Thimmaiah、Marc Armbrüster 等 5 位作者2002-10-23Zeitschrift für anorganische und allgemeine Chemie

The γ-brass type phase Pt2Zn11—δ (0.2 < δ < 0.3) was prepared by reaction of the elements in evacuated silica ampoules. The structures of crystals grown in the presence of excess zinc or alternatively excess platinum were determined from single crystal X-ray diffraction intensities and confirmed by Rietveld profile fi…

Nanoporous metals and alloysQuasicrystal Structures and PropertiesMetallurgy and Material Science

Radiochemical Yields for Cross-Links and Branches in Radiation-Modified Poly(tetrafluoroethylene)

Beate Fuchs、Uwe Lappan、K. Lunkwitz 等 4 位作者2002-10-23Macromolecules

For the enhancement of the compatibility of fluoropolymers with other materials radiation modification is applied, for which irradiation with high-energy electrons provides an efficient and flexible possibility. Poly(tetrafluoroethylene) (PTFE) is known to predominantly undergo chain scission under irradiation. To cou…

Polymer Nanocomposite Synthesis and IrradiationPolymer Nanocomposites and PropertiesSilicone and Siloxane Chemistry

Ferromagnetic Domain Structures and Nanoclusters inNd1/2Sr1/2MnO3

Toru Asaka、Y. Anan、Takuro Nagai 等 8 位作者2002-10-23Physical Review Letters

Magnetic domain structures of $\mathrm{N}{\mathrm{d}}_{\mathrm{1}\mathrm{/}\mathrm{2}}\mathrm{S}{\mathrm{r}}_{\mathrm{1}\mathrm{/}\mathrm{2}}\mathrm{M}\mathrm{n}{\mathrm{O}}_{\mathrm{3}}$ were investigated by means of low-temperature Lorentz electron microscopy. On cooling, magnetic domain walls started to appear at 2…

Magnetic and transport properties of perovskites and related materialsHigh-pressure geophysics and materialsAdvanced Condensed Matter Physics

Microphase Separation inPr0.67Ca0.33MnO3by Small-Angle Neutron Scattering

Ch. Simon、Silvana Mercone、Nicolas Guiblin 等 6 位作者2002-10-23Physical Review Letters

We have evidenced by small-angle neutron scattering at low temperature the coexistence of ferromagnetism (F) and antiferromagnetism (AF) in ${\mathrm{P}\mathrm{r}}_{0.67}\mathrm{C}{\mathrm{a}}_{\mathrm{0.33}}\mathrm{M}\mathrm{n}{\mathrm{O}}_{\mathrm{3}}$. The results are compared to those obtained in ${\mathrm{P}\math…

Rare-earth and actinide compoundsMagnetic Properties of AlloysMagnetic and transport properties of perovskites and related materials