Materials Literature
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We investigate theoretically the spin splitting of the exciton states in semiconductor coupled quantum dots (CQDs) containing a single magnetic ion. We find that the spin splitting can be switched on/off in the CQDs \textit{via} the \textit{sp-d}exchange interaction using the electric field. An interesting bright-to-d…
The Laves phase compound, YCo2, is a well-known exchange-enahnced Pauli paramagnet. We report here that, in the nanocrystalline form, this compound interestingly is an itinerant ferromagnet at room temperature with a low coercive-field. The magnitude of the saturation moment (about 1 Bohr-magneton per formula unit) is…
The preparation of a homogeneous series of chitin/chitosan oligomers (chito-oligomers) with the same distribution of degrees of polymerization (DP) ranging from 2 to 12, but with various average degrees of N-acetylation (DA) from 0 to 90% is described. This DA-series was obtained according to a two-step chemical proce…
We report the influence of an Al(2)O(3) shell on the photoluminescence emission of ZnO nanowires. At room temperature, the spectrum of the core-shell nanowires shows a strong reduction of the relative intensity of the green defect emission with respect to the near-band-edge emission. At 5 K an increase of the relative…
Electrochromic polymers (ECPs) of tunable green: Two symmetrical donor-acceptor based oligomers were designed, synthesized and chemically polymerized affording solution-processable conjugated polymers of distinct green hues in their neutral state. The polyheterocyclic hybrids exhibited highly transmissive oxidized sta…
The spreading of liquid drops on surfaces corrugated with micrometer-scale parallel grooves is studied both experimentally and numerically. Because of the surface patterning, the typical final drop shape is no longer spherical. The elongation direction can be either parallel or perpendicular to the direction of the gr…
The compound, LaMn2Ge2, crystallizing in ThCr2Si2-type tetragonal crystal structure, has been known to undergo ferromagnetic order below (T_C=) 326 K. In this article, we report the magnetic behavior of nanocrystalline form of this compound, obtained by high-energy ball-milling. T_C of this compound is reduced maginal…
We have studied ultrafast photoinduced demagnetization in GaMnAs via two-color time-resolved magneto-optical Kerr spectroscopy. Below band gap midinfrared pump pulses strongly excite the valence band, while near-infrared probe pulses reveal subpicosecond demagnetization that is followed by an ultrafast $(\ensuremath{\…
A surface distribution of the electroluminescence intensity of silicon p-n light emitting diodes is obtained under space scanning experiments at room temperature. An emitting surface of the diodes, represented by a few small bright emitting dots and a weakly emitting area outside the dots, serves as a direct evidence…
We report a large entropy change (DeltaS) below 300 K, peaking near TC= 220 K, due to isothermal change of magnetic field, for Gd4Co3, with a refrigeration capacity higher than that of Gd. Notably, the isothermal magnetization is nonhysteretic - an important criterion for magnetic refrigeration without loss. DeltaS be…
The formation and stability of a shear-induced shish-kebab structure was investigated by in situ rheo-SAXS (small-angle X-ray scattering) and -WAXD (wide-angle X-ray diffraction) measurements of highly entangled polyethylene melts based on two polymer blends, containing small fractions (2 and 5 wt %) of ultra-high mol…
Emulsions stabilized through the adsorption of colloidal particles at the liquid-liquid interface have long been used and investigated in a number of different applications. The interfacial adsorption of particles can be induced by adjusting the particle wetting behavior in the liquid media. Here, we report a new appr…
We derive the Schrödinger equation for a spinless charged particle constrained to move on a curved surface in the presence of an electric and magnetic field. The particle is confined on the surface using a thin-layer procedure, which gives rise to the well-known geometric potential. The electric and magnetic fields ar…
We apply continuum connectedness percolation theory to realistic carbon nanotube systems and predict how bending flexibility, length polydispersity, and attractive interactions between them influence the percolation threshold, demonstrating that it can be used as a predictive tool for designing nanotube-based composit…
We demonstrate a direct correlation between the domain structure of multiferroic BiFeO3 thin films and exchange bias of Co 0.9Fe 0.1/BiFeO3 heterostructures. Two distinct types of interactions - an enhancement of the coercive field ( exchange enhancement) and an enhancement of the coercive field combined with large sh…
The effect of phenols reactivity with formaldehyde on the formation of ordered mesoporous carbons has been investigated. A strategy to accelerate the polymerization of phenolic resins by using strongly acidic conditions is proposed. The self-assembly of resorcinol-formaldehyde and block copolymers (e.g., F127) under h…
A procedure for preparing individualized chitin nanofibers 3-4 nm in cross-sectional width and at least a few microns in length was developed. The key factors to prepare the chitin nanofibers with such high aspect ratios are as follows: (1) squid pen beta-chitin is used as the starting material and (2) ultrasonication…
The molecular formulas and charge state distributions of thus-far known ubiquitous alkanethiolate-protected gold clusters with core-masses of 8 and 29 kDa were assessed using electrospray ionization mass spectrometry. The 8 and 29 kDa clusters were determined to be composed of single species, [Au38(SCn)24]z and [Au144…
If graphene is ever going to live up to the promises of future nanoelectronic devices, an easy and cheap route for mass production is an essential requirement. A way to extend the capabilities of plasma-enhanced chemical vapour deposition to the synthesis of freestanding few-layer graphene is presented. Micrometre-wid…
Multitasking rust ball: The questions of where a tumor is located, whether drugs are properly delivered to the tumor, and what the therapeutic response of the tumor is, could be answered by using simple but smart, drug-loaded superparamagnetic iron oxide nanoparticles that can accumulate in tumor with high efficiency…