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Excitonic Properties and Near‐Infrared Coherent Random Lasing in Vertically Aligned CdSe Nanowires

Rui Chen、M. Iqbal Bakti Utama、Zeping Peng 等 6 位作者2011-02-15Advanced Materials

High-quality, vertically aligned CdSe nanowires (figure, top left) are prepared by the vapor transport growth technique. Strong free-exciton absorption and emission are observed (top right) and, under optical excitation, near-infrared coherent random lasing is demonstrated for the first time from CdSe nanowires at roo…

Semiconductor Quantum Structures and DevicesQuantum Dots Synthesis And PropertiesRandom lasers and scattering media

Nanoparticle-Functionalized Porous Polymer Monolith Detection Elements for Surface-Enhanced Raman Scattering

Jikun Liu、Ian M. White、Don L. DeVoe2011-02-15Analytical Chemistry

The use of porous polymer monoliths functionalized with silver nanoparticles is introduced in this work for high-sensitivity surface-enhanced Raman scattering (SERS) detection. Preparation of the SERS detection elements is a simple process comprising the synthesis of a discrete polymer monolith section within a silica…

Gold and Silver Nanoparticles Synthesis and ApplicationsAdvanced biosensing and bioanalysis techniquesBiosensors and Analytical Detection

Mutual Ferromagnetic–Ferroelectric Coupling in Multiferroic Copper‐Doped ZnO

Tun Seng Herng、Meng Fei Wong、Dongchen Qi 等 17 位作者2011-02-15Advanced Materials

A mutual ferromagnetic and ferroelectric coupling (multiferroic behavior) in Cu-doped ZnO is demonstrated via deterministic control of Cu doping and defect engineering. The coexistence of multivalence Cu ions and oxygen vacancies is important to multiferroic behaviors in ZnO:Cu. The samples show clear ferroelectric an…

Ferroelectric and Piezoelectric MaterialsMultiferroics and related materialsAdvanced Condensed Matter Physics

Spin dynamics in the strong spin-orbit coupling regime

Xin Liu、Xiong-Jun Liu、Jairo Sinova2011-02-15arXiv

We study the spin dynamics in a high-mobility two dimensional electron gas (2DEG) with generic spin-orbit interactions (SOIs). We derive a set of spin dynamic equations which capture the purely exponential to the damped oscillatory spin evolution modes observed in different regimes of SOI strength. Hence we provide a…

Materials Science

Morphological Transformation between Nanofibers and Vesicles in a Controllable Bipyridine–Tripeptide Self‐Assembly

Damei Ke、Chuanlang Zhan、Alexander D. Q. Li 等 4 位作者2011-02-15Angewandte Chemie International Edition

Tuning structures: Stimulus-responsive peptide self-assembly requires a balance of conformational change and structural continuity of stable β sheets. In an amphiphilic bipyridine–tripeptide model, temperature, and ultrasound switch a reversible morphological transformation between vesicles and nanofibers (see picture…

Advanced biosensing and bioanalysis techniquesSupramolecular Self-Assembly in MaterialsPolydiacetylene-based materials and applications

High-Quality Graphene p−n Junctions via Resist-free Fabrication and Solution-Based Noncovalent Functionalization

Hung‐Chieh Cheng、Ren-Jye Shiue、Chia-Chang Tsai 等 5 位作者2011-02-15ACS Nano

An essential issue in graphene nanoelectronics is to engineer the carrier type and density and still preserve the unique band structure of graphene. We report the realization of high-quality graphene p-n junctions by noncovalent chemical functionalization. A generic scheme for the graphene p-n junction fabrication is…

Carbon Nanotubes in CompositesGraphene research and applicationsQuantum and electron transport phenomena

Growth from Below: Graphene Bilayers on Ir(111)

Shu Nie、Andrew L. Walter、N. C. Bartelt 等 7 位作者2011-02-15ACS Nano

We elucidate how graphene bilayers form on Ir(111). Low-energy electron diffraction (LEED) reveals that the two graphene layers are not always rotationally aligned. Monitoring this misalignment during growth shows that second-layer islands nucleate between the existing layer and the substrate. This mechanism occurs bo…

