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第 182355 / 188563 页 · 当前展示 3,647,081–3,647,100 / 3,771,245 条匹配结果 · 摘要仅作预览

Polymers at Interfaces: Using Atom Transfer Radical Polymerization in the Controlled Growth of Homopolymers and Block Copolymers from Silicon Surfaces in the Absence of Untethered Sacrificial Initiator

Krzysztof Matyjaszewski、Peter J. Miller、Nisha Shukla 等 11 位作者1999-12-01OpenAlex

The atom transfer radical polymerization (ATRP) of styrene and acrylates from silicon wafers modified with an initiator layer composed of 2-bromoisobutyrate fragments is described. In the presence of the proper ratio of activating and deactivating transition-metal species, controlled radical polymerizations of styrene…

Advanced Polymer Synthesis and CharacterizationConducting polymers and applicationsPolymer Surface Interaction Studies

Phase-field model for binary alloys

Seong Gyoon Kim、Won Tae Kim、Toshio Suzuki1999-12-01OpenAlex

We present a phase-field model (PFM) for solidification in binary alloys, which is found from the phase-field model for a pure material by direct comparison of the variables for a pure material solidification and alloy solidification. The model appears to be equivalent with the Wheeler-Boettinger-McFadden (WBM) model…

Metallurgical Processes and ThermodynamicsSolidification and crystal growth phenomenaAluminum Alloy Microstructure Properties

The mechanical design of spider silks: from fibroin sequence to mechanical function

John M. Gosline、Paul A. Guerette、Christine Ortlepp 等 4 位作者1999-12-01OpenAlex

Spiders produce a variety of silks, and the cloning of genes for silk fibroins reveals a clear link between protein sequence and structure-property relationships. The fibroins produced in the spider's major ampullate (MA) gland, which forms the dragline and web frame, contain multiple repeats of motifs that include an…

Spider Taxonomy and Behavior StudiesSilk-based biomaterials and applicationsBiochemical and Structural Characterization

Structure of Spinel

Kurt E. Sickafus、J. M. Wills、N. W. Grimes1999-12-01OpenAlex

This paper reviews the crystal structure of compounds with the general formula AB 2 X 4 , which crystallize with the same atomic structure as the mineral spinel, MgAl 2 O 4 . Three degrees of freedom associated with the detailed atomic arrangements of spinels are considered here: (i) the lattice parameter, a ; (ii) th…

Crystal Structures and PropertiesX-ray Diffraction in CrystallographyAdvanced Condensed Matter Physics

Electrical, optical, and structural properties of indium–tin–oxide thin films for organic light-emitting devices

Heungsoo Kim、C. M. Gilmore、Alberto Piqué 等 8 位作者1999-12-01OpenAlex

High-quality indium–tin–oxide (ITO) thin films (200–850 nm) have been grown by pulsed laser deposition (PLD) on glass substrates without a postdeposition annealing treatment. The structural, electrical, and optical properties of these films have been investigated as a function of target composition, substrate depositi…

GaN-based semiconductor devices and materialsChalcogenide Semiconductor Thin FilmsZnO doping and properties

Phase separation in confined systems

Lev D. Gelb、Keith E. Gubbins、Ravi Radhakrishnan 等 4 位作者1999-12-01OpenAlex

We review the current state of knowledge of phase separation and phase equilibria in porous materials. Our emphasis is on fundamental studies of simple fluids (composed of small, neutral molecules) and well-characterized materials. While theoretical and molecular simulation studies are stressed, we also survey experim…

Mesoporous Materials and CatalysisBlock Copolymer Self-AssemblyMaterial Dynamics and Properties

Syntheses, Structures, and Theoretical Study of LaCuSTe and SmCuSTe

Fu Qiang Huang、James A. Ibers1999-11-30Inorganic Chemistry

Two mixed-chalcogen compounds LaCuSTe and SmCuSTe have been synthesized by the reactions of the elements at 1123 K. LaCuSTe crystallizes in a cell of dimensions a = 6.4955(8) Å, b = 7.7692(9) Å, c = 7.4665(9) Å, and beta = 95.045(2) degrees (T = 153 K) with four formula units in space group C(2)(h)()(5)-P2(1)/c of the…

Rare-earth and actinide compoundsIron-based superconductors researchInorganic Chemistry and Materials

Blends of Biodegradable Thermoplastics with Lignin Esters

Indrajit Ghosh、Rajesh K. Jain、Wolfgang G. Glasser1999-11-30ACS symposium series

Thermoplastic blends of several biodegradable polymers with lignin and lignin esters were prepared by solvent casting and melt processing. Among the biodegradable thermoplastics were cellulose acetate butyrate (CAB), a starch-caprolactone copolymer/blend (SCC), and poly(hydroxybutyrate) (PHB). Lignin esters included t…

Lignin and Wood ChemistryAdvanced Cellulose Research Studiesbiodegradable polymer synthesis and properties

