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Effect of initial properties on the flow strength of aluminum during quasi-isentropic compression

J. R. Asay、Tommy Ao、Jean‐Paul Davis 等 6 位作者2008-04-15Journal of Applied Physics

A magnetic loading technique was used to ramp load pure aluminum and 6061 aluminum alloy to peak stresses of approximately 29GPa. The peak loading rate was approximately 106∕s, followed by unloading from peak stress at a rate of about 105∕s. The pure aluminum samples had impurity levels ranging from about 10ppmto0.5wt…

High-pressure geophysics and materialsEnergetic Materials and CombustionHigh-Velocity Impact and Material Behavior

Annealing effects on Czochralski grown Lu2Si2O7:Ce3+ crystals under different atmospheres

Feng He、Dongzhou Ding、Huanying Li 等 7 位作者2008-04-15Journal of Applied Physics

Cerium-doped lutetium pyrosilicate Lu2Si2O7:Ce3+ (LPS:Ce) single crystal samples grown via Czochralski method were annealed under air and H2 atmospheres from 350to1600°C. The x-ray excited luminescence spectra and UV as well as thermal stimulated luminescence spectra were measured. It was found that the luminescence e…

Luminescence Properties of Advanced MaterialsRadiation Detection and Scintillator TechnologiesNuclear materials and radiation effects

Amyloide: nicht nur pathologische Substanzen, sondern auch geordnete Nanomaterialien

Izhack Cherny、Ehud Gazit2008-04-15Angewandte Chemie

Abstract Amyloidfasern gehören zu den wichtigsten selbstorganisierten Strukturen in der Natur. Zahlreiche Proteine und Peptide mit unterschiedlichen Aminosäuresequenzen bilden unter verschiedenen Bedingungen solche sehr stabilen und hochgradig organisierten Assoziate, die man in Phasenzuständen von Flüssigkristallen b…

Alzheimer's disease research and treatmentsSupramolecular Chemistry and ComplexesSupramolecular Self-Assembly in Materials

Negative-zero-positive metamaterial with omega-type metal inclusions

Fuli Zhang、Grégory Houzet、Éric Lheurette 等 6 位作者2008-04-15Journal of Applied Physics

We report on a negative-zero-positive metamaterial based on an omega-type microstructure with special attention on the nonvanishing group velocity for a zero refractive index. We first investigate the dispersion characteristics by full wave analysis, by stressing the necessary conditions of equality between the electr…

Antenna Design and AnalysisMetamaterials and Metasurfaces ApplicationsAdvanced Antenna and Metasurface Technologies

Metal−Carbon Nanotube Contacts: The Link between Schottky Barrier and Chemical Bonding

V. Vitale、Alessandro Curioni、Wanda Andreoni2008-04-15Journal of the American Chemical Society

The field effect transistor based on carbon nanotubes (CNT) is a very promising candidate for post-CMOS microelectronics. Transport in the CNT channel is dominated by the Schottky barriers existing at the metal source contacts. The nature of the metal and the geometry of the contact appear to influence strongly the el…

Carbon Nanotubes in CompositesGraphene research and applicationsSemiconductor materials and interfaces

Interfacial structure and defect analysis of nonpolar ZnO films grown on R-plane sapphire by molecular beam epitaxy

P. Vennéguès、J.‐M. Chauveau、M. Korytov 等 6 位作者2008-04-15Journal of Applied Physics

The interfacial relationship and the microstructure of nonpolar (11−20) ZnO films epitaxially grown on (1−102) R-plane sapphire by molecular beam epitaxy are investigated by transmission electron microscopy. The already-reported epitaxial relationships [1−100]ZnO∥[11−20]sapphire and ⟨0001⟩ZnO∥[−1101]sapphire are confi…

ZnO doping and propertiesGaN-based semiconductor devices and materialsGa2O3 and related materials

Anisotropic optical emission of single CdSe/CdS tetrapod heterostructures: Evidence for a wavefunction symmetry breaking

Christian Mauser、Thomas Limmer、Enrico Da Como 等 7 位作者2008-04-15Physical Review B

Semiconductor tetrapods are expected to exhibit isotropic optical properties due to their tetrahedral symmetry. We have investigated the optical polarization properties of individual $\mathrm{Cd}\mathrm{Se}∕\mathrm{Cd}\mathrm{S}$ tetrapods of high structural quality. In contrast to the light absorption behavior, a pro…

