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Spin spectroscopy of dark excitons in CdSe quantum dots to 60 T

Ezekiel Johnston‐Halperin、D. D. Awschalom、S. A. Crooker 等 7 位作者2001-04-24Physical review. B, Condensed matter

Polarization-resolved magnetophotoluminescence spectroscopy is used to study exciton spin states in 40--80 \AA{} diameter chemically synthesized CdSe quantum dots (QDs) at temperatures $T=1.2--50\mathrm{K}.$ The spin polarization is found not to saturate in magnetic fields to 60 T and time-resolved studies indicate a…

Semiconductor Quantum Structures and DevicesQuantum Dots Synthesis And PropertiesChalcogenide Semiconductor Thin Films

Examinations on the Critical and Primary Crystallite Sizes during θ- to α-Phase Transformation of Ultrafine Alumina Powders

Pei-Ling Chang、Fu‐Su Yen、Kung-Chieh Cheng 等 4 位作者2001-04-24Nano Letters

Examination on the existence of the critical and primary crystallite size ( d c α ∼ 17 nm and d p = 50−55 nm) phenomena during θ- to α-phase transformation of the nanosized Al 2 O 3 powder was designed and conducted using two θ-Al 2 O 3 powders of different crystallite sizes. Due to the critical size, the size depende…

Advanced ceramic materials synthesisAluminum Alloys Composites PropertiesX-ray Diffraction in Crystallography

Effect of surface roughness on the universal thermal conductance

D. H. Santamore、M. C. Cross2001-04-24Physical review. B, Condensed matter

We explain the reduction of the thermal conductance below the predicted universal value observed by Schwab et al. [Nature (London) 404, 974 (2000)] in terms of the scattering of thermal phonons off surface roughness using a scalar model for the elastic waves. Our analysis shows that the thermal conductance depends on…

Thermal properties of materialsAdvanced Thermodynamics and Statistical MechanicsThermal Radiation and Cooling Technologies

Protein crystallization by rational mutagenesis of surface residues: Lys to Ala mutations promote crystallization of RhoGDI

Kenton L. Longenecker、Sarah Garrard、Peter Sheffield 等 4 位作者2001-04-24Acta Crystallographica Section D Biological Crystallography

Crystallization is a unique process that occurs at the expense of entropy, including the conformational entropy of surface residues, which become ordered in crystal lattices during formation of crystal contacts. It could therefore be argued that epitopes free of amino acids with high conformational entropy are more th…

Protein Structure and DynamicsEnzyme Structure and FunctionBiochemical and Molecular Research

Enzymatic Hydrolysis of Poly(lactide)s: Effects of Molecular Weight, l-Lactide Content, and Enantiomeric and Diastereoisomeric Polymer Blending

Hideto Tsuji、Shinya Miyauchi2001-04-24Biomacromolecules

Nonblended poly(L-lactide) (PLLA) films having different molecular weights and nonblended poly(lactide) (PLA) films, enantiomeric blend films from PLLA and poly(D-lactide) (PDLA), and diastereoisomeric blend films of poly(DL-lactide) (PDLLA) with either PLLA or PDLA, having different L-lactide (LLA) contents (X(LLA)s)…

biodegradable polymer synthesis and propertiesElectrospun Nanofibers in Biomedical ApplicationsGraphene and Nanomaterials Applications

Electrical relaxations: Simple versus complex ionic systems

A. S. Nowick、Byeong Soo Lim2001-04-24Physical review. B, Condensed matter

Complex materials are known to show two regions of ac electrical behavior. In the high-temperature/low-frequency domain, they show power-law frequency dependence of the conductivity known as ``universal dielectric response,'' or UDR, while at low temperatures/high frequencies they show ``nearly constant loss,'' or NCL…

Ferroelectric and Piezoelectric MaterialsHigh-pressure geophysics and materialsSolid-state spectroscopy and crystallography

Origin of high transport spin polarization inLa0.7Sr0.3MnO3:Direct evidence for minority spin states