Advancements in Battery MaterialsGraphene research and applicationsQuantum and electron transport phenomena

Excitonic Fano Resonance in Free-Standing Graphene

Dong-Hun Chae、Tobias Utikal、Siegfried Weisenburger 等 7 位作者2011-02-15Nano Letters

We investigate the role of electron-hole correlations in the absorption of free-standing monolayer and bilayer graphene using optical transmission spectroscopy from 1.5 to 5.5 eV. Line shape analysis demonstrates that the ultraviolet region is dominated by an asymmetric Fano resonance. We attribute this to an excitoni…

Graphene research and applicationsPlasmonic and Surface Plasmon ResearchStrong Light-Matter Interactions

Synthesis of Si Nanosheets by a Chemical Vapor Deposition Process and Their Blue Emissions

Ungkil Kim、Ilsoo Kim、Yonghee Park 等 9 位作者2011-02-15ACS Nano

We synthesized free-standing Si nanosheets (NSs) with a thickness of about <2 nm using a chemical vapor deposition process and studied their optical properties. The Si NSs were formed by the formation of frameworks first along six different <110> directions normal to [111], its zone axis, and then by filling the space…

Semiconductor materials and devicesSilicon Nanostructures and PhotoluminescenceNanowire Synthesis and Applications

Temperature and voltage driven tunable metal-insulator transition in individualWxV1−xO2nanowires

Tai-Lung Wu、Luisa Whittaker‐Brooks、Sarbajit Banerjee 等 4 位作者2011-02-15Physical Review B

Results from transport measurements in individual ${\mathrm{W}}_{x}$V${}_{1\ensuremath{-}x}$O${}_{2}$ nanowires with varying extents of $W$ doping are presented. An abrupt thermally driven metal-insulator transition (MIT) is observed in these wires and the transition temperature decreases with increasing W content at…

ZnO doping and propertiesTransition Metal Oxide NanomaterialsGa2O3 and related materials

Amorphous silicon under mechanical shear deformations: shear velocity and temperature effects

Ali Kerrache、Normand Mousseau、Laurent J. Lewis2011-02-15arXiv

Mechanical shear deformations lead, in some cases, to effects similar to those resulting from ion irradiation. Here we characterize the effects of shear velocity and temperature on amorphous silicon (\aSi) modelled using classical molecular dynamics simulations based on the empirical Environment Dependent Inter-atomic…

Materials Science

Super Deformability and Young’s Modulus of GaAs Nanowires

Yan‐Bo Wang、Lifeng Wang、Hannah J. Joyce 等 11 位作者2011-02-15Advanced Materials

A significant size effect on the mechanical properties of GaAs nanowires (NWs) is reported. A remarkable elastic strain of ≈11% for NWs with diameters of 50–150 nm and obvious plastic deformation in NWs with diameters ≤25 nm are revealed. The Young’s modulus of the NWs can be more than double that of bulk GaAs.

Metal and Thin Film MechanicsNanowire Synthesis and ApplicationsBoron and Carbon Nanomaterials Research

Field electron emission characteristic of graphene

Weiliang Wang、Xizhou Qin、Ningsheng Xu 等 4 位作者2011-02-15Journal of Applied Physics

The field electron emission current from graphene is calculated analytically on a semiclassical model. The unique electronic energy band structure of graphene and the field penetration in the edge from which electrons emit have been taken into account. The relation between the effective vacuum barrier height and the a…

Carbon Nanotubes in CompositesGraphene research and applicationsRadiation Effects in Electronics

Water Droplet Motion Control on Superhydrophobic Surfaces: Exploiting the Wenzel-to-Cassie Transition

Guangming Liu、Lan Fu、Andrei V. Rode 等 4 位作者2011-02-15Langmuir

Water droplets on rough hydrophobic surfaces are known to exist in two states; one in which the droplet is impaled on the surface asperities (Wenzel state) and the other, a superhydrophobic state in which air remains trapped beneath the droplet (Cassie state). Here, we demonstrate that water droplets can transit from…

