Materials Literature
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Abstract Controlling liquid adhesion is a fundamental issue in many applications for special wettable surfaces. Compared to superhydrophobic surfaces of different water adhesion, superoleophobic surfaces of controllable oil adhesion are much more practical, as it leads to non‐wetting for both water and oil. However, p…
Shaped and dimpled: Silver nanocrystals enclosed by concave surfaces and thus high-index facets have been prepared by simply controlling the growth habit of Ag cubic seeds. Four types of concave nanocrystals, including octahedron, cube, octapod, and trisoctahedron, were obtained (see picture).
Self-compensation, the tendency of a crystal to lower its energy by forming point defects to counter the effects of a dopant, is here quantitatively proven. Based on a new theoretical formalism and several different experimental techniques, we demonstrate that the addition of 1.4 \ifmmode\times\else\texttimes\fi{} 10$…
An overview of the behavior of Fe-based superconductors (FBSs) in magnetic fields is given with the emphasis on the materials features important for pinning of vortices, critical current densities, melting of the vortex structures and the upper critical fields. We also discuss how the multiband electronic structure of…
BACKGROUND: Degeneration of xenografts or homografts is a major cause for reoperation in young patients after pulmonary valve replacement. We present the early results of fresh decellularized pulmonary homografts (DPH) implantation compared with glutaraldehyde-fixed bovine jugular vein (BJV) and cryopreserved homograf…
Ultrafine metal-oxide-decorated hybrid carbon nanofibers (CNFs) were fabricated by a single-nozzle co-electrospinning process using a phase-separated mixed polymer composite solution and heat treatment. To decorate metal oxides on the CNF surface, core (PAN) and shell (PVP) structured nanofibers (NFs) were fabricated…
The ability of diamond nanoparticles (nanodiamonds, NDs) to deliver small interfering RNA (siRNA) into Ewing sarcoma cells is investigated with a view to the possibility of in-vivo anticancer nucleic-acid drug delivery. siRNA is adsorbed onto NDs that are coated with cationic polymer. Cell uptake of NDs is demonstrate…
We have developed a method for prediction of the hardest crystal structures in a given chemical system. It is based on the evolutionary algorithm USPEX (Universal Structure Prediction: Evolutionary Xtallography) and electronegativity-based hardness model that we have augmented with bond-valence model and graph theory.…
Understanding and predicting the behavior of water, especially in contact with various surfaces, is a scientific challenge. Molecular-level understanding of hydrophobic effects and their macroscopic consequences, in particular, is critical to many applications. Macroscopically, a surface is classified as hydrophilic o…
This tutorial review presents emerging lines of investigations directed towards the development of dynamic combinatorial materials and devices. These can be defined as multi-component chemical systems which, thanks to the reversibility of their interconnections within networks of competing reactions, and thanks to the…
Abstract Novel ordered hierarchical mesoporous/microporous carbon (OHMMC) derived from mesoporous titanium‐carbide/carbon composites was prepared for the first time by synthesizing ordered mesoporous nanocrystalline titanium‐carbide/carbon composites, followed by chlorination of titanium carbides. The mesostructure an…
A universal mechanism that controls the zero thermal expansion (ZTE) behavior of the antiperovskite manganese nitrides is discovered. Modulating the Mn occupancy at its lattice sites leads to a drastic change in the thermal expansion behavior. The Mn site occupancy can be reduced by nanostructuring the material, gener…
We demonstrate the design of composite plasmonic metal/semiconductor photocatalysts, which show enhanced visible light photocatalytic activity compared to the semiconductor alone. We show that the overlap between the illumination source spectrum, semiconductor absorbance spectrum and metal nanoparticle surface plasmon…
We report a proof-of-concept demonstration of negative capacitance effect in a nanoscale ferroelectric-dielectric heterostructure. In a bilayer of ferroelectric Pb(Zr0.2Ti0.8)O3 and dielectric SrTiO3, the composite capacitance was observed to be larger than the constituent SrTiO3 capacitance, indicating an effective n…
ZnO is a promising high figure-of-merit (ZT) thermoelectric material for power harvesting from heat due to its high melting point, high electrical conductivity σ, and Seebeck coefficient α, but its practical use is limited by a high lattice thermal conductivity κ(L). Here, we report Al-containing ZnO nanocomposites wi…
Supramolecular polymer networks are three-dimensional structures of crosslinked macromolecules connected by transient, non-covalent bonds; they are a fascinating class of soft materials, exhibiting properties such as stimuli-responsiveness, self-healing, and shape-memory. This critical review summarizes the current st…
The principles of operation of permanent magnets are summarized, and their development is reviewed. The key figure of merit, the energy product, improved exponentially over much of the 20th century, doubling roughly every 12 years. Yet it has not improved significantly in the last 20 years. Constraints on further deve…
<div class="section abstract"><div class="htmlview paragraph">In 2011-2013, regulations will be tightened for non-road vehicles, via the application of Stage III-B standards in Europe. With state-of-the-art technology (high pressure common rail, cooled EGR), non-road diesel engines will require DPFs to con…
Pseudomonas aeruginosa synthesizes phosphorylcholine phosphatase (PchP) when grown on choline, betaine, dimethylglycine or carnitine. In the presence of Mg(2+) or Zn(2+), PchP catalyzes the hydrolysis of p-nitrophenylphosphate (p-NPP) or phosphorylcholine (Pcho). The regulation of pchP gene expression is under the con…
<div class="section abstract"><div class="htmlview paragraph">Computer simulation is now considered to be a crucial stage in the design of automotive catalysts due to the increasing complexity of modern aftertreatment systems. The resulting models almost invariably include surface reaction kinetics that ar…