B. Nadgorny、I. I. Mazin、M. S. Osofsky 等 10 位作者2001-04-24Physical review. B, Condensed matter

Using the point-contact Andreev reflection technique, we have carried out a systematic study of the spin polarization in the colossal magnetoresistive manganite, ${\mathrm{La}}_{0.7}{\mathrm{Sr}}_{0.3}{\mathrm{MnO}}_{3}$ (LSMO). Surprisingly, we observed a significant increase in the current spin polarization with the…

Magnetic and transport properties of perovskites and related materialsAdvanced Condensed Matter PhysicsElectronic and Structural Properties of Oxides

Electrical current distribution across a metal-insulator-metal structure during bistable switching

C. Rossel、G. I. Meijer、D. Bremaud 等 4 位作者2001-04-24arXiv

Combining scanning electron microscopy (SEM) and electron-beam-induced current (EBIC) imaging with transport measurements, it is shown that the current flowing across a two-terminal oxide-based capacitor-like structure is preferentially confined in areas localized at defects. As the thin-film device switches between t…

Materials Science

A simple one-dimensional model of heat conduction which obeys Fourier's law

Pedro L. Garrido、Pablo I. Hurtado、Bjoern Nadrowski2001-04-24arXiv

We present the computer simulation results of a chain of hard point particles with alternating masses interacting on its extremes with two thermal baths at different temperatures. We found that the system obeys Fourier's law at the thermodynamic limit. This result is against the actual belief that one dimensional syst…

Materials Sciencecond-mat.stat-mech

Sharp interface limit of a phase-field model of crystal grains

Alexander E. Lobkovsky、James A. Warren2001-04-24Physical review. E, Statistical physics, plasmas, fluids, and related interdisciplinary topics

We analyze a two-dimensional phase field model designed to describe the dynamics of crystalline grains. The phenomenological free energy is a functional of two order parameters. The first one reflects the orientational order, while the second reflects the predominantally local orientation of the crystal. We consider t…

Solidification and crystal growth phenomenaAdvanced Mathematical Modeling in Engineeringnanoparticles nucleation surface interactions

two-waves approximation for reflected and transmitted energy in photonic crystals

B. Guizal、D. Felbacq、R. Smaali2001-04-24arXiv

We study electromagnetic waves scattering by a 2D photonic crystal made of a stack of diffraction gratings. In case where there are only two propagative modes in the crystal, we derive an explicit expression for the superior (resp. inferior) envelope of the reflected (resp. transmitted) energy.

Materials Science

Strong ferromagnetism and weak antiferromagnetism in double perovskites:Sr2FeMO6(M=Mo,W, and Re)

Zhilai Fang、K. Terakura、Junjiro Kanamori2001-04-24Physical review. B, Condensed matter

Double perovskites ${\mathrm{Sr}}_{2}\mathrm{Fe}M{\mathrm{O}}_{6}$ $(M=\mathrm{Mo}$ and Re) exhibit significant colossal magnetoresistance even at room temperature due to the high Curie temperatures (419 and 401 K). However, such a high Curie temperature is puzzling, given the large separation between magnetic element…

Magnetic and transport properties of perovskites and related materialsAdvanced Condensed Matter PhysicsThermal Expansion and Ionic Conductivity

Enhanced rigidity of recycled polypropylene from packaging waste by compounding with talc and high‐ crystallinity polypropylene

Stefan Tall、Ann‐Christine Albertsson、Sigbritt Karlsson2001-04-23Polymers for Advanced Technologies

Abstract Polypropylene (PP) constituted 30% of the collected material in a Swedish collection system for rigid plastic packaging waste. The PP fraction was however a complex mixture of grades with widely different properties. In order to enhance the rigidity of the recycled PP, modified grades were prepared by compoun…

Polymer crystallization and propertiesMicroplastics and Plastic PollutionRecycling and Waste Management Techniques

Orientations of side chains and adsorbed liquid crystal molecules on a rubbed polyimide surface studied by optical second harmonic generation

Seok‐Cheol Hong、Masahito Oh‐e、Xiaowei Zhuang 等 7 位作者2001-04-23Physical review. E, Statistical physics, plasmas, fluids, and related interdisciplinary topics

Surface second harmonic generation was used to obtain approximate orientational distributions of the side chains and the adsorbed liquid crystal (LC) molecules on a rubbed side-chain polyimide surface. Both the side chains and the LC molecules appear to be well aligned in the rubbing direction but tilted away from the…