Quantum Dots Synthesis And PropertiesChalcogenide Semiconductor Thin FilmsAdvanced Semiconductor Detectors and Materials

Defects in nematic membranes can buckle into pseudospheres

John R. Frank、Mehran Kardar2008-04-15Physical Review E

Many factors influence the shapes of living and manufactured membranes. In addition to boundary conditions, surface tension, and curvature, the ordering of particles embedded in or attached to a membrane can strongly influence its equilibrium shape. As a simple model of such ordering, we consider rodlike particles tha…

Liquid Crystal Research AdvancementsMicro and Nano RoboticsAdvanced Materials and Mechanics

Sensitivity of porous silicon rugate filters for chemical vapor detection

Mohamed Shaker Salem、Michael J. Sailor、Kazuhiro Fukami 等 5 位作者2008-04-15Journal of Applied Physics

The characteristics of chemical vapor sensors constructed from porous Si rugate filters are examined. The peak position of the resonant wavelength exhibits a redshift response upon exposure to ethanol vapors. The filter response scales with the vapor partial pressure; the concentration level is estimated based on theo…

Photonic and Optical DevicesPhotonic Crystals and ApplicationsSilicon Nanostructures and Photoluminescence

Capturing Transient Structures in the Elimination Reaction of Haloalkane in Solution by Transient X-ray Diffraction

Jae Hyuk Lee、Tae Kyu Kim、Joonghan Kim 等 8 位作者2008-04-15Journal of the American Chemical Society

This Communication reports simultaneous tracking of structural and kinetic information for the photoinduced elimination reaction of 1,2-diiodotetrafluoroethane in solution by transient X-ray diffraction. The transient structure of .CF2CF2I is determined to be a classical mixture whereas .CH2CH2I is bridged. Compared w…

Advanced Chemical Physics StudiesAnalytical Chemistry and ChromatographyCrystallization and Solubility Studies

Structural, electronic and magnetic properties of manganese doping in the upper layer of bilayer graphene

Yuliang Mao、Jianxin Zhong2008-04-15Nanotechnology

First-principles spin-polarized calculations have been conducted to investigate the structural, electronic and magnetic properties of 3d transition metal Mn doping into two typical sites in the upper layer of bilayer graphene with the AB Bernal structure. One of the doping sites is above the center of a carbon hexagon…

Advancements in Battery MaterialsGraphene research and applicationsQuantum and electron transport phenomena

Size‐Controlled Ex‐nihilo Ferromagnetism in Capped CdSe Quantum Dots

M. S. Seehra、Prasanta Dutta、S. Neeleshwar 等 9 位作者2008-04-15Advanced Materials

Hysteresis loops in D = 1.8 nm CdSe-TOPO nanoparticles show ferromagnetism at 5 K and 300 K. Charge transfer from Cd to the Cd–O bond is shown by arrow in the Fourier transforms amplitudes of the EXAFS k2χ data at the Cd K-edge in the smaller 2.8 and 4.1 nm particles. This charge transfer produces holes in the Cd 4d b…

ZnO doping and propertiesQuantum Dots Synthesis And PropertiesChalcogenide Semiconductor Thin Films

Single-Molecule Magnets: A Family of MnIII/CeIV Complexes with a [Mn8CeO8]12+ Core

Abhudaya Mishra、Anastasios J. Tasiopoulos、Wolfgang Wernsdorfer 等 8 位作者2008-04-15Inorganic Chemistry

Four heterometallic, enneanuclear Mn8Ce clusters [Mn8CeO8(O2CMe)12(H2O)4] (4), [Mn8CeO8(O2CMe)12(py)4] (5), [Mn8CeO8(O2CPh)12(MeCN)4] [Mn8CeO8(O2CPh)12(dioxane)4] (6), and [Mn8CeO8(O2CCHPh2)12(H2O)4] (7) have been prepared by various methods. Their cores are essentially isostructural and comprise a nonplanar, saddleli…

Magnetism in coordination complexesLanthanide and Transition Metal ComplexesMetal-Catalyzed Oxygenation Mechanisms