Surface Modification and SuperhydrophobicityFluid Dynamics and Heat TransferAdhesion, Friction, and Surface Interactions

Bio‐inspired Heterostructured Bead‐on‐String Fibers That Respond to Environmental Wetting

Xuelin Tian、Hao Bai、Yongmei Zheng 等 4 位作者2011-02-15Advanced Functional Materials

Abstract Inspired by the geometric structure of ecribellate spider capture silk and its spinning characteristics, we propose a one‐step electrohydrodynamic method to fabricate bead‐on‐string heterostructured fibers (BSHFs). By combining electrospinning and electrospraying strategies using a sprayable outer fluid with…

Surface Modification and SuperhydrophobicityElectrospun Nanofibers in Biomedical ApplicationsAdvanced Materials and Mechanics

Small Hysteresis Nanocarbon-Based Integrated Circuits on Flexible and Transparent Plastic Substrate

Woo Jong Yu、Si Young Lee、Sang Hoon Chae 等 7 位作者2011-02-15Nano Letters

We report small hysteresis integrated circuits by introducing monolayer graphene for the electrodes and a single-walled carbon nanotube network for the channel. Small hysteresis of the device originates from a defect-free graphene surface, where hysteresis was modulated by oxidation. This uniquely combined nanocarbon…

Carbon Nanotubes in CompositesGraphene research and applicationsNanowire Synthesis and Applications

Active protein aggregates induced by terminally attached self-assembling peptide ELK16 in Escherichia coli

Wei Wu、Lei Xing、Bihong Zhou 等 4 位作者2011-02-15Microbial Cell Factories

BACKGROUND: In recent years, it has been gradually realized that bacterial inclusion bodies (IBs) could be biologically active. In particular, several proteins including green fluorescent protein, β-galactosidase, β-lactamase, alkaline phosphatase, D-amino acid oxidase, polyphosphate kinase 3, maltodextrin phosphoryla…

Monoclonal and Polyclonal Antibodies ResearchBacteriophages and microbial interactionsSupramolecular Self-Assembly in Materials

Combining Surface Plasmon Resonance (SPR) Spectroscopy with Surface-Enhanced Raman Scattering (SERS)

Stefan Meyer、Eric C. Le Ru、P. Etchegoin2011-02-15Analytical Chemistry

The simultaneous measurement of surface plasmon resonance (SPR) spectroscopy and surface-enhanced Raman scattering (SERS) on flat metallic surfaces is demonstrated on a relatively simple experimental setup based on the Kretschmann configuration. This setup requires only minor modifications to standard Raman microscope…

Gold and Silver Nanoparticles Synthesis and ApplicationsAdvanced biosensing and bioanalysis techniquesPlasmonic and Surface Plasmon Research

XPS Analysis of Combustion Aerosols for Chemical Composition, Surface Chemistry, and Carbon Chemical State

Randy L. Vander Wal、Vicky M. Bryg、Michael D. Hays2011-02-15Analytical Chemistry

Carbonaceous aerosols can vary in elemental content, surface chemistry, and carbon nano-structure. Each of these properties is related to the details of soot formation. Fuel source, combustion process (affecting formation and growth conditions), and postcombustion exhaust where oxidation occurs all contribute to the p…

Advanced Chemical Physics StudiesCatalytic Processes in Materials ScienceCatalysis and Oxidation Reactions

Electronic structure of fully epitaxial Co2TiSn thin films

Markus Meinert、J. Schmalhorst、Hendrik Wulfmeier 等 7 位作者2011-02-15Physical Review B

We report on the properties of thin films of the full Heusler compound Co${}_{2}$TiSn prepared by dc magnetron co-sputtering. Fully epitaxial, stoichiometric films were obtained by deposition on MgO (001) substrates at substrate temperatures above ${600}^{\ifmmode^\circ\else\textdegree\fi{}}$C. The films are well orde…

2D Materials and ApplicationsMXene and MAX Phase MaterialsHeusler alloys: electronic and magnetic properties