Molybdate- and Tungstate-Exchanged Layered Double Hydroxides as Catalysts for 1O2 Formation: Characterization of Reactive Oxygen Species and a Critical Evaluation of 1O2 Detection Methods

Bert F. Sels、Dirk De Vos、Piet J. Grobet 等 6 位作者1999-11-30The Journal of Physical Chemistry B

Layered double hydroxides (LDHs) with the formula [Mg 0.7 Al 0.3 (OH) 2 ](NO 3 ) 0.3 were partially exchanged with MoO 4 2- and WO 4 2- and were used as heterogeneous catalysts for the decomposition of H 2 O 2 into singlet molecular oxygen ( 1 O 2 ). The oxometalate anions are present on the LDH as monomeric, tetrahed…

Layered Double Hydroxides Synthesis and ApplicationsPolyoxometalates: Synthesis and ApplicationsAdvanced Photocatalysis Techniques

Mesoporous Magnetic Materials Based on Rare Earth Oxides

Mitsunori Yada、Hirohumi Kitamura、Akira Ichinose 等 5 位作者1999-11-30Angewandte Chemie International Edition

A novel family of mesoporous oxides of rare earth metals (Gd, Tb, Dy, Ho, Er, Tm, Yb, Lu) were synthesized with specific surface areas of 253-348 m(2) g(-1) and pore diameters of 2.5-3.0 nm (see Scheme). The mesoporous solids and their surfactant mesophase precursors are paramagnetic and exhibit a magnetic anomaly due…

Supercapacitor Materials and FabricationLayered Double Hydroxides Synthesis and ApplicationsMesoporous Materials and Catalysis

Self-Assembly of a Radially Functionalized Hexagonal Molecule: Hexakis(4-hydroxyphenyl)benzene

Kenji Kobayashi、Toshiaki Shirasaka、Azumi Sato 等 5 位作者1999-11-30Angewandte Chemie International Edition

Two different porous hydrogen-bonded networks are formed by self-assembly of the radially substituted host 1. In the network of type A, formed by 1 small middle dot4 Et(2)O, all OH groups of 1 are involved in hydrogen bonding, and the molecular sheets are stacked without translation to generate extended channels that…

Mesoporous Materials and CatalysisMetal-Organic Frameworks: Synthesis and ApplicationsSupramolecular Self-Assembly in Materials

Using Liquid Crystals To Image Reactants and Products of Acid−Base Reactions on Surfaces with Micrometer Resolution

Rahul R. Shah、Nicholas L. Abbott1999-11-30Journal of the American Chemical Society

We report that nematic liquid crystals (LCs) of 4-cyano-4‘-pentylbiphenyl (5CB) and p -methoxybenzylidene- p - n -butylaniline (MBBA) can be used to image reactants and products of reversible, acid−base reactions on surfaces with micrometer resolution. When supported on obliquely deposited films of gold, azimuthal ori…

Surfactants and Colloidal SystemsLiquid Crystal Research AdvancementsPhotonic Crystals and Applications

Enantioselective Single-Crystal-to-Single-Crystal Photodimerization of Coumarin and Thiocoumarin in Inclusion Complexes with Chiral Host Compounds

Koichi Tanaka、Fumio Toda、Eiko Mochizuki 等 7 位作者1999-11-30Angewandte Chemie International Edition

An intermolecular enantioselective photoreaction by a single-crystal-to-single-crystal transformation has been carried out for the first time, as is evident from X-ray structure analysis and X-ray powder diffractometric studies. This reaction, the dimerization of the title compound to cyclobutane derivative 1 (X=O, S)…

Crystallization and Solubility StudiesCrystallography and molecular interactionsPhotochromic and Fluorescence Chemistry

Molecular Magnetic Sponges

Olivier Kahn、Joulia Larionova≠、J. V. Yakhmi1999-11-30Chemistry - A European Journal

Reversible release or reabsorption of water like sponges, a process which is accompanied by a dramatic change of structure and magnetic properties, can be achieved by some molecular magnetic materials. When the sponges are hydrated, or wet, the structure consists of isolated units with a nonmagnetic ground state. When…

Magnetism in coordination complexesPorphyrin and Phthalocyanine ChemistryLanthanide and Transition Metal Complexes

Chlorine adsorption on the Cu(111) surface

K. Doll、N. M. Harrison1999-11-30arXiv

We investigate the adsorption of chlorine on the Cu(111) surface with full potential all-electron density functional calculations. Chlorine adsorption at the fcc hollow sites is slightly preferred over that at the hcp hollow. The adsorption geometry is in excellent agreement with electron diffraction and ion scatterin…

Materials Science

Wannier-functions characterization of floating bonds in a-Si

M. Fornari、N. Marzari、M. Peressi 等 4 位作者1999-11-30arXiv

We investigate the electronic structure of over-coordinated defects in amorphous silicon via density-functional total-energy calculations, with the aim of understanding the relationship between topological and electronic properties on a microscopic scale. Maximally-localized Wannier functions are computed in order to…

Materials Science