Comparison of morphology and mechanical properties of PLGA bioscaffolds

Louis M. Leung、Carmen Chan、Sang Dae Baek 等 4 位作者2008-04-15Biomedical Materials

In this study, bioscaffolds using poly(DL-lactide-co-glycolide) acid (PLGA) were fabricated and studied. The gas foaming/salt leaching technique in a batch foaming setup was employed, and the effects of material composition of PLGA on the morphology and mechanical properties using this process were investigated. Two m…

Bone Tissue Engineering Materialsbiodegradable polymer synthesis and propertiesElectrospun Nanofibers in Biomedical Applications

Cylindrical Polymer Nanostructures by Solution Template Wetting

Stefanie Schlitt、Andreas Greiner、Joachim H. Wendorff2008-04-15Macromolecules

Wetting of porous templates, e.g., porous aluminum oxide with pore diameters in the range from 25 up to several 100 nm, by polymer melts has been demonstrated previously to be a highly effective way toward the preparation of polymer nanotubes. The concept evaluated in this contribution is to perform wetting from polym…

Surface Modification and SuperhydrophobicityNanopore and Nanochannel Transport StudiesAnodic Oxide Films and Nanostructures

Effects of blend composition and dynamic vulcanization on the morphology and dynamic viscoelastic properties of PP/EPDM blends

É. V. Prut、N.A. Erina、J. Karger‐Kocsis 等 4 位作者2008-04-15Journal of Applied Polymer Science

Abstract The morphology and dynamic viscoelastic properties of isotactic polypropylene (PP) blended with oil‐free/oil‐extended ethylene–propylene–diene (EPDM) rubbers were studied. Unvulcanized and dynamically vulcanized blends with the compositions PP/EPDM = 50/50 and = 30/70 were investigated. The morphology was obs…

Polymer crystallization and propertiesPolymer Nanocomposites and PropertiesRheology and Fluid Dynamics Studies

Er 3 + -doped boro-tellurite glass for optical amplification in the 1530–1580nm

Purushottam Joshi、Shaoxiong Shen、Animesh Jha2008-04-15Journal of Applied Physics

The paper investigates the influence of boric oxide (B2O3), which has a phonon energy of 1500cm−1, on enhancement in the population of the I13∕24 level via the increased multiphonon relaxation in the Er-ion doped tellurite fibers. The paper discusses the structural compatibility of TeO4 structures with BO4 structural…

Luminescence Properties of Advanced MaterialsGlass properties and applicationsSolid State Laser Technologies

Thermal conductivity of nitrogenated ultrananocrystalline diamond films on silicon

M. Shamsa、Subhajit Ghosh、Irene Calizo 等 6 位作者2008-04-15Journal of Applied Physics

The authors report on the experimental investigation of the thermal conductivity of nitrogenated ultrananocrystalline diamond (UNCD) films on silicon. For better accuracy, the thermal conductivity was measured by using two different approaches: the 3ω method and transient “hot disk” technique. The temperature dependen…

Metal and Thin Film MechanicsHigh-pressure geophysics and materialsDiamond and Carbon-based Materials Research

The Role of Surface Basal Planes of Layered Mixed Metal Oxides in Selective Transformation of Lower Alkanes: Propane Ammoxidation over Surface ab Planes of Mo−V−Te−Nb−O M1 Phase

N. Raveendran Shiju、Xin-Hua Liang、Alan W. Weimer 等 6 位作者2008-04-15Journal of the American Chemical Society

The surface ab planes of the M1 phase exposed selectively after atomic layer deposition (ALD) of alumina followed by crushing showed significantly improved selectivity to acrylonitrile during propane ammoxidation. The results demonstrated the importance of surface ab planes for the activity and selectivity of the M1 p…

Catalytic Processes in Materials ScienceCatalysis and Hydrodesulfurization StudiesCatalysis and Oxidation Reactions

Co‐expression of elastin and collagen leads to highly compliant engineered blood vessels

Jin Gao、Peter M. Crapo、Robert M. Nerem 等 4 位作者2008-04-15Journal of Biomedical Materials Research Part A

Elastin synthesis and physiologic compliance are significant challenges in blood vessel tissue engineering. Here, we report that a biocompatible elastomeric scaffold can support the co-expression of elastin and collagen, which likely yielded the physiologic compliance in the constructs. A biodegradable elastomer, poly…

Electrospun Nanofibers in Biomedical ApplicationsAortic aneurysm repair treatmentsConnective tissue disorders research