Materials Literature
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A ball-bearing structure based triboelectric nanogenerator (B-TENG) with interdigitative-electrodes was developed that can not only collect energy from rotational kinetic energy, but also serve as a self-powered and multifunctional sensor. The B-TENG relies on the rolling electrification between PTFE balls on Cu inter…
Abstract The encapsulation of metal nanoparticles (MNPs) within metal–organic frameworks (MOFs) to form core–shell structural nanocomposites is one of the most promising methods to enhance the durability and selectivity of MOF‐supported metal catalysts. However, it is still a challenge to fully encapsulate tiny MNPs i…
The efficiency roll‐off in blue phosphorescent organic light emitting diodes (OLEDs) using different carbazole compounds as the host is systematically studied. While there is no significant difference in device efficiency, OLEDs using ter‐carbazole as the host show a reduction in efficiency roll‐off at high luminance.…
Color printing technology is developing rapidly; in less than 40 years, it moved from dot matrix printers with an ink-soaked cloth ribbon to 3D printers used to make three-dimensional color objects. Nevertheless, what remained unchanged over this time is the fact that in each case, dye inks (CMYK or RGB color schemes)…
BACKGROUND: Water-soluble form of fullerene C60 is a promising tool for the control of ROS-dependent inflammation including allergic diseases. Anti-inflammatory effects of C60 (nC60) aqueous dispersion were evaluated in the mouse models of atopic dermatitis using subcutaneous (SC) and epicutaneous (EC) applications du…
Periodic nanocone–nanopillar dual-structured arrays are wet chemical etched on 20 μm-thick crystalline silicon substrates, enabling the realization of excellent light absorption properties and enhanced electrical contact with PEDOT:PSS. The finally textured silicon/PEDOT:PSS thin film hybrid solar cell shows a power c…
Abstract Peptide‐tuned self‐assembly of functional components offers a strategy towards improved properties and unique functions of materials, but the requirement of many different functions and a lack of understanding of complex structures present a high barrier for applications. Herein, we report a photosensitive dr…
Spatial positioning of nanocrystal building blocks on a solid surface is a prerequisite for assembling individual nanoparticles into functional devices. Here, we report on the graphoepitaxial liquid-solid growth of nanowires of the photovoltaic compound CH3NH3PbI3 in open nanofluidic channels. The guided growth, visua…
Poly(vinyl caprolactam) (PNVCL) is one of the most important thermoresponsive polymers because it is similar to poly(N-isopropyl acrylamide). PNVCL precipitates from aqueous solutions in a physiological temperature range (32⁻34 °C). The use of PNVCL instead of PNIPAM is considered advantageous because of the assumed l…
Identification of specific operating mechanisms becomes particularly challenging when mixed ionic-electronic conductors are used in optoelectronic devices. Ionic effects in perovskite solar cells are believed to distort operation curves and possess serious doubts about their long term stability. Current hysteresis and…
Resolution in the X-ray structure determination of noncrystalline samples has been limited to several tens of nanometers, because deep X-ray irradiation required for enhanced resolution causes radiation damage to samples. However, theoretical studies predict that the femtosecond (fs) durations of X-ray free-electron l…
The elucidation of formation mechanisms is mandatory for understanding and planning of synthetic routes. For (bio-)organic and organometallic compounds, this has long been realized even for very complicated molecules, whereas the formation of ligand-free inorganic molecules has widely remained a black box to date. Thi…
Oriented nano-microstructure-assisted controllable fabrication, a facile and versatile preparation strategy, is developed to fabricate metal-organic framework (MOF) membranes. With this method, several MOF membranes with tailored structures are prepared, including HKUST-1 (with 3D pores) and M3 (HCOO)6 (with 1D pores;…
The adsorption mechanism of ethane, ethylene, and acetylene (C 2 H n; n = 2, 4, 6) on two microporous metal organic frameworks (MOFs) is described here that is consistent with observations from single crystal and powder X-ray diffraction, calorimetric measurements, and gas adsorption isotherm measurements. Two calcium…
Surface properties of refractory ceramic transition metal nitride thin films grown by magnetron sputtering are essential for resistance towards oxidation necessary in all modern applications. Here, typically neglected factors, including exposure to residual process gases following the growth and the venting temperatur…
Understanding the interfacial electronic structures of heterojunctions, a challenging undertaking, is extremely important to the design of photoelectrodes for efficient water splitting. The heterostructured interfaces in terms of crystal defects at the atomic‐level exemplified by TiO 2 /BiVO 4 are studied. Results fro…
We describe the modular synthesis of three novel large N-heteroarenes, containing 9, 11, and 13 annulated rings. This modular system features fused azaacene units to a coronene nucleus. We evaluate the optical and electronic properties and the solid-state packing of the targets. The electronic properties of the 13-rin…
A robust silicon electrode for lithium-ion battery has been developed via prepolymerizing dopamine on silicon particle surface and then chemical binding with poly(acrylic acid) (PAA). In this favorable electrode, silicon nanoparticles are covered by a thin layer of polydopamine (PD) through firm hydrogen bonds between…
Neutron diffraction under operando battery cycling is used to study the lithium and oxygen dynamics of high Li‐rich Li(Lix/3Ni(3/8‐3x/8)Co(1/4‐x/4)Mn(3/8+7x/24)O2 (x = 0.6, HLR) and low Li‐rich Li(Lix/3Ni(1/3‐x/3)Co(1/3‐x/3)Mn(1/3+x/3)O2 (x = 0.24, LLR) compounds that exhibit different degrees of oxygen activation at…
Nature often exhibits various interesting and unique adhesive surfaces. The attempt to understand the natural adhesion phenomena can continuously guide the design of artificial adhesive surfaces by proposing simplified models of surface adhesion. Among those models, a peeling model can often effectively reflect the ad…