Liquid Crystal Research AdvancementsPhotonic Crystals and ApplicationsPhotochemistry and Electron Transfer Studies

NMR as a local probe of magnetic anisotropy: The possibility of orbital ordering and orbital liquid states in colossal magnetoresistance manganites

M. Belesi、G. C. Papavassiliou、M. Fardis 等 6 位作者2001-04-23Physical review. B, Condensed matter

${}^{139}\mathrm{La}$ rf enhancement experiments are shown to be an excellent tool for detecting changes of the local magnetic anisotropy in colossal magnetoresistance manganites. Based on this, we discuss the possibility of orbital ordering in ferromagnetic (FM) ${\mathrm{La}}_{1\ensuremath{-}x}{\mathrm{Ca}}_{x}{\mat…

Magnetic and transport properties of perovskites and related materialsRare-earth and actinide compoundsAdvanced Condensed Matter Physics

In‐plane birefringence and elongation behavior of uniaxially drawn aromatic polyimide films

Shinji Ando、Takashi Sawada、Shigekuni Sasaki2001-04-23Polymers for Advanced Technologies

Abstract Six kinds of aromatic poly(amic acid) films, the precursor of polyimides, were uniaxially drawn by constant loads during thermal curing with varying the final curing temperature and the load. The in‐plane birefringence (Δn) generated by uniaxial orientation of polyimide molecules in the film plane was investi…

Epoxy Resin Curing ProcessesSynthesis and properties of polymersSilicone and Siloxane Chemistry

Structural Investigations on Smectic Blue Phases

Eric Grelet、Brigitte Pansu、Min‐Hui Li 等 4 位作者2001-04-23Physical Review Letters

Smectic blue phases ( BP(Sm)) are thermotropic liquid crystalline phases which exhibit both three-dimensional orientational order, such as classical blue phases, and smectic positional order. BP(Sm) appear as the three-dimensional counterpart of twist grain boundary phases. X-ray scattering and optical polarizing micr…

Liquid Crystal Research AdvancementsMaterial Dynamics and PropertiesPhotonic Crystals and Applications

Local structure of Ge nanoislands on Si(111) surfaces with a SiO2 coverage

Alexander V. Kolobov、A. A. Shklyaev、H. Ōyanagi 等 6 位作者2001-04-23Applied Physics Letters

We have investigated the local structure and photoluminescence properties of ultrasmall Ge islands grown on Si(111) covered with SiO2. Scanning electron microscopy and transmission electron microscopy measurements show that the islands have a hemispherical shape, and depending on the growth temperature, can be either…

Semiconductor materials and devicesSilicon Nanostructures and PhotoluminescenceSemiconductor materials and interfaces

Dielectric properties of strained (Ba, Sr)TiO3 thin films epitaxially grown on Si with thin yttria-stabilized zirconia buffer layer

Sungjin Jun、Young Sung Kim、Jaichan Lee 等 4 位作者2001-04-23Applied Physics Letters

We have grown epitaxial (Ba0.5, Sr0.5)TiO3 (BST) thin films on Si with very thin yttria-stabilized zirconia (YSZ) buffer layer. The thin YSZ buffer layer affects the stress state of the epitaxial BST layer as well as the growth behavior of the BST layer, i.e., the degree of epitaxy. The epitaxial BST films grown on Si…

Ferroelectric and Piezoelectric MaterialsSemiconductor materials and devicesElectronic and Structural Properties of Oxides

Temperature dependence of excitonic absorption spectra in ZnO/Zn0.88Mg0.12O multiquantum wells grown on lattice-matched substrates

Handong Sun、T. Makino、N. T. Tuan 等 8 位作者2001-04-23Applied Physics Letters

The excitonic properties of high-quality ZnO/Zn0.88Mg0.12O multiquantum wells grown by laser-molecular-beam epitaxy were investigated using temperature-dependent optical absorption spectra from 5 K to room temperature. The strength of exciton-longitudinal-optical (LO) -phonon coupling was deduced from the temperature…

ZnO doping and propertiesPerovskite Materials and ApplicationsChalcogenide Semiconductor Thin Films