Materials Literature
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High quantum yield, low transverse energy spread and prompt response time make GaAs activated to negative electron affnity, an ideal candidate for a photocathode in high brightness photoinjectors. Even after decades of investigation, the exact mechanism of electron emission from GaAs is not well understood. We show th…
PART I: Introduction WHY ARE GREEN POLYMERIZATION METHODS RELEVANT TO SOCIETY, INDUSTRY, AND ACADEMICS? Status and Outlook for Environmentally Benign Processes Importance of Catalysis Brief Summaries of Contributions PART II: Integration of Renewable Starting Materials PLANT OILS AS RENEWABLE FEEDSTOCK FOR POLYMER SCI…
In the two-dimensional case the transition between ordinary and topological insulator states can be described by a massive Dirac model with the mass term changing its sign at the transition point. We theoretically investigate how such a transition manifests itself in resonant transport via localized helical edge state…
Constraint of the growth directions or exposed facets of nano-/microstructures has been long regarded as a popular research topic due to the various anisotropic properties of crystals. We report here, for the first time, not only uniform and phase-pure but also tunable perovskite BiFeO 3 crystallites with different pr…
Direct observation of light elements (Li and O) in oxygen-deficient lithium manganese spinel by spherical aberration-corrected scanning transmission electron microscopy is reported. A previously unknown ordered structure was revealed by annular dark-field (ADF) imaging of oxygen columns, while Li ions are visualized s…
We propose a type of elastic metamaterial comprising fluid-solid composite inclusions which can possess negative shear modulus and negative mass density over a large frequency region. Such a solid metamaterial has a unique elastic property that only transverse waves can propagate with a negative dispersion while longi…
We develop a new chemical route to prepare carbon nanotubes at room temperature. Graphite powder is immersed in a mixed solution of nitric and sulfuric acid with potassium chlorate. After heating the solution up to 70°C and leaving them in the air for 3 days, we obtained carbon nanotube bundles. This process could pro…
A study of high pressure solid Te was carried out at room temperature using Raman spectroscopy and Density Functional Theory (DFT) calculations. The analysis of the P-dependence of the experi- mental phonon spectrum reveals the occurrence of phase transitions at 4 GPa and 8 GPa confirming the high-pressure scenario re…
We report on experiments conducted on single walled carbon nanotube bundles aligned in chains and connected through a natural contact barrier. The dependence upon the temperature of the transport properties is investigated for samples having different characteristics. Starting from two bundles separated by one barrier…
Novel polydiolcitrate elastomers with thermally induced shape-memory properties are synthesized. These thermoresponsive polymers can be prepared as films or porous 3D sponges. Above their transition temperature, these materials display an elastomeric behavior, but below their transition temperature they have a glassy…
A biocompatible, robust polymer micelle bearing pH-hydrolyzable shell cross-links was developed for efficient intracellular delivery of doxorubicin (DOX). The rationally designed triblock copolymer of poly(ethylene glycol)-poly(L-aspartic acid)-poly(L-phenylalanine) (PEG-PAsp-PPhe) self-assembled to form polymer micel…
A relation derived from the Kubo formula shows that optical conductivity measurements below the gap frequency in doped semiconductors can be used to probe directly the time-dependent quantum dynamics of charge carriers. This allows to extract fundamental quantities such as the elastic and inelastic scattering rates, a…
Though graphene has been intensively studied by Raman spectroscopy, in this letter, we report a study of the second-order overtone and combination Raman modes in a mostly unexplored frequency range of 1690-2150 cm(-1) in nonsuspended commensurate (AB-stacked), incommensurate (folded) and suspended graphene layers. On…
Thermally induced spin transport in magnetized zigzag graphene nanoribbons (M-ZGNRs) is explored using first-principles calculations. By applying temperature difference between the source and the drain of a M-ZGNR device, spin-up and spin-down currents flowing in opposite directions can be induced. This spin Seebeck e…
Despite intense research efforts by research groups worldwide, the potential of self-assembled nanocrystal superlattices (NCSLs) has not been realized due to an incomplete understanding of the fundamental molecular interactions governing the self-assembly process. Because NCSLs reside naturally at length-scales betwee…
BACKGROUND: Engineered nanomaterials display unique properties that may have impact on human health, and thus require a reliable evaluation of their potential toxicity. Here, we performed a standardized in vitro screening of 23 engineered nanomaterials. We thoroughly characterized the physicochemical properties of the…
We demonstrate the use of high-resolution electron beam lithography to fabricate complex nanocavities with nanometric spatial and positional control. The plasmon modes of these nanostructures are then mapped using electron energy-loss spectroscopy in a scanning transmission electron microsope. This powerful combinatio…
A switchable magnetic metamaterial is demonstrated via reshaping micromachined metamaterial molecules. It is experimentally verified that the effective permeability can be switched from negative to positive near the resonant frequency. The micromachining technology offers a powerful platform for switchable metamateri…
Superparamagnetic Fe(3)O(4) nanoparticles prepared by a classical coprecipitation method were used as the stabilizer to prepare magnetic Pickering emulsions, and the effects of particle concentration, oil/water volume ratio, and oil polarity on the type, stability, composition, and morphology of these functional emuls…
We present a comprehensive experimental study of the optical properties of plasmonic oligomers. We show that both the constitution and configuration of plasmonic oligomers have a large influence on their resonant behavior, which draws a compelling analogy to molecular theory in chemistry. To elucidate the constitution…